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1. Efficient and highly tunable second-harmonic generation in Z-cut periodically poled lithium niobate nanowaveguides

   https://doi.org/10.1364/OL.393445  

   Chen, Jia-Yang ; Tang, Chao ; Ma, Zhao-Hui ; Li, Zhan ; Meng Sua, Yong ; Huang, Yu-Ping ( July 2020 , Optics Letters)

   Thin-film lithium-niobate-on-insulator (LNOI) has emerged as a superior integrated-photonics platform for linear, nonlinear, and electro-optics. Here we combine quasi-phase-matching, dispersion engineering, and tight mode confinement to realize nonlinear parametric processes with both high efficiency and wide wavelength tunability. On a millimeter-long, Z-cut LNOI waveguide, we demonstrate efficient ($1900\pm <\#comment/>500\mathrm{\%<\#comment/>}{\mathrm{W}}^{-<\#comment/>1}{\mathrm{c}\mathrm{m}}^{-<\#comment/>2}$) and highly tunable ($-<\#comment/>1.71\mathrm{n}\mathrm{m}/\mathrm{K}$) second-harmonic generation from 1530 to 1583 nm by type-0 quasi-phase-matching. Our technique is applicable to optical harmonic generation, quantum light sources, frequency conversion, and many other photonic information processes across visible to mid-IR spectral bands.
2. “Seeing Is Believing”—In-Depth Analysis by Co-Imaging of Periodically-Poled X-Cut Lithium Niobate Thin Films

   https://doi.org/10.3390/cryst11030288  

   Reitzig, Sven ; Rüsing, Michael ; Zhao, Jie ; Kirbus, Benjamin ; Mookherjea, Shayan ; Eng, Lukas M. ( March 2021 , Crystals)

   Nonlinear and quantum optical devices based on periodically-poled thin film lithium niobate (PP-TFLN) have gained considerable interest lately, due to their significantly improved performance as compared to their bulk counterparts. Nevertheless, performance parameters such as conversion efficiency, minimum pump power, and spectral bandwidth strongly depend on the quality of the domain structure in these PP-TFLN samples, e.g., their homogeneity and duty cycle, as well as on the overlap and penetration depth of domains with the waveguide mode. Hence, in order to propose improved fabrication protocols, a profound quality control of domain structures is needed that allows quantifying and thoroughly analyzing these parameters. In this paper, we propose to combine a set of nanometer-to-micrometer-scale imaging techniques, i.e., piezoresponse force microscopy (PFM), second-harmonic generation (SHG), and Raman spectroscopy (RS), to access the relevant and crucial sample properties through cross-correlating these methods. Based on our findings, we designate SHG to be the best-suited standard imaging technique for this purpose, in particular when investigating the domain poling process in x-cut TFLNs. While PFM is excellently recommended for near-surface high-resolution imaging, RS provides thorough insights into stress and/or defect distributions, as associated with these domain structures. In this context, our work here indicates unexpectedly largemore »signs for internal fields occurring in x-cut PP-TFLNs that are substantially larger as compared to previous observations in bulk LN.« less
3. Broadband ultraviolet-visible frequency combs from cascaded high-harmonic generation in quasi-phase-matched waveguides

   https://doi.org/10.1364/JOSAB.427086  

   Rutledge, Jay ; Catanese, Anthony ; Hickstein, Daniel D. ; Diddams, Scott A. ; Allison, Thomas K. ; Kowligy, Abijith S. ( July 2021 , Journal of the Optical Society of America B)

   High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to the ninth order (333 nm) in chirped periodically poled lithium niobate waveguides driven by phase-stable$\le <\#comment/>12\mathrm{n}\mathrm{J}$, 100 fs pulses at 3 µm with 100 MHz repetition rate. A mid-infrared to ultraviolet-visible conversion efficiency as high as 10% is observed, among an overall 23% conversion of the fundamental to all harmonics. We verify the coherence of the harmonic frequency combs despite the complex highly nonlinear process. Accommodating the extreme spectral bandwidth, numerical simulations based on a single broadband envelope equation with only quadratic nonlinearity give estimates for the conversion efficiency within approximately 1 order of magnitude over a wide range of experimental parameters. From this comparison between theory and experiment, we identify a dimensionless parameter capturing the competition between three-wave mixing and group-velocity walk-off of the harmonics that governs the cascaded HHG physics. We also gain insights into spectral optimization via tuning the waveguide poling profile and pump pulse parameters. These results can inform cascaded HHG in a range of different platforms.
4. Engineered second-order nonlinearity in silicon nitride

   https://doi.org/10.1364/OME.478811  

   Zhang, Yi ; Nauriyal, Juniyali ; Song, Meiting ; Granados Baez, Marissa ; He, Xiaotong ; Macdonald, Timothy ; Cardenas, Jaime ( December 2022 , Optical Materials Express)

   The lack of a bulk second-order nonlinearity (χ⁽²⁾) in silicon nitride (Si₃N₄) keeps this low-loss, CMOS-compatible platform from key active functions such as Pockels electro-optic (EO) modulation and efficient second harmonic generation (SHG). We demonstrate a successful induction ofχ⁽²⁾in Si₃N₄through electrical poling with an externally-applied field to align the Si-N bonds. This alignment breaks the centrosymmetry of Si₃N₄, and enables the bulkχ⁽²⁾. The sample is heated to over 500°C to facilitate the poling. The comparison between the EO responses of poled and non-poled Si₃N₄, measured using a Si₃N₄micro-ring modulator, shows at least a 25X enhancement in ther₃₃EO component. The maximumχ⁽²⁾we obtain through poling is 0.30pm/V. We observe a remarkable improvement in the speed of the measured EO responses from 3 GHz to 15 GHz (3 dB bandwidth) after the poling, which confirms theχ⁽²⁾nature of the EO response induced by poling. This work paves the way for high-speed active functions on the Si₃N₄platform.
5. Bidirectional interconversion of microwave and light with thin-film lithium niobate

   https://doi.org/10.1038/s41467-021-24809-y  

   Xu, Yuntao ; Sayem, Ayed Al ; Fan, Linran ; Zou, Chang-Ling ; Wang, Sihao ; Cheng, Risheng ; Fu, Wei ; Yang, Likai ; Xu, Mingrui ; Tang, Hong X. ( July 2021 , Nature Communications)

   Superconducting cavity electro-optics presents a promising route to coherently convert microwave and optical photons and distribute quantum entanglement between superconducting circuits over long-distance. Strong Pockels nonlinearity and high-performance optical cavity are the prerequisites for high conversion efficiency. Thin-film lithium niobate (TFLN) offers these desired characteristics. Despite significant recent progresses, only unidirectional conversion with efficiencies on the order of 10⁻⁵has been realized. In this article, we demonstrate the bidirectional electro-optic conversion in TFLN-superconductor hybrid system, with conversion efficiency improved by more than three orders of magnitude. Our air-clad device architecture boosts the sustainable intracavity pump power at cryogenic temperatures by suppressing the prominent photorefractive effect that limits cryogenic performance of TFLN, and reaches an efficiency of 1.02% (internal efficiency of 15.2%). This work firmly establishes the TFLN-superconductor hybrid EO system as a highly competitive transduction platform for future quantum network applications.