skip to main content


Title: Additional global climate cooling by clouds due to ice crystal complexity
Abstract. Ice crystal submicron structures have a large impact on the opticalproperties of cirrus clouds and consequently on their radiative effect.Although there is growing evidence that atmospheric ice crystals are rarelypristine, direct in situ observations of the degree of ice crystal complexityare largely missing. Here we show a comprehensive in situ data set of icecrystal complexity coupled with measurements of the cloud angular scatteringfunctions collected during a number of observational airborne campaigns atdiverse geographical locations. Our results demonstrate that an overwhelmingfraction (between 61 % and 81 %) of atmospheric ice crystals sampledin the different regions contain mesoscopic deformations and, as aconsequence, a similar flat and featureless angular scattering function isobserved. A comparison between the measurements and a database of opticalparticle properties showed that severely roughened hexagonal aggregatesoptimally represent the measurements in the observed angular range. Based onthis optical model, a new parameterization of the cloud bulk asymmetry factorwas introduced and its effects were tested in a global climate model. Themodelling results suggest that, due to ice crystal complexity, ice-containingclouds can induce an additional short-wave cooling effect of−1.12 W m2 on the top-of-the-atmosphere radiative budget that hasnot yet been considered.  more » « less
Award ID(s):
1762096
NSF-PAR ID:
10234574
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ;
Date Published:
Journal Name:
Atmospheric Chemistry and Physics
Volume:
18
Issue:
21
ISSN:
1680-7324
Page Range / eLocation ID:
15767 to 15781
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract

    Ice crystals commonly adopt a horizontal orientation under certain aerodynamic and electrodynamic conditions that occur in the atmosphere. While the radiative impact of horizontally oriented ice crystals (HOIC) has been theoretically studied with respect to their impact on shortwave cloud albedo, the longwave impact remains unexplored. This work analyzes the occurrence of HOIC at Summit, Greenland, from July 2015 to June 2017. Using polarization lidar and ancillary atmospheric sensors, ice crystal orientations are identified and used to interpret cloud radiative impact on the surface radiation budget. We find HOIC occur in at least 25.6% of all ice‐only column observations. We find that the shortwave impact of HOIC is to increase cloud radiative effect by approximately 22% for a given solar zenith angle. We also find that the longwave impact of HOIC compared to randomly oriented ice crystals are statistically different at the p < 0.01 significance level, increasing the surface radiative effect by approximately 8% for clouds with infrared optical depths < ~1. We suggest that the observed difference between the surface radiative effect for clouds containing randomly oriented ice crystals and HOIC may be due to enhanced scattering, but this hypothesis needs to be further explored with more detailed observations and modeling.

     
    more » « less
  2. Aerosols affect cirrus formation and evolution, yet quantification of these effects remain difficult based on in-situ observations due to the complexity of nucleation mechanisms and large variabilities in ice microphysical properties. This work employed a method to distinguish five evolution phases of cirrus clouds based on in-situ aircraft-based observations from seven U.S. National Science Foundation (NSF) and five NASA flight campaigns. Both homogeneous and heterogeneous nucleation were captured in the 1-Hz aircraft observations, inferred from the distributions of relative humidity in the nucleation phase. Using linear regressions to quantify the correlations between cirrus microphysical properties and aerosol number concentrations, we found that ice water content (IWC) and ice crystal number concentration (Ni) show strong positive correlations with larger aerosols (> 500 nm) in the nucleation phase, indicating strong contributions of heterogeneous nucleation when ice crystals first start to nucleate. For the later growth phase, IWC and Ni show similar positive correlations with larger and smaller (i.e., > 100 nm) aerosols, possibly due to fewer remaining ice nucleating particles in the later growth phase that allows more homogeneous nucleation to occur. Both 200-m and 100-km observations were compared with the nudged simulations from the National Center for Atmospheric Research (NCAR) Community Atmosphere Model version 6 (CAM6). Simulated aerosol indirect effects are weaker than the observations for both larger and smaller aerosols. Observations show stronger aerosol indirect effects (i.e., positive correlations between IWC, Ni and Na) in the Southern Hemisphere (SH) compared with the Northern Hemisphere (NH), while the simulations show negative correlations in the SH. The simulations underestimate IWC by a factor of 3 – 30 in the early/later growth phase, indicating that the low bias of simulated IWC was due to insufficient ice particle growth. Such hypothesis is consistent with the model biases of lower frequencies of ice supersaturation and lower vertical velocity standard deviation in the early/later growth phases. Overall, these findings show that aircraft observations can capture the competitions between heterogeneous and homogeneous nucleation, and their contributions vary as cirrus clouds evolve. Future model development is also recommended to evaluate and improve the representation of water vapor and vertical velocity on the sub-grid scale to resolve the insufficient ice particle growth. 
    more » « less
  3. Abstract

    Cirrus dominate the longwave radiative budget of the tropics. For the first time, the variability in cirrus properties and longwave cloud radiative effects (CREs) that arises from using different microphysical schemes within nudged global storm‐resolving simulations from a single model, is quantified. Nudging allows us to compute radiative biases precisely using coincident satellite measurements and to fix the large‐scale dynamics across our set of simulations to isolate the influence of microphysics. We run 5‐day simulations with four commonly‐used microphysics schemes of varying complexity (SAM1MOM, Thompson, M2005 and P3) and find that the tropical average longwave CRE varies over 20 W m−2between schemes. P3 best reproduces observed longwave CRE. M2005 and P3 simulate cirrus with realistic frozen water path but unrealistically high ice crystal number concentrations which commonly hit limiters and lack the variability and dependence on frozen water content seen in aircraft observations. Thompson and SAM1MOM have too little cirrus.

     
    more » « less
  4. Abstract

    Maritime boundary‐layer clouds over the Southern Ocean (SO) have a large shortwave radiative effect. Yet, climate models have difficulties in representing these clouds and, especially, their phase in this observationally sparse region. This study aims to increase the knowledge of SO cloud phase by presenting in‐situ cloud microphysical observations from the Southern Ocean Clouds, Radiation, Aerosol, Transport Experimental Study (SOCRATES). We investigate the occurrence of ice in summertime marine stratocumulus and cumulus clouds in the temperature range between 6 and −25°C. Our observations show that in ice‐containing clouds, maximum ice number concentrations of up to several hundreds per liter were found. The observed ice crystal concentrations were on average one to two orders of magnitude higher than the simultaneously measured ice nucleating particle (INP) concentrations in the temperature range below −10°C and up to five orders of magnitude higher than estimated INP concentrations in the temperature range above −10°C. These results highlight the importance of secondary ice production (SIP) in SO summertime marine boundary‐layer clouds. Evidence for rime splintering was found in the Hallett‐Mossop (HM) temperature range but the exact SIP mechanism active at lower temperatures remains unclear. Finally, instrument simulators were used to assess simulated co‐located cloud ice concentrations and the role of modeled HM rime‐splintering. We found that CAM6 is deficient in simulating number concentrations across the HM temperature range with little sensitivity to the model HM process, which is inconsistent with the aforementioned observational evidence of highly active SIP processes in SO low‐level clouds.

     
    more » « less
  5. Cirrus cloud radiative effects are largely affected by ice microphysical properties, including ice water content (IWC), ice crystal number concentration (Ni) and mean diameter (Di). These characteristics vary significantly due to thermodynamic, dynamical and aerosol conditions. In this work, a global-scale observation dataset is used to examine regional variations of cirrus cloud microphysical properties, as well as several key controlling factors, i.e., temperature, relative humidity with respect to ice (RHi), vertical velocity (w), and aerosol number concentrations (Na). Results are compared with simulations from the National Center for Atmospheric Research (NCAR) Community Atmosphere Model version 6 (CAM6). The differences between simulations and observations are found to vary with latitude and temperature. Specifically, simulations are found to underestimate IWC by a factor of 5–30 in all regions. Simulated Ni is overestimated in most regions except Northern Hemisphere midlatitude and polar regions. Simulated Di is underestimated, especially for warmer conditions (−50 °C to −40 °C) and higher Na, possibly due to less effective ice particle growth/sedimentation and weaker aerosol indirect effects, respectively. For RHi effects, the frequency and magnitude of ice supersaturation is underestimated in simulations for clear-sky conditions, and the simulated IWC and Ni show maximum values at 80 % RHi instead of 110 % as observed. For w effects, both observations and simulations show variances of w (σw) decreasing from tropics to polar regions, but simulations show much higher σw for in-cloud condition than clear-sky condition. These findings provide an observation-based guideline for improving simulated ice microphysical properties and their relationships with key controlling factors at various geographical locations. 
    more » « less