A passively phase-stable, broadband ( , ) two-dimensional (2D) electronic spectroscopy apparatus that achieves rapid acquisition rates by continuously—rather than step-wise—scanning the Fourier-transform dimension is demonstrated for the first time, to the best of our knowledge. This is made possible through use of a partially common path interferometer design in which the coherence time is sampled in a “rotating frame.” Rapid, continuous scanning of increases the duty cycle of signal collection, rejects the majority of excitation pulse scatter, and enables the measurement of a complete 2D spectrum in 92 ms, which minimizes the influence of pulse intensity and delay fluctuations on the 2D spectrum. In practice, these improvements make possible the acquisition of hundreds of 2D spectra in tens of minutes, which opens the door to dense sampling of ultrafast relaxation dynamics and to generating extremely broadband 3D Fourier-transform spectra.
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2D beam shaping via 1D spatial light modulator using static phase masks
Many emerging, high-speed, reconfigurable optical systems are limited by routing complexity when producing dynamic, two-dimensional (2D) electric fields. We propose a gradient-based inverse-designed, static phase-mask doublet to generate arbitrary 2D intensity wavefronts using a one-dimensional (1D) intensity spatial light modulator (SLM). We numerically simulate the capability of mapping each point in a 49 element 1D array to a distinct 2D spatial distribution. Our proposed method will significantly relax the routing complexity of electrical control signals, possibly enabling high-speed, sub-wavelength 2D SLMs leveraging new materials and pixel architectures.
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- PAR ID:
- 10225767
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Optics Letters
- Volume:
- 46
- Issue:
- 10
- ISSN:
- 0146-9592; OPLEDP
- Format(s):
- Medium: X Size: Article No. 2280
- Size(s):
- Article No. 2280
- Sponsoring Org:
- National Science Foundation
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