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1. Electric-field control of spin dynamics during magnetic phase transitions

   https://doi.org/10.1126/sciadv.abd2613  

   Nan, Tianxiang; Lee, Yeonbae; Zhuang, Shihao; Hu, Zhongqiang; Clarkson, James D.; Wang, Xinjun; Ko, Changhyun; Choe, HwanSung; Chen, Zuhuang; Budil, David; et al (October 2020, Science Advances)

   null (Ed.)

   Controlling magnetization dynamics is imperative for developing ultrafast spintronics and tunable microwave devices. However, the previous research has demonstrated limited electric-field modulation of the effective magnetic damping, a parameter that governs the magnetization dynamics. Here, we propose an approach to manipulate the damping by using the large damping enhancement induced by the two-magnon scattering and a nonlocal spin relaxation process in which spin currents are resonantly transported from antiferromagnetic domains to ferromagnetic matrix in a mixed-phased metallic alloy FeRh. This damping enhancement in FeRh is sensitive to its fraction of antiferromagnetic and ferromagnetic phases, which can be dynamically tuned by electric fields through a strain-mediated magnetoelectric coupling. In a heterostructure of FeRh and piezoelectric PMN-PT, we demonstrated a more than 120% modulation of the effective damping by electric fields during the antiferromagnetic-to-ferromagnetic phase transition. Our results demonstrate an efficient approach to controlling the magnetization dynamics, thus enabling low-power tunable electronics. 

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2. Symmetry Control of Unconventional Spin–Orbit Torques in IrO ₂

   https://doi.org/10.1002/adma.202301608  

   Patton, Michael; Gurung, Gautam; Shao, Ding‐Fu; Noh, Gahee; Mittelstaedt, Joseph A.; Mazur, Marcel; Kim, Jong‐Woo; Ryan, Philip J.; Tsymbal, Evgeny Y.; Choi, Si‐Young; et al (July 2023, Advanced Materials)

   Abstract Spin–orbit torques generated by a spin current are key to magnetic switching in spintronic applications. The polarization of the spin current dictates the direction of switching required for energy‐efficient devices. Conventionally, the polarizations of these spin currents are restricted to be along a certain direction due to the symmetry of the material allowing only for efficient in‐plane magnetic switching. Unconventional spin–orbit torques arising from novel spin current polarizations, however, have the potential to switch other magnetization orientations such as perpendicular magnetic anisotropy, which is desired for higher density spintronic‐based memory devices. Here, it is demonstrated that low crystalline symmetry is not required for unconventional spin–orbit torques and can be generated in a nonmagnetic high symmetry material, iridium dioxide (IrO₂), using epitaxial design. It is shown that by reducing the relative crystalline symmetry with respect to the growth direction large unconventional spin currents can be generated and hence spin–orbit torques. Furthermore, the spin polarizations detected in (001), (110), and (111) oriented IrO₂thin films are compared to show which crystal symmetries restrict unconventional spin transport. Understanding and tuning unconventional spin transport generation in high symmetry materials can provide a new route towards energy‐efficient magnetic switching in spintronic devices. 

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3. Ultra-thin lithium aluminate spinel ferrite films with perpendicular magnetic anisotropy and low damping

   https://doi.org/10.1038/s41467-023-40733-9  

   Zheng, Xin Yu; Channa, Sanyum; Riddiford, Lauren J; Wisser, Jacob J; Mahalingam, Krishnamurthy; Bowers, Cynthia T; McConney, Michael E; N’Diaye, Alpha T; Vailionis, Arturas; Cogulu, Egecan; et al (December 2023, Nature Communications)

   Abstract Ultra-thin films of low damping ferromagnetic insulators with perpendicular magnetic anisotropy have been identified as critical to advancing spin-based electronics by significantly reducing the threshold for current-induced magnetization switching while enabling new types of hybrid structures or devices. Here, we have developed a new class of ultra-thin spinel structure Li_0.5Al_1.0Fe_1.5O₄(LAFO) films on MgGa₂O₄(MGO) substrates with: 1) perpendicular magnetic anisotropy; 2) low magnetic damping and 3) the absence of degraded or magnetic dead layers. These films have been integrated with epitaxial Pt spin source layers to demonstrate record low magnetization switching currents and high spin-orbit torque efficiencies. These LAFO films on MGO thus combine all of the desirable properties of ferromagnetic insulators with perpendicular magnetic anisotropy, opening new possibilities for spin based electronics. 

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4. Large spin–orbit torque in bismuthate-based heterostructures

   https://doi.org/10.1038/s41928-023-01080-1  

   Edgeton, Anthony L; Harris, Isaac A; Campbell, Neil G; Chai, Yahong; Mazur, Marcel M; Gurung, Gautam; Huang, Xiaoxi; Susarla, Sandhya; Tsymbal, Evgeny Y; Ralph, Daniel C; et al (December 2023, Nature Electronics)

   The wider application of spintronic devices requires the development of new material platforms that can efficiently manipulate spin. Bismuthate-based superconductors are centrosymmetric systems that are generally thought to offer weak spin–orbit coupling. Here, we report a large spin–orbit torque driven by spin polarization generated in heterostructures based on the bismuthate BaPb1-xBixO3 (which is in a non-superconducting state). Using spin-torque ferromagnetic resonance and d.c. non-linear Hall measurements, we measure a spin–orbit torque efficiency of around 2.7 and demonstrate current driven magnetization switching at current densities of 4×10^5 A〖cm〗^(-2). We suggest that the unexpectedly large current-induced torques could be the result of an orbital Rashba effect associated with local inversion symmetry breaking in BaPb1-xBixO3. 

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5. Angular dependence of spin-orbit torque in monolayer ${\mathrm{Fe}}_3{\mathrm{GeTe}}_2$

   https://doi.org/10.1103/PhysRevB.108.144422  

   Xue, Fei; Stiles, Mark D.; Haney, Paul M. (October 2023, Physical Review B)

   In ferromagnetic systems lacking inversion symmetry, an applied electric field can control the ferromagnetic order parameters through the spin-orbit torque. The prototypical example is a bilayer heterostructure composed of a ferromagnet and a heavy metal that acts as a spin current source. In addition to such bilayers, spin-orbit coupling can mediate spin-orbit torques in ferromagnets that lack bulk inversion symmetry. A recently discovered example is the two-dimensional monolayer ferromagnet Fe3GeTe2. In this paper, we use first-principles calculations to study the spin-orbit torque and ensuing magnetic dynamics in this material. By expanding the torque versus magnetization direction as a series of vector spherical harmonics, we find that higher order terms (up to ℓ=4) are significant and play important roles in the magnetic dynamics. They give rise to deterministic, magnetic field-free electrical switching of perpendicular magnetization. 

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