skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Topological phonon-polariton funneling in midinfrared metasurfaces
Topological photonics offers enhanced control over electromagnetic fields by providing a platform for robust trapping and guiding of topological states of light. By combining the strong coupling between topological photons with phonons in hexagonal boron nitride (hBN), we demonstrate a platform to control and guide hybrid states of light and lattice vibrations. The observed topological edge states of phonon-polaritons are found to carry nonzero angular momentum locked to their propagation direction, which enables their robust transport. Thus, these topological quasiparticles enable the funneling of infrared phonons mediated by helical infrared photons along arbitrary pathways and across sharp bends, thereby offering opportunities for applications ranging from Raman and vibrational spectroscopy with structured phonon-polaritons to directional heat dissipation.  more » « less
Award ID(s):
1809915
PAR ID:
10347553
Author(s) / Creator(s):
; ; ; ; ; ; ;
Date Published:
Journal Name:
Science
Volume:
374
Issue:
6564
ISSN:
0036-8075
Page Range / eLocation ID:
225 to 227
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract Polar dielectrics are key materials of interest for infrared (IR) nanophotonic applications due to their ability to host phonon‐polaritons that allow for low‐loss, subdiffractional control of light. The properties of phonon‐polaritons are limited by the characteristics of optical phonons, which are nominally fixed for most “bulk” materials. Superlattices composed of alternating atomically thin materials offer control over crystal anisotropy through changes in composition, optical phonon confinement, and the emergence of new modes. In particular, the modified optical phonons in superlattices offer the potential for so‐called crystalline hybrids whose IR properties cannot be described as a simple mixture of the bulk constituents. To date, however, studies have primarily focused on identifying the presence of new or modified optical phonon modes rather than assessing their impact on the IR response. This study focuses on assessing the impact of confined optical phonon modes on the hybrid IR dielectric function in superlattices of GaSb and AlSb. Using a combination of first principles theory, Raman, FTIR, and spectroscopic ellipsometry, the hybrid dielectric function is found to track the confinement of optical phonons, leading to optical phonon spectral shifts of up to 20 cm−1. These results provide an alternative pathway toward designer IR optical materials. 
    more » « less
  2. Abstract Heat conduction in solids is typically governed by the Fourier’s law describing a diffusion process due to the short wavelength and mean free path for phonons and electrons. Surface phonon polaritons couple thermal photons and optical phonons at the surface of polar dielectrics, possessing much longer wavelength and propagation length, representing an excellent candidate to support extraordinary heat transfer. Here, we realize clear observation of thermal conductivity mediated by surface phonon polaritons in SiO2nanoribbon waveguides of 20-50 nm thick and 1-10 μm wide and also show non-Fourier behavior in over 50-100 μm distance at room and high temperature. This is enabled by rational design of the waveguide to control the mode size of the surface phonon polaritons and its efficient coupling to thermal reservoirs. Our work laid the foundation for manipulating heat conduction beyond the traditional limit via surface phonon polaritons waves in solids. 
    more » « less
  3. Efficient control of photons is enabled by hybridizing light with matter. The resulting light-matter quasi-particles can be readily programmed by manipulating either their photonic or matter constituents. Here, we hybridized infrared photons with graphene Dirac electrons to form surface plasmon polaritons (SPPs) and uncovered a previously unexplored means to control SPPs in structures with periodically modulated carrier density. In these periodic structures, common SPPs with continuous dispersion are transformed into Bloch polaritons with attendant discrete bands separated by bandgaps. We explored directional Bloch polaritons and steered their propagation by dialing the proper gate voltage. Fourier analysis of the near-field images corroborates that this on-demand nano-optics functionality is rooted in the polaritonic band structure. Our programmable polaritonic platform paves the way for the much-sought benefits of on-the-chip photonic circuits. 
    more » « less
  4. Abstract The topological features of optical vortices have been opening opportunities for free-space and on-chip photonic technologies, e.g., for multiplexed optical communications and robust information transport. In a parallel but disjoint effort, polar anisotropic van der Waals nanomaterials supporting hyperbolic phonon polaritons (HP 2 s) have been leveraged to drastically boost light-matter interactions. So far HP 2 studies have been mainly focusing on the control of their amplitude and scale features. Here we report the generation and observation of mid-infrared hyperbolic polariton vortices (HP 2 Vs) associated with reconfigurable topological charges. Spiral-shaped gold disks coated with a flake of hexagonal boron nitride are exploited to tailor spin–orbit interactions and realise deeply subwavelength HP 2 Vs. The complex interplay between excitation spin, spiral geometry and HP 2 dispersion enables robust reconfigurability of the associated topological charges. Our results reveal unique opportunities to extend the application of HP 2 s into topological photonics, quantum information processing by integrating these phenomena with single-photon emitters, robust on-chip optical applications, sensing and nanoparticle manipulation. 
    more » « less
  5. Abstract Phonon polaritons (PhPs), excitations arising from the coupling of light with lattice vibrations, enable light confinement and local field enhancement, which is essential for various photonic and thermal applications. To date, PhPs with high confinement and low loss are mainly observed in the mid‐infrared regime and mostly in manually exfoliated flakes of van der Waals (vdW) materials. In this work, the existence of low‐loss, thickness‐tunable phonon polaritons in the far‐infrared regime within transferable freestanding SrTiO3membranes synthesized through a scalable approach, achieving high figures of merit is demonstrated, which are comparable to the previous record values from the vdW materials. Leveraging atomic precision in thickness control, large dimensions, and compatibility with mature oxide electronics, functional oxide membranes present a promising large‐scale 2D platform alternative to vdW materials for on‐chip polaritonic technologies in the infrared regime. 
    more » « less