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Quantum states of light can enable sensing configurations with sensitivities beyond the shot-noise limit (SNL). In order to better take advantage of available quantum resources and obtain the maximum possible sensitivity, it is necessary to determine fundamental sensitivity limits for different possible configurations for a given sensing system. Here, due to their wide applicability, we focus on optical resonance sensors, which detect a change in a parameter of interest through a resonance shift. We compare their fundamental sensitivity limits set by the quantum Cramér-Rao bound (QCRB) based on the estimation of changes in transmission or phase of a probing bright two-mode squeezed state (bTMSS) of light. We show that the fundamental sensitivity results from an interplay between the QCRB and the transfer function of the system. As a result, for a resonance sensor with a Lorentzian lineshape a phase-based scheme outperforms a transmission-based one for most of the parameter space; however, this is not the case for lineshapes with steeper slopes, such as higher order Butterworth lineshapes. Furthermore, such an interplay results in conditions under which the phase-based scheme provides a higher sensitivity but a smaller degree of quantum enhancement than the transmission-based scheme. We also study the effect of losses external to the sensor on the degree of quantum enhancement and show that for certain conditions, probing with a classical state can provide a higher sensitivity than probing with a bTMSS. Finally, we discuss detection schemes, namely optimized intensity-difference and optimized homodyne detection, that can achieve the fundamental sensitivity limits even in the presence of external losses.
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Fast phase cycling in non-collinear optical two-dimensional coherent spectroscopy
As optical two-dimensional coherent spectroscopy (2DCS) is extended to a broader range of applications, it is critical to improve the detection sensitivity of optical 2DCS. We developed a fast phase-cycling scheme in a non-collinear optical 2DCS implementation by using liquid crystal phase retarders to modulate the phases of two excitation pulses. The background in the signal can be eliminated by combining either two or four interferograms measured with a proper phase configuration. The effectiveness of this method was validated in optical 2DCS measurements of an atomic vapor. This fast phase-cycling scheme will enable optical 2DCS in novel emerging applications that require enhanced detection sensitivity.
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- Award ID(s):
- 1707364
- PAR ID:
- 10371332
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Optics Letters
- Volume:
- 45
- Issue:
- 20
- ISSN:
- 0146-9592; OPLEDP
- Format(s):
- Medium: X Size: Article No. 5852
- Size(s):
- Article No. 5852
- Sponsoring Org:
- National Science Foundation
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