skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Near‐Field Characterization of Higher‐Order Topological Photonic States at Optical Frequencies
Abstract Higher‐order topological insulators (HOTIs) represent a new type of topological system, supporting boundary states localized over boundaries, two or more dimensions lower than the dimensionality of the system itself. Interestingly, photonic HOTIs can possess a richer physics than their original condensed matter counterpart, supporting conventional HOTI states based on tight‐binding coupling, and a new type of topological HOTI states enabled by long‐range interactions. Here, a new mechanism to establish all‐dielectric infrared HOTI metasurfaces exhibiting both types of HOTI states is proposed, supported by a topological transition accompanied by the emergence of topological Wannier‐type polarization. Two kinds of near‐field experimental studies are performed: i) the solid immersion spectroscopy and ii) near‐field imaging using scattering scanning near‐field optical microscopy to directly observe the topological transition and the emergence of HOTI states of two types. It is shown that the near‐field profiles indicate the displacement of the Wannier center across the topological transition leading to the topological dipole polarization and emergence of the topological boundary states. The proposed all‐dielectric HOTI metasurface offers a new approach to confine the optical field in micro‐ and nano‐scale topological cavities and thus paves the way to achieve a novel nanophotonic technology.  more » « less
Award ID(s):
1641069 1626101
PAR ID:
10359873
Author(s) / Creator(s):
 ;  ;  ;  ;  ;  ;  ;  ;  ;  
Publisher / Repository:
Wiley Blackwell (John Wiley & Sons)
Date Published:
Journal Name:
Advanced Materials
Volume:
33
Issue:
18
ISSN:
0935-9648
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Classical wave systems have constituted an excellent platform for emulating complex quantum phenomena, such as demonstrating topological phenomena in photonics and acoustics. Recently, a new class of topological states localized in more than one dimension of a D -dimensional system, referred to as higher-order topological (HOT) states, has been reported, offering an even more versatile platform to confine and control classical radiation and mechanical motion. Here, we design and experimentally study a 3D topological acoustic metamaterial supporting third-order (0D) topological corner states along with second-order (1D) edge states and first-order (2D) surface states within the same topological bandgap, thus establishing a full hierarchy of nontrivial bulk polarization–induced states in three dimensions. The assembled 3D topological metamaterial represents the acoustic analog of a pyrochlore lattice made of interconnected molecules, and is shown to exhibit topological bulk polarization, leading to the emergence of boundary states. 
    more » « less
  2. Abstract The rise of quantum science and technologies motivates photonics research to seek new platforms with strong light-matter interactions to facilitate quantum behaviors at moderate light intensities. Topological polaritons (TPs) offer an ideal platform in this context, with unique properties stemming from resilient topological states of light strongly coupled with matter. Here we explore polaritonic metasurfaces based on 2D transition metal dichalcogenides (TMDs) as a promising platform for topological polaritonics. We show that the strong coupling between topological photonic modes of the metasurface and excitons in TMDs yields a topological polaritonic Z2phase. We experimentally confirm the emergence of one-way spin-polarized edge TPs in metasurfaces integrating MoSe2and WSe2. Combined with the valley polarization in TMD monolayers, the proposed system enables an approach to engage the photonic angular momentum and valley and spin of excitons, offering a promising platform for photonic/solid-state interfaces for valleytronics and spintronics. 
    more » « less
  3. Due to the enhanced nature of the interactions of light with quantum excitations, topological polaritonic (TP) systems form a unique platform that offers on‐chip control over half‐light, half‐matter excitations via synthetic degrees of freedom. Among other polaritonic platforms, van der Waals materials (vdW) have recently attracted significant interest due to the relative simplicity of their integration into topological photonic structures. Several TP insulators based on vdW materials have been demonstrated; however, they rely on hybrid structures with nanopatterned dielectric substrates, which limit the strength of light‐matter interactions. Here, a monolithic all‐vdW TP insulator based on bulk crystals of transition metal dichalcogenide WS2is designed and experimentally realized. Due to their high refractive index and the presence of exciton modes, these nanomaterials prove to be excellent platforms for TPs, offering both excellent confinement and strong light‐matter interactions in monolithic structures. The emergence of TP boundary modes is confirmed by Fourier and real‐space imaging, and a dramatic reduction in dissipation is observed at cryogenic temperatures. The proposed monolithic all‐vdW topological insulators, which are characterized by extreme confinement of optical fields and moderate losses, can serve as an alternative to silicon photonics‐based systems in the quest for the development of polaritonic quantum technologies. 
    more » « less
  4. A topological phase transition in high-temperature superconductor FeTe1−xSex, occurring at a critical range of Se concentration x, underlies their intrinsic topological superconductivity and emergence of Majorana states within vortices. However, how Se concentration and distribution determine the electronic states, particularly the presence or absence of Majorana states, in FeTe1−xSex remains unclear. In this study, we combine density functional theory calculations with pz–dxz/yz-based analysis and Wannier-based Hamiltonian analysis to systematically explore the electronic structures of diverse FeTe1−xSex compositions. Our investigation reveals a nonlinear variation of the spin–orbit coupling (SOC) gap between pz and dxz/yz bands in response to the Se concentration x, with the maximum gap occurring at x = 0.5. The pz–pz and dx2−y2–pz interactions are found to be critical for pd band inversion. Furthermore, the distribution of Se significantly modulates the SOC gap, thereby influencing the emergence of Majorana states within local vortices. 
    more » « less
  5. Abstract The recent discovery of topological flat bands in twisted transition metal dichalcogenide homobilayers and multilayer graphene has sparked significant research interest. Here, a new platform for realizing tunable topological moiré flat bands: twisted type‐II Rashba homobilayers, is proposed. By maintaining centrosymmetry, the interplay between Rashba spin‐orbit coupling and interlayer interactions generates an effective pseudo‐antiferromagnetic field, opening a gap within the Dirac cone with non‐zero Berry curvature. Using twisted BiTeI bilayers as an example, it is predicted that the emergence of flat topological bands with a remarkably narrow bandwidth (below 20 meV). Notably, the system undergoes a transition from a valley Hall insulator to a quantum spin Hall insulator as the twisting angle increases. This transition arises from a competition between the twisting‐driven effective spin‐orbit coupling and sublattice onsite energies presented in type‐II Rashba moiré structures. The high tunability of Rashba materials in terms of the spin‐orbit coupling strength, interlayer interaction, and twisting angle expands the range of materials suitable for functionalizing and manipulating correlated topological properties. 
    more » « less