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  1. Abstract

    Supercooled liquid water (SLW) and mixed phase clouds containing SLW and ice over the Southern Ocean (SO) are poorly represented in global climate and numerical weather prediction models. Observed SLW exists at lower temperatures than threshold values used to characterize its detrainment from convection in model parameterizations, and processes controlling its formation and removal are poorly understood. High‐resolution observations are needed to better characterize SLW over the SO. This study characterizes the frequency and spatial distribution of different cloud phases (liquid, ice, and mixed) using in situ observations acquired during the Southern Ocean Clouds, Radiation, Aerosol Transport Experiment Study. Cloud particle phase is identified using multiple cloud probes. Results show occurrence frequencies of liquid phase samples up to 70% between −20°C and 0°C and of ice phase samples up to 10% between −5°C and 0°C. Cloud phase spatial heterogeneity is determined by relating the total number of 1 s samples from a given cloud to the number of segments whose neighboring samples are the same phase. Mixed phase conditions are the most spatially heterogeneous from −20°C to 0°C, whereas liquid phase conditions from −10°C to 0°C and ice phase conditions from −20°C to −10°C are the least spatially heterogeneous. Greater spatial heterogeneity is associated with broader distributions of vertical velocity. Decreasing droplet concentrations and increasing number‐weighted mean liquid diameters occur within mixed phase clouds as the liquid water fraction decreases, possibly suggesting preferential evaporation of smaller drops during the Wegener‐Bergeron‐Findeisen process.

     
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  2. Abstract

    For a given cloud, whether the cloud top is predominately made up of ice crystals or supercooled liquid droplets plays a large role in the clouds overall radiative effects. This study uses collocated airborne radar, lidar, and thermodynamic data from 12 high‐altitude flight legs during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) to characterize Southern Ocean (SO) cold sector cloud top phase (i.e., within 96 m of top) as a function of cloud top temperature (CTT). A training data set was developed to create probabilistic phase classifications based on High Spectral Resolution Lidar data and Cloud Radar data. These classifications were then used to identify dominant cloud top phase. Case studies are presented illustrating examples of supercooled liquid water at cloud top at different CTT ranges over the SO (−3°C < CTTs < −28°C). During SOCRATES, 67.4% of sampled cloud top had CTTs less than 0°C. Of the subfreezing cloud tops sampled, 91.7% had supercooled liquid water present in the top 96 m and 74.9% were classified entirely as liquid‐bearing. Liquid‐bearing cloud tops were found at CTTs as cold as −30°C. Horizontal cloud extent was also determined as a function of median cloud top height.

     
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  3. Abstract

    The characteristics of cloud droplet size distributions and statistical relations of the relative dispersion (ε) with the vertical velocity (w) and with the interstitial aerosol concentration (Nia) are investigated for ubiquitous supercooled shallow stratocumulus observed over the Southern Ocean (SO) using aircraft measurements obtained during the Southern Ocean Cloud Radiation Aerosol Transport Experimental Study. Distinct vertical variations have been found using 36 non‐precipitating cloud profiles. The cloud droplet effective radius (re) increases nearly monotonically from 5.3 ± 1.9 μm at cloud base to 9.4 ± 2.2 μm at cloud top. Theεdecreases rapidly from cloud base (0.42 ± 0.13) and then remains relatively constant in the upper cloud layer (0.27 ± 0.09). This study also shows robust dependence ofεon bothNiaandw. Theεincreases (decreases) with increasingNia(w) at a 95% confidence level when values ofw(lowNia) are restricted to a small range. The important roles of aerosols and dynamics onεare demonstrated and are crucial to estimating aerosol indirect radiative forcing, especially for pristine SO regions where models almost universally underestimate reflected radiation.

     
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  4. Abstract

    Southern Ocean (S. Ocean) clouds are important for climate prediction. Yet previous global climate models failed to accurately represent cloud phase distributions in this observation‐sparse region. In this study, data from the Southern Ocean Clouds, Radiation, Aerosol, Transport Experimental Study (SOCRATES) experiment is compared to constrained simulations from a global climate model (the Community Atmosphere Model, CAM). Nudged versions of CAM are found to reproduce many of the features of detailed in situ observations, such as cloud location, cloud phase, and boundary layer structure. The simulation in CAM6 has improved its representation of S. Ocean clouds with adjustments to the ice nucleation and cloud microphysics schemes that permit more supercooled liquid. Comparisons between modeled and observed hydrometeor size distributions suggest that the modeled hydrometeor size distributions represent the dual peaked shape and form of observed distributions, which is remarkable given the scale difference between model and observations. Comparison to satellite observations of cloud physics is difficult due to model assumptions that do not match retrieval assumptions. Some biases in the model's representation of S. Ocean clouds and aerosols remain, but the detailed cloud physical parameterization provides a basis for process level improvement and direct comparisons to observations. This is crucial because cloud feedbacks and climate sensitivity are sensitive to the representation of S. Ocean clouds.

     
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  5. Abstract

    An atmospheric river (AR) impacting Tasmania, Australia, and the Southern Ocean during the austral summer on 28–29 January 2018 during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study campaign is analyzed using a modeling and observational approach. Gulfstream‐V dropsonde measurements and Global Precipitation Measurement radar analyses were used in conjunction with Weather Research and Forecasting model simulations with water vapor tracers to investigate the relative contributions of tropical and midlatitude moisture sources to the AR. Moisture associated with a monsoonal tropical depression became entrained into a midlatitude frontal system that extended to 60°S, reaching the associated low‐pressure system 850 km off the coast of Antarctica—effectively connecting the tropics and the polar region. Tropical moisture contributed to about 50% of the precipitable water within the AR as the flow moved over the Southern Ocean near Tasmania. The tropical contribution to precipitation decreased with latitude, from >70% over Australia, to ~50% off the Australian coast, to less than 5% poleward of 55°S. The integrated vapor transport (IVT) through the core of the AR reached above 500 kg m−1 s−1during 1200 UTC 28 January to 0600 UTC 29 January, 1.29 times the average amount of water carried by the world's largest terrestrial river, the Amazon. The high IVT strength might be attributed to the higher water vapor content associated with the warmer temperatures across Australia and the Southern Ocean in austral summer.

     
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  6. Abstract

    An atmospheric river affecting Australia and the Southern Ocean on 28–29 January 2018 during the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) is analyzed using nadir‐pointing W‐band cloud radar measurements and in situ microphysical measurements from a Gulfstream‐V aircraft. The AR had a two‐band structure, with the westernmost band associated with a cold frontal boundary. The bands were primarily stratiform with distinct radar bright banding. The microphysical evolution of precipitation is described in the context of the tropical‐ and midlatitude‐sourced moisture zones above and below the 0°C isotherm, respectively, identified in Part I. In the tropical‐sourced moisture zone, ice particles at temperatures less than −8°C had concentrations on the order of 10 L−1, with habits characteristic of lower temperatures, while between −8°C and −4°C, an order of magnitude increase in ice particle concentrations was observed, with columnar habits consistent with Hallett‐Mossop secondary ice formation. Ice particles falling though the 0°C level into the midlatitude‐sourced moisture region and melting provided “seed” droplets from which subsequent growth by collision‐coalescence occurred. In this region, raindrops grew to sizes of 3 mm and precipitation rates averaged 16 mm hr−1.

     
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  7. Abstract

    The bulk microphysical properties and number distribution functions (N(D)) of supercooled liquid water (SLW) and ice inside and between ubiquitous generating cells (GCs) observed over the Southern Ocean (SO) during the Southern Ocean Clouds Radiation Aerosol Transport Experimental Study (SOCRATES) measured by in situ cloud probes onboard the NCAR/NSF G‐V aircraft are compared. SLW was detected inside all GCs with an average liquid water content of 0.31 ± 0.19 g m−3, 11% larger than values between GCs. TheN(D)of droplets (maximum dimensionD < 50 μm) inside and between GCs had only slight differences. For ice particles, on the other hand, the mean concentration (median mass diameter) withD > 200 μm inside GCs was 2.0 ± 3.3 L−1(323 ± 263 μm), 65% (37%) larger than values outside GCs. AsDincreases, the percentage differences became larger (up to ~500%). The more and larger ice particles inside GCs suggest the GC updrafts provide a favorable environment for particle growth by deposition and riming and that mixing processes are less efficient at redistributing larger particles. The horizontal scale of observed GCs ranged from 200 to 600 m with a mean of 395 ± 162 m, smaller than GC widths observed in previous studies. This study expands knowledge of the microphysical properties and processes acting in GCs over a wider range of conditions than previously available.

     
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  8. null (Ed.)
    Abstract. Ice crystal submicron structures have a large impact on the opticalproperties of cirrus clouds and consequently on their radiative effect.Although there is growing evidence that atmospheric ice crystals are rarelypristine, direct in situ observations of the degree of ice crystal complexityare largely missing. Here we show a comprehensive in situ data set of icecrystal complexity coupled with measurements of the cloud angular scatteringfunctions collected during a number of observational airborne campaigns atdiverse geographical locations. Our results demonstrate that an overwhelmingfraction (between 61 % and 81 %) of atmospheric ice crystals sampledin the different regions contain mesoscopic deformations and, as aconsequence, a similar flat and featureless angular scattering function isobserved. A comparison between the measurements and a database of opticalparticle properties showed that severely roughened hexagonal aggregatesoptimally represent the measurements in the observed angular range. Based onthis optical model, a new parameterization of the cloud bulk asymmetry factorwas introduced and its effects were tested in a global climate model. Themodelling results suggest that, due to ice crystal complexity, ice-containingclouds can induce an additional short-wave cooling effect of−1.12 W m2 on the top-of-the-atmosphere radiative budget that hasnot yet been considered. 
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