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Recently, the occurrence of fog and haze over China has increased. The retrieval of trace gases from the multi-axis differential optical absorption spectroscopy (MAX-DOAS) is challenging under these conditions. In this study, various reported retrieval settings for formaldehyde (HCHO) and sulfur dioxide (SO2) are compared to evaluate the performance of these settings under different meteorological conditions (clear day, haze, and fog). The dataset from 1st December 2019 to 31st March 2020 over Nanjing, China, is used in this study. The results indicated that for HCHO, the optimal settings were in the 324.5–359 nm wavelength window with a polynomial order of five. At these settings, the fitting and root mean squared (RMS) errors for column density were considerably improved for haze and fog conditions, and the differential slant column densities (DSCDs) showed more accurate values compared to the DSCDs between 336.5 and 359 nm. For SO2, the optimal settings for retrieval were found to be at 307–328 nm with a polynomial order of five. Here, root mean square (RMS) and fitting errors were significantly lower under all conditions. The observed HCHO and SO2 vertical column densities were significantly lower on fog days compared to clear days, reflecting a decreased chemical production of HCHO and aqueous phase oxidation of SO2 in fog droplets.
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Impact of the Eurasian Teleconnection on the Interannual Variability of Haze-Fog in Northern China in January
Using meteorological observation data and NCEP/NCAR (National Centers for Environmental Prediction/National Center for Atmospheric Research) reanalysis data, the impacts of the atmospheric circulation pattern on the interannual variability of haze-fog in northern China in January are studied by means of statistical methods. The results showed that the Eurasian teleconnection (EU) at the 500 hPa isostatic surface is the most important pattern affecting the haze-fog frequency in northern China. However, the existing EU index cannot perfectly describe this pattern. To this end, this study selects three main activity centers to define a new EU index, which are located in the Europe (10 °E, 55 °N), Siberia (80 °E, 60 °N), and Shandong, China (120 °E, 40 °N). The difference between the existing EU index and the new EU index is mainly the position of the anomaly center of the 500 hPa geopotential height. The EU is in a negative phase in higher haze-fog years but is in a positive phase in lower haze-fog years. The 500 hPa geopotential height shows negative anomalies in Europe and East Asian and a positive anomaly in Siberia in the negative EU phase. Using Plumb wave activity flux analysis, it was found that the cold wave affecting northern China is less in the negative EU phase than that in the positive EU phase, which resulted in more haze-fog days. In addition, the results also showed that the EU pattern goes through a considerable development and decay within 13 days. The visibility starts to significantly decrease at a lag of −1 to 2 days in the negative EU peak phase and is influenced by the weak north wind that is caused by the high pressure.
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- Award ID(s):
- 1743401
- PAR ID:
- 10132417
- Date Published:
- Journal Name:
- Atmosphere
- Volume:
- 10
- Issue:
- 3
- ISSN:
- 2073-4433
- Page Range / eLocation ID:
- 113
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.3390/atmos10030113
