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Title: Superconducting phase diagram of H3S under high magnetic fields
Abstract

The discovery of superconductivity at 260 K in hydrogen-rich compounds like LaH10re-invigorated the quest for room temperature superconductivity. Here, we report the temperature dependence of the upper critical fieldsμ0Hc2(T) of superconducting H3S under a record-high combination of applied pressures up to 160 GPa and fields up to 65 T. We find thatHc2(T) displays a linear dependence on temperature over an extended range as found in multigap or in strongly-coupled superconductors, thus deviating from conventional Werthamer, Helfand, and Hohenberg (WHH) formalism. The best fit ofHc2(T) to the WHH formalism yields negligible values for the Maki parameterαand the spin–orbit scattering constantλSO. However,Hc2(T) is well-described by a model based on strong coupling superconductivity with a coupling constantλ~ 2. We conclude that H3S behaves as a strong-coupled orbital-limited superconductor over the entire range of temperatures and fields used for our measurements.

 
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NSF-PAR ID:
10153410
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ;
Publisher / Repository:
Nature Publishing Group
Date Published:
Journal Name:
Nature Communications
Volume:
10
Issue:
1
ISSN:
2041-1723
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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