skip to main content

Explore Research Products in the NSF-PAR

Title: The Fracture of Highly Deformable Soft Materials: A Tale of Two Length Scales
The fracture of highly deformable soft materials is of great practical importance in a wide range of technological applications, emerging in fields such as soft robotics, stretchable electronics, and tissue engineering. From a basic physics perspective, the failure of these materials poses fundamental challenges due to the strongly nonlinear and dissipative deformation involved. In this review, we discuss the physics of cracks in soft materials and highlight two length scales that characterize the strongly nonlinear elastic and dissipation zones near crack tips in such materials. We discuss physical processes, theoretical concepts, and mathematical results that elucidate the nature of the two length scales and show that the two length scales can classify a wide range of materials. The emerging multiscale physical picture outlines the theoretical ingredients required for the development of predictive theories of the fracture of soft materials. We conclude by listing open challenges and directions for future investigations.  more » « less
Award ID(s):
1752449
NSF-PAR ID:
10229711
Author(s) / Creator(s):
; ; ;
Date Published:
Journal Name:
Annual Review of Condensed Matter Physics
Volume:
12
Issue:
1
ISSN:
1947-5454
Page Range / eLocation ID:
71 to 94
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. ; ; ; ; ( , Journal of the mechanics and physics of solids)
    null (Ed.)
    Recent theoretical and computational progress has led to unprecedented understanding of symmetry-breaking instabilities in 2D dynamic fracture. At the heart of this progress resides the identification of two intrinsic, near crack tip length scales — a nonlinear elastic length scale ℓ and a dissipation length scale ξ — that do not exist in Linear Elastic Fracture Mechanics (LEFM), the classical theory of cracks. In particular, it has been shown that at a propagation velocity v of about 90% of the shear wave-speed, cracks in 2D brittle materials undergo an oscillatory instability whose wavelength varies linearly with ℓ, and at larger loading levels (corresponding to yet higher propagation velocities), a tip-splitting instability emerges, both in agreements with experiments. In this paper, using phase-field models of brittle fracture, we demonstrate the following properties of the oscillatory instability: (i) It exists also in the absence of near-tip elastic nonlinearity, i.e. in the limit ℓ→0, with a wavelength determined by the dissipation length scale ξ. This result shows that the instability crucially depends on the existence of an intrinsic length scale associated with the breakdown of linear elasticity near crack tips, independently of whether the latter is related to nonlinear elasticity or to dissipation. (ii) It is a supercritical Hopf bifurcation, featuring a vanishing oscillations amplitude at onset. (iii) It is largely independent of the phenomenological forms of the degradation functions assumed in the phase-field framework to describe the cohesive zone, and of the velocity-dependence of the fracture energy Γ(v) that is controlled by the dissipation time scale in the Ginzburg-Landau-type evolution equation for the phase-field. These results substantiate the universal nature of the oscillatory instability in 2D. In addition, we provide evidence indicating that the tip-splitting instability is controlled by the limiting rate of elastic energy transport inside the crack tip region. The latter is sensitive to the wave-speed inside the dissipation zone, which can be systematically varied within the phase-field approach. Finally, we describe in detail the numerical implementation scheme of the employed phase-field fracture approach, allowing its application in a broad range of materials failure problems. 
    more » « less
  2. ; ; ; ; ; ; ; ; ; ; et al ( , Journal of Physics: Materials)
    Soft materials are usually defined as materials made of mesoscopic entities, often self-organised, sensitive to thermal fluctuations and to weak perturbations. Archetypal examples are colloids, polymers, amphiphiles, liquid crystals, foams. The importance of soft materials in everyday commodity products, as well as in technological applications, is enormous, and controlling or improving their properties is the focus of many efforts. From a fundamental perspective, the possibility of manipulating soft material properties, by tuning interactions between constituents and by applying external perturbations, gives rise to an almost unlimited variety in physical properties. Together with the relative ease to observe and characterise them, this renders soft matter systems powerful model systems to investigate statistical physics phenomena, many of them relevant as well to hard condensed matter systems. Understanding the emerging properties from mesoscale constituents still poses enormous challenges, which have stimulated a wealth of new experimental approaches, including the synthesis of new systems with, e.g. tailored self-assembling properties, or novel experimental techniques in imaging, scattering or rheology. Theoretical and numerical methods, and coarse-grained models, have become central to predict physical properties of soft materials, while computational approaches that also use machine learning tools are playing a progressively major role in many investigations. This Roadmap intends to give a broad overview of recent and possible future activities in the field of soft materials, with experts covering various developments and challenges in material synthesis and characterisation, instrumental, simulation and theoretical methods as well as general concepts. 
    more » « less
  3. ; ( , Physical Chemistry Chemical Physics)
    null (Ed.)
    Phonon-mediated thermal transport is inherently multi-scale. The wave-length of phonons (considering phonons as waves) is typically at the nanometer scale; the typical size of a phonon wave energy packet is tens of nanometers, while the phonon mean free path (MFP) can be as long as microns. At different length scales, the phonons will interact with structures of different feature sizes, which can be as small as 0D defects (point defects), short to medium range linear defects (dislocations), medium to large range 2D planar defects (stacking faults and twin boundaries), and large scale 3D defects (voids, inclusions, and various microstructures). The nature of multi-scale thermal transport is that there are different heat transfer physics across different length scales and in the meantime the physics crossing the different scales is interdependent and coupled. Since phonon behavior is usually mode dependent, thermal transport in materials with a combined micro-/nano-structure complexity becomes complicated, making modeling this kind of transport process very challenging. In this perspective, we first summarize the advantages and disadvantages of computational methods for mono-scale heat transfer and the state-of-the-art multi-scale thermal transport modeling. We then discuss a few important aspects of the future development of multi-scale modeling, in particular with the aid of modern machine learning and uncertainty quantification techniques. As more sophisticated theoretical and computational methods continue to advance thermal transport predictions, novel heat transfer physics and thermally functional materials will be discovered for the pertaining energy systems and technologies. 
    more » « less
  4. ; ( , Advanced Science)
    Abstract

    Emerging interest to synthesize active, engineered matter suggests a future where smart material systems and structures operate autonomously around people, serving diverse roles in engineering, medical, and scientific applications. Similar to biological organisms, a realization of active, engineered matter necessitates functionality culminating from a combination of sensory and control mechanisms in a versatile material frame. Recently, metamaterial platforms with integrated sensing and control have been exploited, so that outstanding non‐natural material behaviors are empowered by synergistic microstructures and controlled by smart materials and systems. This emerging body of science around active mechanical metamaterials offers a first glimpse at future foundations for autonomous engineered systems referred to here as soft, smart matter. Using natural inspirations, synergy across disciplines, and exploiting multiple length scales as well as multiple physics, researchers are devising compelling exemplars of actively controlled metamaterials, inspiring concepts for autonomous engineered matter. While scientific breakthroughs multiply in these fields, future technical challenges remain to be overcome to fulfill the vision of soft, smart matter. This Review surveys the intrinsically multidisciplinary body of science targeted to realize soft, smart matter via innovations in active mechanical metamaterials and proposes ongoing research targets that may deliver the promise of autonomous, engineered matter to full fruition.

     
    more » « less
  5. ; ; ; ; ; ( , Advanced Materials)
    Abstract

    The field of quantum materials has experienced rapid growth over the past decade, driven by exciting new discoveries with immense transformative potential. Traditional synthetic methods to quantum materials have, however, limited the exploration of architectural control beyond the atomic scale. By contrast, soft matter self‐assembly can be used to tailor material structure over a large range of length scales, with a vast array of possible form factors, promising emerging quantum material properties at the mesoscale. This review explores opportunities for soft matter science to impact the synthesis of quantum materials with advanced properties. Existing work at the interface of these two fields is highlighted, and perspectives are provided on possible future directions by discussing the potential benefits and challenges which can arise from their bridging.

     
    more » « less
  • Citation Formats
  • MLA
  • APA
  • Chicago
  • BibTeX
  • Save / Share this Record
  • Send to Email