Recent observational studies have shown that stratospheric air rich in ozone (O3) is capable of being transported into the upper troposphere in association with tropopause‐penetrating convection (anvil wrapping). This finding challenges the current understanding of upper tropospheric sources of O3, which is traditionally thought to come from thunderstorm outflows where lightning‐generated nitrogen oxides facilitate O3formation. Since tropospheric O3is an important greenhouse gas and the frequency and strength of tropopause‐penetrating storms may change in a changing climate, it is important to understand the mechanisms driving this transport process so that it can be better represented in chemistry‐climate models. Simulations of a mesoscale convective system (MCS) around which this transport process was observed are performed using the Weather Research and Forecasting model coupled with Chemistry. The Weather Research and Forecasting model coupled with Chemistry model adequately simulates anvil wrapping of ozone‐rich air. Possible mechanisms that influence the transport, including small‐scale static and dynamic instabilities and MCS‐induced mesoscale circulations, are evaluated. Model results suggest that anvil wrapping is a two‐step transport process (1) compensating subsidence surrounding the MCS, which is driven by mass conservation as the MCS transports tropospheric air into the upper troposphere and lower stratosphere, followed by (2) differential advection beneath the core of the MCS upper‐tropospheric outflow jet which wraps high O3air around and under the MCS cloud anvil. Static and dynamic instabilities are not a leading contributor to this transport process. Continued fine‐scale modeling of these events is needed to fully represent the stratosphere‐to‐troposphere transport process.
On the Formation of Tropopause Folds and Constituent Gradient Enhancement Near Westerly Jets
Abstract The role of differential advection in creating tropopause folds and strong constituent gradients near midlatitude westerly jets is investigated using the University of Wisconsin Non-hydrostatic Modeling System (UWNMS). Dynamical structures are compared with aircraft observations through a fold and subpolar jet (SPJ) during RF04 of the Stratosphere-Troposphere Analyses of Regional Transport (START08) campaign. The observed distribution of water vapor and ozone during RF04 provides evidence of rapid transport in the SPJ, enhancing constituent gradients above relative to below the intrusion. The creation of a tropopause fold by quasi-isentropic differential advection on the upstream side of the trough is described. This fold was created by a southward jet streak in the SPJ, where upper tropospheric air displaced the tropopause eastward in the 6-10 km layer, thereby overlying stratospheric air in the 3-6 km layer. The subsequent superposition of the subtropical and subpolar jets is also shown to result from quasi-isentropic differential advection. The occurrence of low values of ozone, water vapor, and potential vorticity on the equatorward side of the SPJ can be explained by convective transport of low-ozone air from the boundary layer, dehydration in the updraft, and detrainment of inertially-unstable air in the outflow layer. An example of rapid juxtaposition with stratospheric air in the jet core is shown for RF01. The net effect of upstream convective events is suggested as a fundamental cause of the strong constituent gradients observed in midlatitude jets. Idealized diagrams illustrate the role of differential advection in creating tropopause folds and constituent gradient enhancement.
more »
« less
- Award ID(s):
- 1947658
- NSF-PAR ID:
- 10318123
- Date Published:
- Journal Name:
- Journal of the Atmospheric Sciences
- ISSN:
- 0022-4928
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
more » « less
Abstract -
Abstract. The El Niño–Southern Oscillation (ENSO) is known to modulate the strength and frequency of stratosphere-to-troposphere transport (STT) of ozone over the Pacific–North American region during late winter to early summer. Dynamical processes that have been proposed to account for this variability include variations in the amount of ozone in the lowermoststratosphere that is available for STT and tropospheric circulation-relatedvariations in the frequency and geographic distribution of individual STTevents. Here we use a large ensemble of Whole Atmosphere Community Climate Model(WACCM) simulations (forced by sea-surface temperature (SST) boundaryconditions consistent with each phase of ENSO) to show that variability inlower-stratospheric ozone and shifts in the Pacific tropospheric jetconstructively contribute to the amount of STT of ozone in the NorthAmerican region during both ENSO phases. In terms of stratosphericvariability, ENSO drives ozone anomalies resembling the Pacific–NorthAmerican teleconnection pattern that span much of the lower stratospherebelow 50 hPa. These ozone anomalies, which dominate over other ENSO-drivenchanges in the Brewer–Dobson circulation (including changes due to both thestratospheric residual circulation and quasi-isentropic mixing), stronglymodulate the amount of ozone available for STT transport. As a result,during late winter (February–March), the stratospheric ozone response to theteleconnections constructively reinforces anomalous ENSO-jet-driven STT ofozone. However, as ENSO forcing weakens as spring progresses into summer(April–June), the direct effects of the ENSO-jet-driven STT transportweaken. Nevertheless, the residual impacts of the teleconnections on theamount of ozone in the lower stratosphere persist, and these anomalies inturn continue to cause anomalous STT of ozone. These results should provehelpful for interpreting the utility of ENSO as a subseasonal predictor ofboth free-tropospheric ozone and the probability of stratospheric ozoneintrusion events that may cause exceedances in surface air qualitystandards.more » « less
-
Abstract. Stratosphere-to-troposphere transport (STT) is an important sourceof ozone for the troposphere, particularly over western North America. STTin this region is predominantly controlled by a combination of thevariability and location of the Pacific jet stream and the amount of ozonein the lower stratosphere, two factors which are likely to change ifgreenhouse gas concentrations continue to increase. Here we use WholeAtmosphere Community Climate Model experiments with a tracer ofstratospheric ozone (O3S) to study how end-of-the-century RepresentativeConcentration Pathway (RCP) 8.5 sea surface temperatures (SSTs) andgreenhouse gases (GHGs), in isolation and in combination, influence STT ofozone over western North America relative to a preindustrial controlbackground state. We find that O3S increases by up to 37 % during late winter at 700 hPaover western North America in response to RCP8.5 forcing, with the increasestapering off somewhat during spring and summer. When this response to RCP8.5greenhouse gas forcing is decomposed into the contributions made by futureSSTs alone versus future GHGs alone, the latter are found to be primarilyresponsible for these O3S changes. Both the future SSTs alone and the futureGHGs alone accelerate the Brewer–Dobson circulation, which modifiesextratropical lower-stratospheric ozone mixing ratios. While the future GHGsalone promote a more zonally symmetric lower-stratospheric ozone change dueto enhanced ozone production and some transport, the future SSTs aloneincrease lower-stratospheric ozone predominantly over the North Pacific viatransport associated with a stationary planetary-scale wave. Ozoneaccumulates in the trough of this anomalous wave and is reduced over thewave's ridges, illustrating that the composition of the lower-stratosphericozone reservoir in the future is dependent on the phase and position of thestationary planetary-scale wave response to future SSTs alone, in additionto the poleward mass transport provided by the accelerated Brewer–Dobsoncirculation. Further, the future SSTs alone account for most changes to thelarge-scale circulation in the troposphere and stratosphere compared to theeffect of future GHGs alone. These changes include modifying the positionand speed of the future North Pacific jet, lifting the tropopause,accelerating both the Brewer–Dobson circulation's shallow and deep branches,and enhancing two-way isentropic mixing in the stratosphere.more » « less
-
more » « less
Abstract Perturbations to the potential vorticity (PV) waveguide, which can result from latent heat release within the warm conveyor belt (WCB) of midlatitude cyclones, can lead to the downstream radiation of Rossby waves, and in turn high-impact weather events. Previous studies have hypothesized that forecast uncertainty associated with diabatic heating in WCBs can result in large downstream forecast variability; however, these studies have not established a direct connection between the two. This study evaluates the potential impact of latent heating variability in the WCB on subsequent downstream forecasts by applying the ensemble-based sensitivity method to European Centre for Medium-Range Weather Forecasts (ECMWF) ensemble forecasts of a cyclogenesis event over the North Atlantic. For this case, ensemble members with a more amplified ridge are associated with greater negative PV advection by the irrotational wind, which is associated with stronger lower-tropospheric southerly moisture transport east of the upstream cyclone in the WCB. This transport is sensitive to the pressure trough to the south of the cyclone along the cold front, which in turn is modulated by earlier differences in the motion of the air masses on either side of the front. The position of the cold air behind the front is modulated by upstream tropopause-based PV anomalies, such that a deeper pressure trough is associated with a more progressive flow pattern, originating from Rossby wave breaking over the North Pacific. Overall, these results suggest that more accurate forecasts of upstream PV anomalies and WCBs may reduce forecast uncertainty in the downstream waveguide.
-
Abstract. Here we present a newly developed ice core gas-phase proxy that directlysamples a component of the large-scale atmospheric circulation:synoptic-scale pressure variability. Surface pressure changes weakly disrupt gravitational isotopic settling in the firn layer, which is recorded in krypton-86 excess (86Krxs). The 86Krxs may therefore reflect the time-averaged synoptic pressure variability over several years (site “storminess”), but it likely cannot record individual synoptic events as ice core gas samples typically average over several years. We validate 86Krxs using late Holocene ice samples from 11 Antarctic ice cores and 1 Greenland ice core that collectively represent a wide range of surface pressure variability in the modern climate. We find a strong spatial correlation (r=-0.94, p<0.01) between site average 86Krxs and time-averaged synoptic variability from reanalysis data. The main uncertainties in the analysis are the corrections for gas loss and thermal fractionation and the relatively large scatter in the data. Limited scientific understanding of the firn physics and potential biases of 86Krxs require caution in interpreting this proxy at present. We show that Antarctic 86Krxs appears to be linked to the position of the Southern Hemisphere eddy-driven subpolar jet (SPJ), with a southern position enhancing pressure variability. We present a 86Krxs record covering the last 24 kyr from the West Antarctic Ice Sheet (WAIS) Divide ice core. Based on the empirical spatial correlation of synoptic activity and 86Krxs at various Antarctic sites, we interpret this record to show that West Antarctic synoptic activity is slightly below modern levels during the Last Glacial Maximum (LGM), increases during the Heinrich Stadial 1 and Younger Dryas North Atlantic cold periods, weakens abruptly at the Holocene onset, remains low during the early and mid-Holocene, and gradually increases to its modern value. The WAIS Divide 86Krxs record resembles records of monsoon intensity thought to reflect changes in the meridional position of the Intertropical Convergence Zone (ITCZ) on orbital and millennial timescales such that West Antarctic storminess is weaker when the ITCZ is displaced northward and stronger when it is displaced southward. We interpret variations in synoptic activity as reflecting movement of the South Pacific SPJ in parallel to the ITCZ migrations, which is the expected zonal mean response of the eddy-driven jet in models and proxy data. Past changes to Pacific climate and the El Niño–Southern Oscillation (ENSO) may amplify the signal of the SPJ migration. Our interpretation is broadly consistent with opal flux records from the Pacific Antarctic zone thought to reflect wind-driven upwelling. We emphasize that 86Krxs is a new proxy, and more work is called for to confirm, replicate, and better understand these results; until such time, our conclusions regarding past atmospheric dynamics remainspeculative. Current scientific understanding of firn air transport andtrapping is insufficient to explain all the observed variations in86Krxs. A list of suggested future studies is provided.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1175/JAS-D-20-0013.1
