More Like this

1. Hardware, methodology and applications of 2 + D backscatter Mössbauer spectroscopy with simultaneous x-ray and γ-ray detection

   https://doi.org/10.1088/1361-6501/ad044b  

   O’Brien, Jack ; Ahmadian Baghbaderani, Hasan ; Keller, Frederico O. ; Dempsey, Nora ; H Lewis, Laura ; Stamenov, Plamen ( November 2023 , Measurement Science and Technology)

   A unique method is presented for the acquisition and analysis of⁵⁷Fe backscatter Mössbauer spectra with simultaneous detection of the resonant 14.4 keVγ-rays and the characteristic 6.4 keV x-rays, using a custom-built multi-parameter analyser constructed on the basis of commercial analogue to digital converters and high-speed digital latches. The system allows for the simultaneous registration of Doppler-modulation velocities and photon energies, with up to 4096 and 8192 digital channels respectively. This arrangement is in contrast to most related systems, which detect at a single narrow energy window per detector. Samples of arbitrary atomic structure, morphology and surface topography can be studied without altering the setup or the analysis procedure, provided that the samples are at least micrometre sized. The hardware and software that are used to acquire data with minimal dead time are described and the custom and self-contained methods for post-measurement energy discrimination, background correction and velocity-axis folding are discussed. The data are fit using a general Hamiltonian model for the nuclear energy levels of⁵⁷Fe and a quantum mechanical description of the angular momentum coupling is utilised, with consideration of the crystalline and chemical disorder of the sample under examination. Three examples of distinct magnetic systems, with thicknesses ranging from$5\text{μ}$m to 6 mm, that were studied using this method are presented, these are: an amorphous CoFeB-based ribbon with ultra-soft coercivity for high-frequency applications, magnetically hard Nd-Fe-B thick films on Si substrates, examined in both as-deposited and annealed states, and a sample from the nickel-rich iron meteorite NWA 6259 that contains the atomically ordered, elevated coercivity,$L{1}_0$phase of FeNi, tetrataenite. The wide applicability and usefulness of this method is thus demonstrated on three distinct sample morphologies that required little to no surface preparation prior to examination.

    

   more » « less
2. Early photon optical tomography signal-to-noise ratio improved by almost two orders-of-magnitude by running in the “deadtime” regime

   Sinha, L. ; Zhou, W. ; Brankov, J.G. ; Tichauer, K.M ( January 2017 , World Molecular Imaging Congress 2017)

   Optical projection tomography (OPT) is a powerful imaging modality for attaining high resolution absorption and fluorescence imaging in tissue samples and embryos with a diameter of roughly 1 mm. Moving past this 1 mm limit, scattered light becomes the dominant fraction detected, adding significant “blur” to OPT. Time-domain OPT has been used to select out early-arriving photons that have taken a more direct route through the tissue to reduce detection of scattered photons in these larger samples, which are the cause of image domain blur1. In addition, it was recently demonstrated by our group that detection of scattered photons could be further depressed by running in a “deadtime” regime where laser repetition rates are selected such that the deadtime incurred by early-arriving photons acts as a shutter to later-arriving scattered photons2. By running in this deadtime regime, far greater early photon count rates are achievable than with standard early photon OPT. In this work, another advantage of this enhanced early photon collection approach is demonstrated: specifically, a significant improvement in signal-to-noise ratio. In single photon counting detectors, the main source of noise is “afterpulsing,” which is essentially leftover charge from a detected photon that spuriously results in a second photon count. When the arrival of the photons are time-stamped by the time correlated single photon counting (TCSPC) module , the rate constant governing afterpusling is slow compared to the time-scale of the light pulse detected so it is observed as a background signal with very little time-correlation. This signal is present in all time-gates and so adds noise to the detection of early photons. However, since the afterpusling signal is proportional to the total rate of photon detection, our enhanced early photon approach is uniquely able to have increased early photon counts with no appreciable increase in the afterpulsing since overall count-rate does not change. This is because as the rate of early photon detection goes up, the rate of late-photon detection reduces commensurately, yielding no net change in the overall rate of photons detected. This hypothesis was tested on a 4 mm diameter tissue-mimicking phantom (μa = 0.02 mm-1, μs’ = 1 mm-1) by ranging the power of a 10 MHz pulse 780-nm laser with pulse spread of < 100 fs (Calmar, USA) and an avalanche photodiode (MPD, Picoquant, Germany) and TCSPC module (HydraHarp, Picoquant, Germany) for light detection. Details of the results are in Fig. 1a, but of note is that we observed more than a 60-times improvement in SNR compared to conventional early photon detection that would have taken 1000-times longer to achieve the same early photon count. A demonstration of the type of resolution possible is in Fig 1b with an image of a 4-mm-thick human breast cancer biopsy where tumor spiculations of less than 100 μm diameter are observable. 1Fieramonti, L. et al. PloS one (2012). 2Sinha, L., et al. Optics letters (2016). 

   more » « less
3. Dithered depth imaging

   https://doi.org/10.1364/OE.408800  

   Rapp, Joshua ; Dawson, Robin M. A. ; Goyal, Vivek K. ( November 2020 , Optics Express)

   Single-photon lidar (SPL) is a promising technology for depth measurement at long range or from weak reflectors because of the sensitivity to extremely low light levels. However, constraints on the timing resolution of existing arrays of single-photon avalanche diode (SPAD) detectors limit the precision of resulting depth estimates. In this work, we describe an implementation of subtractively-dithered SPL that can recover high-resolution depth estimates despite the coarse resolution of the detector. Subtractively-dithered measurement is achieved by adding programmable delays into the photon timing circuitry that introduce relative time shifts between the illumination and detection that are shorter than the time bin duration. Careful modeling of the temporal instrument response function leads to an estimator that outperforms the sample mean and results in depth estimates with up to 13 times lower root mean-squared error than if dither were not used. The simple implementation and estimation suggest that globally dithered SPAD arrays could be used for high spatial- and temporal-resolution depth sensing.

    

   more » « less
4. Search for point sources of ultra-high-energy photons with the Telescope Array surface detector

   https://doi.org/10.1093/mnras/stz3618  

   Abbasi, R.U. ( February 2020 , Monthly notices of the Royal Astronomical Society)

   Ultra-high-energy (UHE) photons are an important tool for studying the high-energy Universe. A plausible source of photons with exa-eV (EeV) energy is provided by UHE cosmic rays (UHECRs) undergoing the Greisen–Zatsepin–Kuzmin process (Greisen 1966; Zatsepin & Kuzmin 1966) or pair production process (Blumenthal 1970) on a cosmic background radiation. In this context, the EeV photons can be a probe of both UHECR mass composition and the distribution of their sources (Gelmini, Kalashev & Semikoz 2008; Hooper, Taylor & Sarkar 2011). At the same time, the possible flux of photons produced by UHE protons in the vicinity of their sources by pion photoproduction or inelastic nuclear collisions would be noticeable only for relatively near sources, as the attenuation length of UHE photons is smaller than that of UHE protons; see, for example, Bhattacharjee & Sigl (2000) for a review. There also exists a class of so-called top-down models of UHECR generation that efficiently produce the UHE photons, for instance by the decay of heavy dark-matter particles (Berezinsky, Kachelriess & Vilenkin 1997; Kuzmin & Rubakov 1998) or by the radiation from cosmic strings (Berezinsky, Blasi & Vilenkin 1998). The search for the UHE photons was shown to be the most sensitive method of indirect detection of heavy dark matter (Kalashev & Kuznetsov 2016, 2017; Kuznetsov 2017; Kachelriess, Kalashev & Kuznetsov 2018; Alcantara, Anchordoqui & Soriano 2019). Another fundamental physics scenario that could be tested with UHE photons (Fairbairn, Rashba & Troitsky 2011) is the photon mixing with axion-like particles (Raffelt & Stodolsky 1988), which could be responsible for the correlation of UHECR events with BL Lac type objects observed by the High Resolution Fly’s Eye (HiRes) experiment (Gorbunov et al. 2004; Abbasi et al. 2006). In most of these scenarios, a clustering of photon arrival directions, rather than diffuse distribution, is expected, so point-source searches can be a suitable test for photon - axion-like particle mixing models. Finally, UHE photons could also be used as a probe for the models of Lorentz-invariance violation (Coleman & Glashow 1999; Galaverni & Sigl 2008; Maccione, Liberati & Sigl 2010; Rubtsov, Satunin & Sibiryakov 2012, 2014). The Telescope Array (TA; Tokuno et al. 2012; Abu-Zayyad et al. 2013c) is the largest cosmic ray experiment in the Northern Hemisphere. It is located at 39.3° N, 112.9° W in Utah, USA. The observatory includes a surface detector array (SD) and 38 fluorescence telescopes grouped into three stations. The SD consists of 507 stations that contain plastic scintillators, each with an area of 3 m2 (SD stations). The stations are placed in the square grid with 1.2 km spacing and cover an area of ∼700 km2. The TA SD is capable of detecting extensive air showers (EASs) in the atmosphere caused by cosmic particles of EeV and higher energies. The TA SD has been operating since 2008 May. A hadron-induced EAS significantly differs from an EAS induced by a photon because the depth of the shower maximum Xmax for a photon shower is larger, and a photon shower contains fewer muons and has a more curved front (see Risse & Homola 2007 for a review). The TA SD stations are sensitive to both muon and electromagnetic components of the shower and therefore can be triggered by both hadron-induced and photon-induced EAS events. In the present study, we use 9 yr of TA SD data for a blind search for point sources of UHE photons. We utilize the statistics of the SD data, which benefit from a high duty cycle. The full Monte Carlo (MC) simulation of proton-induced and photon-induced EAS events allows us to perform the photon search up to the highest accessible energies, E ≳ 1020 eV. As the main tool for the present photon search, we use a multivariate analysis based on a number of SD parameters that make it possible to distinguish between photon and hadron primaries. While searches for diffuse UHE photons were performed by several EAS experiments, including Haverah Park (Ave et al. 2000), AGASA (Shinozaki et al. 2002; Risse et al. 2005), Yakutsk (Rubtsov et al. 2006; Glushkov et al. 2007, 2010), Pierre Auger (Abraham et al. 2007, 2008a; Bleve 2016; Aab et al. 2017c) and TA (Abu-Zayyad et al. 2013b; Abbasi et al. 2019a), the search for point sources of UHE photons has been done only by the Pierre Auger Observatory (Aab et al. 2014, 2017a). The latter searches were based on hybrid data and were limited to the 1017.3 < E < 1018.5 eV energy range. In the present paper, we use the TA SD data alone. We perform the searches in five energy ranges: E > 1018, E > 1018.5, E > 1019, E > 1019.5 and E > 1020 eV. We find no significant evidence of photon point sources in all energy ranges and we set the point-source flux upper limits from each direction in the TA field of view (FOV). The search for unspecified neutral particles was also previously performed by the TA (Abbasi et al. 2015). The limit on the point-source flux of neutral particles obtained in that work is close to the present photon point-source flux limits. 

   more » « less
5. Single-photoelectron collection efficiency in 4D ultrafast electron microscopy

   https://doi.org/10.1039/d2cp01250b  

   Curtis, Wyatt A. ; Willis, Simon A. ; Flannigan, David J. ( June 2022 , Physical Chemistry Chemical Physics)

   In femtosecond (fs) 4D ultrafast electron microscopy (UEM), a tradeoff is made between photoelectrons per packet and time resolution. One consequence of this can be longer-than-desirable acquisition times for low-density packets, and particularly for low repetition rates when complete photothermal dissipation is required. Thus, gaining an understanding of photoelectron trajectories in the gun region is important for identifying factors that limit collection efficiency (CE; fraction of photoelectrons that enter the illumination system). Here, we continue our work on the systematic study of photoelectron trajectories in the gun region of a Thermo Fisher/FEI Tecnai Femto UEM, focusing specifically on CE in the single-electron regime. Using General Particle Tracer, calculated field maps, and the exact architecture of the Tecnai Femto UEM, we simulated the effects of fs laser parameters and key gun elements on CE. The results indicate CE strongly depends upon the laser spot size on the source, the (unbiased) Wehnelt aperture diameter, and the incident photon energy. The CE dispersion with laser spot size is found to be strongly dependent on aperture diameter, being nearly dispersionless for the largest apertures. A gun crossover is also observed, with the beam-waist position being dependent on the aperture diameter, further illustrating that the Wehnelt aperture acts as a simple, fixed electrostatic lens in UEM mode. This work provides further insights into the operational aspects of fs 4D UEM. 

   more » « less