ℏω versus ℏk: dispersion and energy constraints on time-varying photonic materials and time crystals [Invited]

Photonic time-varying systems have attracted significant attention owing to their rich physics and potential opportunities for new and enhanced functionalities. In this context, the duality of space and time in wave physics has been particularly fruitful to uncover interesting physical effects in the temporal domain, such as reflection/refraction at temporal interfaces and momentum-bandgaps in time crystals. However, the characteristics of the temporal/frequency dimension, particularly its relation to causality and energy conservation ($ℏ<#comment/>ω<#comment/>$is energy, whereas$ℏ<#comment/>k$is momentum), create challenges and constraints that are unique to time-varying systems and are not present in their spatially varying counterparts. Here, we overview two key physical aspects of time-varying photonics that have only received marginal attention so far, namely temporal dispersion and external power requirements, and explore their implications. We discuss how temporal dispersion, an inherent property of any physical causal material, makes the fields evolve continuously at sharp temporal interfaces and may limit the strength of fast temporal modulations and of various resulting effects. Furthermore, we show that changing the refractive index in time always involves large amounts of energy. We derive power requirements to observe a time-crystal response in one of the most popular material platforms in time-varying photonics, more »

Authors:
; ;
Publication Date:
NSF-PAR ID:
10371574
Journal Name:
Optical Materials Express
Volume:
12
Issue:
10
Page Range or eLocation-ID:
Article No. 3904
ISSN:
2159-3930
Publisher:
Optical Society of America
1. High-gain optical parametric amplification is an important nonlinear process used both as a source of coherent infrared light and as a source of nonclassical light. In this work, we experimentally demonstrate an approach to optical parametric amplification that enables extremely large parametric gains with low energy requirements. In conventional nonlinear media driven by femtosecond pulses, multiple dispersion orders limit the effective interaction length available for parametric amplification. Here, we use the dispersion engineering available in periodically poled thin-film lithium niobate nanowaveguides to eliminate several dispersion orders at once. The result is a quasi-static process; the large peak intensity associated with a short pump pulse can provide gain to signal photons without undergoing pulse distortion or temporal walk-off. We characterize the parametric gain available in these waveguides using optical parametric generation, where vacuum fluctuations are amplified to macroscopic intensities. In the unsaturated regime, we observe parametric gains as large as 71 dB (118 dB/cm) spanning 1700–2700 nm with pump energies of only 4 pJ. When driven with pulse energies$><#comment/>10pJ$, we observe saturated parametric gains as large as 88 dB ($><#comment/>146dB/cm$). The devices shown heremore »
2. Materials with strong second-order ($χ<#comment/>(2)$) optical nonlinearity, especially lithium niobate, play a critical role in building optical parametric oscillators (OPOs). However, chip-scale integration of low-loss$χ<#comment/>(2)$materials remains challenging and limits the threshold power of on-chip$χ<#comment/>(2)$OPO. Here we report an on-chip lithium niobate optical parametric oscillator at the telecom wavelengths using a quasi-phase-matched, high-quality microring resonator, whose threshold power ($∼<#comment/>30µ<#comment/>W$) is 400 times lower than that in previous$χ<#comment/>(2)$integrated photonics platforms. An on-chip power conversion efficiency of 11% is obtained from pump to signal and idler fields at a pump power of 93 µW. The OPO wavelength tuning is achieved by varying the pump frequency and chip temperature. With the lowest power threshold among all on-chip OPOs demonstrated so far, as well as advantages including high conversion efficiency, flexibility in quasi-phase-matching, and device scalability, the thin-film lithium niobate OPO opens new opportunities for chip-based tunable classical and quantum light sources and provides a potential platform for realizing photonic neural networks.
3. Ultrashort pulses propagating in nonlinear nanophotonic waveguides can simultaneously leverage both temporal and spatial field confinement, promising a route towards single-photon nonlinearities in an all-photonic platform. In this multimode quantum regime, however, faithful numerical simulations of pulse dynamics naïvely require a representation of the state in an exponentially large Hilbert space. Here, we employ a time-domain, matrix product state (MPS) representation to enable efficient simulations by exploiting the entanglement structure of the system. To extract physical insight from these simulations, we develop an algorithm to unravel the MPS quantum state into constituent temporal supermodes, enabling, e.g., access to the phase-space portraits of arbitrary pulse waveforms. As a demonstration, we perform exact numerical simulations of a Kerr soliton in the quantum regime. We observe the development of non-classical Wigner-function negativity in the solitonic mode as well as quantum corrections to the semiclassical dynamics of the pulse. A similar analysis of$χ<#comment/>(2)$simultons reveals a unique entanglement structure between the fundamental and second harmonics. Our approach is also readily compatible with quantum trajectory theory, allowing full quantum treatment of propagation loss and decoherence. We expect this work to establish the MPS technique as part of a unified engineering framework formore »
4. Thin-film lithium-niobate-on-insulator (LNOI) has emerged as a superior integrated-photonics platform for linear, nonlinear, and electro-optics. Here we combine quasi-phase-matching, dispersion engineering, and tight mode confinement to realize nonlinear parametric processes with both high efficiency and wide wavelength tunability. On a millimeter-long, Z-cut LNOI waveguide, we demonstrate efficient ($1900±<#comment/>500%<#comment/>W−<#comment/>1cm−<#comment/>2$) and highly tunable ($−<#comment/>1.71nm/K$) second-harmonic generation from 1530 to 1583 nm by type-0 quasi-phase-matching. Our technique is applicable to optical harmonic generation, quantum light sources, frequency conversion, and many other photonic information processes across visible to mid-IR spectral bands.
5. Traveling-wave optomechanical interactions, known as Brillouin interactions, have now been established as a powerful and versatile resource for photonic sources, sensors, and radio-frequency processors. However, established Brillouin-based interactions with sufficient interaction strengths involve short phonon lifetimes, which critically limit their performance for applications, including radio-frequency filtering and optomechanical storage devices. Here, we investigate a new paradigm of optomechanical interactions with tightly confined fundamental acoustic modes, which enables the unique and desirable combination of high optomechanical coupling, long phonon lifetimes, tunable phonon frequencies, and single-sideband amplification. Using sensitive four-wave mixing spectroscopy controlling for noise and spatial mode coupling, optomechanical interactions with long$><#comment/>2µ<#comment/>s$phonon lifetimes and strong$><#comment/>400W−<#comment/>1m−<#comment/>1$coupling are observed in a tapered fiber. In addition, we demonstrate novel phonon self-interference effects resulting from the unique combination of an axially varying device geometry with long phonon lifetimes. A generalized theoretical model, in excellent agreement with experiments, is developed with broad applicability to inhomogeneous optomechanical systems.