Abstract. In this study, we developed a novel algorithm based on the collocatedModerate Resolution Imaging Spectroradiometer (MODIS) thermal infrared (TIR)observations and dust vertical profiles from the Cloud–Aerosol Lidar withOrthogonal Polarization (CALIOP) to simultaneously retrieve dust aerosoloptical depth at 10 µm (DAOD10 µm) and the coarse-mode dusteffective diameter (Deff) over global oceans. The accuracy of theDeff retrieval is assessed by comparing the dust lognormal volumeparticle size distribution (PSD) corresponding to retrieved Deff withthe in situ-measured dust PSDs from the AERosol Properties – Dust(AER-D), Saharan Mineral Dust Experiment (SAMUM-2), and Saharan Aerosol Long-Range Transport and Aerosol–Cloud-InteractionExperiment (SALTRACE) fieldcampaigns through case studies. The new DAOD10 µm retrievals wereevaluated first through comparisons with the collocated DAOD10.6 µmretrieved from the combined Imaging Infrared Radiometer (IIR) and CALIOPobservations from our previous study (Zheng et al., 2022). The pixel-to-pixelcomparison of the two DAOD retrievals indicates a good agreement(R∼0.7) and a significant reduction in (∼50 %) retrieval uncertainties largely thanks to the better constraint ondust size. In a climatological comparison, the seasonal and regional(2∘×5∘) mean DAOD10 µm retrievals basedon our combined MODIS and CALIOP method are in good agreement with the twoindependent Infrared Atmospheric Sounding Interferometer (IASI) productsover three dust transport regions (i.e., North Atlantic (NA; R=0.9),Indian Ocean (IO; R=0.8) and North Pacific (NP; R=0.7)). Using the new retrievals from 2013 to 2017, we performed a climatologicalanalysis of coarse-mode dust Deff over global oceans. We found thatdust Deff over IO and NP is up to 20 % smaller than that over NA.Over NA in summer, we found a ∼50 % reduction in the numberof retrievals with Deff>5 µm from 15 to35∘ W and a stable trend of Deff average at 4.4 µm from35∘ W throughout the Caribbean Sea (90∘ W). Over NP inspring, only ∼5 % of retrieved pixels with Deff>5 µm are found from 150 to 180∘ E, whilethe mean Deff remains stable at 4.0 µm throughout eastern NP. To the best of our knowledge, this study is the first to retrieve both DAOD andcoarse-mode dust particle size over global oceans for multiple years. Thisretrieval dataset provides insightful information for evaluating dustlongwave radiative effects and coarse-mode dust particle size in models.
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Strong links between Saharan dust fluxes, monsoon strength, and North Atlantic climate during the last 5000 years
Despite the multiple impacts of mineral aerosols on global and regional climate and the primary climatic control on atmospheric dust fluxes, dust-climate feedbacks remain poorly constrained, particularly at submillennial time scales, hampering regional and global climate models. We reconstruct Saharan dust fluxes over Western Europe for the last 5000 years, by means of speleothem strontium isotope ratios ( 87 Sr/ 86 Sr) and karst modeling. The record reveals a long-term increase in Saharan dust flux, consistent with progressive North Africa aridification and strengthening of Northern Hemisphere latitudinal climatic gradients. On shorter, centennial to millennial scales, it shows broad variations in dust fluxes, in tune with North Atlantic ocean-atmosphere patterns and with monsoonal variability. Dust fluxes rapidly increase before (and peaks at) Late Holocene multidecadal- to century-scale cold climate events, including those around 4200, 2800, and 1500 years before present, suggesting the operation of previously unknown strong dust-climate negative feedbacks preceding these episodes.
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- Award ID(s):
- 1702816
- PAR ID:
- 10292166
- Date Published:
- Journal Name:
- Science Advances
- Volume:
- 7
- Issue:
- 26
- ISSN:
- 2375-2548
- Page Range / eLocation ID:
- eabe6102
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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