We report spectroscopic and time-resolved experimental observations to characterize the state in ions. We access this state from the metastable manifold and observe an unexpectedly long lifetime of that allows visible Rabi oscillations and resolved-sideband spectroscopy. Using a combination of coherent population dynamics, high-fidelity detection and heralded state preparation, and optical pumping methods, we measure the branching ratios to the , and states to be , 0.639(2), and , respectively. The branching ratio to the is compatible with zero within our experimental resolution. We also report measurements of Landé -factor of the state. Further, the branching ratio of the to decay in was measured to be 0.188(3), improving its relative uncertainty by an order of magnitude. Our measurements provide experimental benchmarks for better understanding the atomic structure of ions, which still lacks accurate numerical descriptions, and the use of high-lying excited states for partial detection and qubit manipulation in the architecture.
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Measurements of the 5D4∘−5P3 transition of singly ionized atomic iodine using intermodulated laser induced fluorescence
- Award ID(s):
- 1827325
- PAR ID:
- 10320922
- Date Published:
- Journal Name:
- Journal of Quantitative Spectroscopy and Radiative Transfer
- Volume:
- 277
- Issue:
- C
- ISSN:
- 0022-4073
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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