Holographic particle characterization uses in-line holographic microscopy and the Lorenz-Mie theory of light scattering to measure the diameter and the refractive index of individual colloidal particles in their native dispersions. This wealth of information has proved invaluable in fields as diverse as soft-matter physics, biopharmaceuticals, wastewater management, and food science but so far has been available only for dispersions in transparent media. Here, we demonstrate that holographic characterization can yield precise and accurate results even when the particles of interest are dispersed in turbid media. By elucidating how multiple light scattering contributes to image formation in holographic microscopy, we establish the range conditions under which holographic characterization can reliably probe turbid samples. We validate the technique with measurements on model colloidal spheres dispersed in commercial nanoparticle slurries.
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Beyond mie theory: systematic computation of bulk scattering parameters based on microphysical wave optics
Light scattering in participating media and translucent materials is typically modeled using the radiative transfer theory. Under the assumption of independent scattering between particles, it utilizes several bulk scattering parameters to statistically characterize light-matter interactions at the macroscale. To calculate these parameters based on microscale material properties, the Lorenz-Mie theory has been considered the gold standard. In this paper, we present a generalized framework capable of systematically and rigorously computing bulk scattering parameters beyond the far-field assumption of Lorenz-Mie theory. Our technique accounts for microscale wave-optics effects such as diffraction and interference as well as interactions between nearby particles. Our framework is general, can be plugged in any renderer supporting Lorenz-Mie scattering, and allows arbitrary packing rates and particles correlation; we demonstrate this generality by computing bulk scattering parameters for a wide range of materials, including anisotropic and correlated media.
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- Award ID(s):
- 1813553
- PAR ID:
- 10345696
- Date Published:
- Journal Name:
- ACM Transactions on Graphics
- Volume:
- 40
- Issue:
- 6
- ISSN:
- 0730-0301
- Page Range / eLocation ID:
- 1 to 12
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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