Extremely high beam-to-radiation energy conversion efficiencies can be obtained in a THz FEL using a strongly tapered helical undulator at the zero-slippage resonant condition, where a circular waveguide is used to match the radiation group velocity to the electron beam longitudinal velocity. In this paper we report on the first electro-optic sampling (EOS) based measurements of the broadband THz FEL radiation pulses emitted in this regime. The THz field waveforms are reconstructed in the spatial and temporal domains using multi-shot and single-shot EOS schemes respectively. The measurements are performed varying the input electron beam energy in the undulator providing insights on the complex dynamics in a waveguide FEL.
- Award ID(s):
- 1708006
- NSF-PAR ID:
- 10135167
- Date Published:
- Journal Name:
- 39th Free Electron Laser Conf./ FEL2019, Hamburg, Germany
- Page Range / eLocation ID:
- 282-287
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Constraints on the state of stress in the lithosphere are fundamental to understanding a breadth of geological phenomena. Paleo-stresses are generally estimated using microstructural elements for which there are experimentally calibrated relationships with applied stress, with an emphasis on recrystallised grain-size piezometers. However, it is often difficult to clearly distinguish newly recrystallised grains from the relict matrix. Furthermore, these grain-size piezometers are only applicable to rocks consisting of a single mineral. An alternative proxy for paleo-stress in polymineralic rocks is the average subgrain size. Unfortunately, estimates of subgrain size differ significantly among different measurement methods, and therefore, piezometers must be individually calibrated for the method used. Existing subgrain-size piezometers are based on calibrations using optical or transmission electron microscopy. We use electron backscatter diffraction (EBSD), a common method of subgrain-boundary characterisation, to calibrate subgrain-size piezometers for both olivine and quartz. To test the application of our olivine subgrain-size piezometer to polymineralic rocks, we deformed synthetic mixtures of olivine and orthopyroxene. Experiments were conducted using a Deformation-DIA apparatus at beamline 6BM-B Advanced Photon Source, Argonne National Laboratory. These experiments offer the unique possibility of simultaneously deforming the sample and measuring the average stresses within each phase using X-ray diffraction, before applying subgrain-size piezometry to the recovered samples. The results provide tests of (1) the manner in which stress is partitioned between phases, (2) whether the stresses measured in each phase by X-ray diffraction are comparable to those estimated by subgrain-size piezometry, and (3) whether stresses from subgrain piezometry can be used to estimate the macroscopic average applied stress. Stresses estimated from X-ray diffraction agree well with those made from subgrain-size piezometry in both monomineralic and polymineralic samples. In harzburgites, average stresses are similar in both phases and indicate that in this system, subgrain-size piezometric measurements from a single phase can be used to estimate the bulk stress.more » « less
-
Abstract The key to type 1 copper (T1Cu) function lies in the fine tuning of the CuII/Ireduction potential (
E °′T1Cu) to match those of its redox partners, enabling efficient electron transfer in a wide range of biological systems. While the secondary coordination sphere (SCS) effects have been used to tuneE °′T1Cuin azurin over a wide range, these principles are yet to be generalized to other T1Cu‐containing proteins to tune catalytic properties. To this end, we have examined the effects of Y229F, V290N and S292F mutations around the T1Cu of small laccase (SLAC) fromStreptomyces coelicolor to match the highE °′T1Cuof fungal laccases. Using ultraviolet‐visible absorption and electron paramagnetic resonance spectroscopies, together with X‐ray crystallography and redox titrations, we have probed the influence of SCS mutations on the T1Cu and correspondingE °′T1Cu. While minimal and smallE °′T1Cuincreases are observed in Y229F‐ and S292F‐SLAC, the V290N mutant exhibits a majorE °′T1Cuincrease. Moreover, the influence of these mutations onE °′T1Cuis additive, culminating in a triple mutant Y229F/V290N/S292F‐SLAC with the highestE °′T1Cuof 556 mV vs. SHE reported to date. Further activity assays indicate that all mutants retain oxygen reduction reaction activity, and display improved catalytic efficiencies (k cat/K M) relative to WT‐SLAC. -
Abstract The key to type 1 copper (T1Cu) function lies in the fine tuning of the CuII/Ireduction potential (
E °′T1Cu) to match those of its redox partners, enabling efficient electron transfer in a wide range of biological systems. While the secondary coordination sphere (SCS) effects have been used to tuneE °′T1Cuin azurin over a wide range, these principles are yet to be generalized to other T1Cu‐containing proteins to tune catalytic properties. To this end, we have examined the effects of Y229F, V290N and S292F mutations around the T1Cu of small laccase (SLAC) fromStreptomyces coelicolor to match the highE °′T1Cuof fungal laccases. Using ultraviolet‐visible absorption and electron paramagnetic resonance spectroscopies, together with X‐ray crystallography and redox titrations, we have probed the influence of SCS mutations on the T1Cu and correspondingE °′T1Cu. While minimal and smallE °′T1Cuincreases are observed in Y229F‐ and S292F‐SLAC, the V290N mutant exhibits a majorE °′T1Cuincrease. Moreover, the influence of these mutations onE °′T1Cuis additive, culminating in a triple mutant Y229F/V290N/S292F‐SLAC with the highestE °′T1Cuof 556 mV vs. SHE reported to date. Further activity assays indicate that all mutants retain oxygen reduction reaction activity, and display improved catalytic efficiencies (k cat/K M) relative to WT‐SLAC. -
Aims. We analyse particle, radio, and X-ray observations during the first relativistic proton event of solar cycle 25 detected on Earth. The aim is to gain insight into the relationship between relativistic solar particles detected in space and the processes of acceleration and propagation in solar eruptive events. Methods. To this end, we used ground-based neutron monitor measurements of relativistic nucleons and space-borne measurements of electrons with similar speed to determine the arrival times of the first particles at 1 AU and to infer their solar release times. We compared the release times with the time histories of non-thermal electrons in the solar atmosphere and their escape to interplanetary space, as traced by radio spectra and X-ray light curves and images. Results. Non-thermal electrons in the corona are found to be accelerated in different regions. Some are confined in closed magnetic structures expanding during the course of the event. Three episodes of electron escape to the interplanetary space are revealed by groups of decametric-to-kilometric type III bursts. The first group appears on the low-frequency side of a type II burst produced by a coronal shock wave. The two latter groups are accompanied at higher frequencies by bursts with rapid drifts to both lower and higher frequencies (forward- or reverse-drifting bursts). They are produced by electron beams that propagate both sunward and anti-sunward. The first relativistic electrons and nucleons observed near Earth are released with the third group of type III bursts, more than ten minutes after the first signatures of non-thermal electrons and of the formation of the shock wave in the corona. Although the eruptive active region is near the central meridian, several tens of degrees east of the footpoint of the nominal Parker spiral to the Earth, the kilometric spectrum of the type III bursts and the in situ detection of Langmuir waves demonstrate a direct magnetic connection between the L1 Lagrange point and the field lines onto which the electron beams are released at the Sun. Conclusions. We interpret the forward- and reverse-drifting radio bursts as evidence of reconnection between the closed expanding magnetic structures of an erupting flux rope and ambient open magnetic field lines. We discuss the origin of relativistic particles near the Earth across two scenarios: (1) acceleration at the CME-driven shock as it intercepts interplanetary magnetic field lines rooted in the western solar hemisphere and (2) an alternative where the relativistic particles are initially confined in the erupting magnetic fields and get access to the open field lines to the Earth through these reconnection events.more » « less