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1. Transition to strong coupling regime in hybrid plasmonic systems: Exciton-induced transparency and Fano interference

   Shahbazyan, Tigran V. (January 2021, arXiv)

   null (Ed.)

   We present a microscopic model describing the transition to strong coupling regime for an emitter resonantly coupled to a surface plasmon in a metal-dielectric structure. We demonstrate that the shape of scattering spectra is determined by an interplay of two distinct mechanisms. First is the near-field coupling between the emitter and the plasmon mode which underpins energy exchange between the system components and gives rise to exciton-induced transparency minimum in scattering spectra prior the transition to strong coupling regime. The second mechanism is Fano interference between the plasmon dipole and the plasmon-induced emitter's dipole as the system interacts with the radiation field. We show that the Fano interference can strongly affect the overall shape of scattering spectra, leading to the inversion of spectral asymmetry that was recently reported in the experiment. 

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2. Transition to strong coupling regime in hybrid plasmonic systems: exciton-induced transparency and Fano interference

   https://doi.org/10.1515/nanoph-2021-0246  

   Shahbazyan, Tigran V. (August 2021, Nanophotonics)

   Abstract We present a microscopic model describing the transition to a strong coupling regime for an emitter resonantly coupled to a surface plasmon in a metal–dielectric structure. We demonstrate that the shape of scattering spectra is determined by an interplay of two distinct mechanisms. First is the near-field coupling between the emitter and the plasmon mode which underpins energy exchange between the system components and gives rise to exciton-induced transparency minimum in scattering spectra prior to the transition to a strong coupling regime. The second mechanism is the Fano interference between the plasmon dipole and the plasmon-induced emitter’s dipole as the system interacts with the radiation field. We show that the Fano interference can strongly affect the overall shape of scattering spectra, leading to the inversion of spectral asymmetry that was recently reported in the experiment. 

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3. Plasmon-induced coherence, exciton-induced transparency, and Fano interference for hybrid plasmonic systems in strong coupling regime

   https://doi.org/10.1063/5.0083197  

   Scott, Zoe; Muhammad, Shafi; Shahbazyan, Tigran V. (May 2022, The Journal of Chemical Physics)

   We present an analytical model describing the transition to a strong coupling regime for an ensemble of emitters resonantly coupled to a localized surface plasmon in a metal–dielectric structure. The response of a hybrid system to an external field is determined by two distinct mechanisms involving collective states of emitters interacting with the plasmon mode. The first mechanism is the near-field coupling between the bright collective state and the plasmon mode, which underpins the energy exchange between the system components and gives rise to exciton-induced transparency minimum in scattering spectra in the weak coupling regime and to emergence of polaritonic bands as the system transitions to the strong coupling regime. The second mechanism is the Fano interference between the plasmon dipole moment and the plasmon-induced dipole moment of the bright collective state as the hybrid system interacts with the radiation field. The latter mechanism is greatly facilitated by plasmon-induced coherence in a system with the characteristic size below the diffraction limit as the individual emitters comprising the collective state are driven by the same alternating plasmon near field and, therefore, all oscillate in phase. This cooperative effect leads to scaling of the Fano asymmetry parameter and of the Fano function amplitude with the ensemble size, and therefore, it strongly affects the shape of scattering spectra for large ensembles. Specifically, with increasing emitter numbers, the Fano interference leads to a spectral weight shift toward the lower energy polaritonic band. 

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4. Tip-enhanced strong coupling spectroscopy, imaging, and control of a single quantum emitter

   https://doi.org/10.1126/sciadv.aav5931  

   Park, Kyoung-Duck; May, Molly A.; Leng, Haixu; Wang, Jiarong; Kropp, Jaron A.; Gougousi, Theodosia; Pelton, Matthew; Raschke, Markus B. (July 2019, Science Advances)

   Optical cavities can enhance and control light-matter interactions. This level of control has recently been extended to the nanoscale with single emitter strong coupling even at room temperature using plasmonic nanostructures. However, emitters in static geometries, limit the ability to tune the coupling strength or to couple different emitters to the same cavity. Here, we present tip-enhanced strong coupling (TESC) with a nanocavity formed between a scanning plasmonic antenna tip and the substrate. By reversibly and dynamically addressing single quantum dots, we observe mode splitting up to 160 meV and anticrossing over a detuning range of ~100 meV, and with subnanometer precision over the deep subdiffraction-limited mode volume. Thus, TESC enables previously inaccessible control over emitter-nanocavity coupling and mode volume based on near-field microscopy. This opens pathways to induce, probe, and control single-emitter plasmon hybrid quantum states for applications from optoelectronics to quantum information science at room temperature. 

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5. The Effects of Exit Boundary Condition on Precessing Vortex Core Dynamics

   Mason, Danielle; Clees, Sean; Frederick, Mark; O'Connor, Jacqueline (June 2019, ASME Turbo Expo)

   Many industrial combustion systems, especially power generation gas turbines, use fuel-lean combustion to reduce NOx emissions. However, these systems are highly susceptible to combustion instability, the coupling between combustor acoustics and heat release rate oscillations of the flame. It has been shown in previous work by the authors that a precessing vortex core (PVC) can suppress shear layer receptivity to external perturbations, reducing the potential for thermoacoustic coupling. The goal of this study is to understand the effect of combustor exit boundary condition on the flow structure of a swirling jet to increase fundamental understanding of how combustor design impacts PVC dynamics. The swirling jet is generated with a radial-entry, variable-angle swirler, and a quartz cylinder is fixed on the dump plane for confinement. Combustor exit constriction plates of different diameters are used to determine the impact of exit boundary condition on the flow field. Particle image velocimetry (PIV) is used to capture the velocity field inside the combustor. Spectral proper orthogonal decomposition, a frequency-resolved eigenvalue decomposition that can identify energetic structures in the flow, is implemented to identify the PVC at each condition in both energy and frequency space. We find that exit boundary diameter affects both the structure of the flow and the dynamics of the PVC. Higher levels of constriction (smaller diameters) force the downstream stagnation point of the vortex breakdown bubble upstream, resulting in greater divergence of the swirling jet. Further, as the exit diameter decreases, the PVC becomes less energetic and less spatially defined. Despite these changes in the base flow and PVC coherence, the PVC frequency is not altered by the exit boundary constriction. These trends will help inform our understanding of the impact of boundary conditions on both static and dynamic flame stability. 

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