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1. Efficient second-harmonic generation in high Q-factor asymmetric lithium niobate metasurfaces

   https://doi.org/10.1364/OL.413764  

   Kang, Lei ; Bao, Huaguang ; Werner, Douglas H. ( January 2021 , Optics Letters)

   Lithium niobate (LN) has been widely used for second-harmonic generation (SHG) from bulk crystals. Recent studies have reported improved SHG efficiency in LN micro-ring resonators and hybrid waveguiding structures, as well as in LN nanostructures supporting anapole modes and plasmon-assisted dipole resonances. Here we numerically demonstrate that high$Q$-factor resonances associated with symmetry-protected bound states in the continuum can lead to highly efficient frequency doubling in LN metasurfaces. Simulations show that the radiative$Q$-factor and on-resonance field enhancement factor observed in the metasurface are closely dependent on the asymmetric parameter$\mathrm{\alpha <\#comment/>}$of the system. Furthermore, high$Q$-factor resonances boost the SH conversion process in the LN nanostructures. In particular, for a LN metasurface with a$Q$-factor of$\sim <\#comment/>8\times <\#comment/>{10}^4$, a 0.49% peak SH conversion efficiency is achieved at a pump intensity of$3.3{\mathrm{k}\mathrm{W}/\mathrm{c}\mathrm{m}}^2$. This suggests that such high$Q$-factor LN metasurfaces may be good candidates for practical blue–ultraviolet light sources. Our work provides insight into the possible implementation of metadevices based on nanoengineering of conventional nonlinear crystals.
2. Mid-IR spectroscopy of Er ³⁺ doped low-phonon CsCdCl ₃ and CsPbCl ₃ crystals

   https://doi.org/10.1364/JOSAB.470152  

   Brown, Ei Ei ; Fleischman, Zackery D. ; McKay, Jason ; Hommerich, Uwe ; Kabir, Al Amin ; Riggins, Jazmine ; Trivedi, Sudhir ; Dubinskii, Mark ( September 2022 , Journal of the Optical Society of America B)

   The mid-IR spectroscopic properties of${\mathrm{E}\mathrm{r}}^{3+}$doped low-phonon${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$crystals grown by the Bridgman technique have been investigated. Using optical excitations at$\sim <\#comment/>800\mathrm{n}\mathrm{m}$and$\sim <\#comment/>660\mathrm{n}\mathrm{m}$, both crystals exhibited IR emissions at$\sim <\#comment/>1.55$,$\sim <\#comment/>2.75$,$\sim <\#comment/>3.5$, and$\sim <\#comment/>4.5\text{µ<\#comment/>}\mathrm{m}$at room temperature. The mid-IR emission at 4.5 µm, originating from the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition, showed a long emission lifetime of$\sim <\#comment/>11.6\mathrm{m}\mathrm{s}$for${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$, whereas${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$exhibited a shorter lifetime of$\sim <\#comment/>1.8\mathrm{m}\mathrm{s}$. The measured emission lifetimes of the${}^4{\mathrm{I}}_{9/2}$state were nearly independent of the temperature, indicating a negligibly small nonradiative decay rate through multiphonon relaxation, as predicted by the energy-gap law for low-maximum-phonon energy hosts. The room temperature stimulatedmore »emission cross sections for the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition in${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$were determined to be$\sim <\#comment/>0.14\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$and$\sim <\#comment/>0.41\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$, respectively. The results of Judd–Ofelt analysis are presented and discussed.

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3. Terahertz nonlinear index extraction via full-phase analysis

   https://doi.org/10.1364/OL.399999  

   Garriga Francis, Kareem J. ; Lim Pac Chong, Mervin ; E, Yiwen ; Zhang, X. -C. ( October 2020 , Optics Letters)

   We experimentally show the spectrally averaged nonlinear refractive index and absorption coefficient for liquid water, water vapor,$\mathrm{\alpha <\#comment/>}$-pinene, and Si using a full-phase analysis in the terahertz regime through a standard time-domain spectrometer. Our results confirm that the nonlinear index of refraction of the liquid samples in this regime exceeds the near-infrared optical nonlinear index by six orders of magnitude. In the case of liquid water and water vapor at atmospheric pressure, we find a nonlinear index of$7.8\times <\#comment/>{10}^{-<\#comment/>10}{\mathrm{c}\mathrm{m}}^2/\mathrm{W}$and$6\times <\#comment/>{10}^{-<\#comment/>11}{\mathrm{c}\mathrm{m}}^2/\mathrm{W}$, respectively, which are both much larger than expected.
4. Spectroscopic study of the 4 f ⁷ 6 s ^{2 8} S 7/2∘−4 f ⁷ ( ⁸ S ^∘ )6 s 6 p ( ¹ P ^∘ ) ⁸ P _9/2 transition in neutral europium-151 and europium-153: absolute frequency and hyperfine structure

   https://doi.org/10.1364/JOSAB.467968  

   Herd, M. T. ; Maruko, C. ; Herzog, M. M. ; Brand, A. ; Cannon, G. ; Duah, B. ; Hollin, N. ; Karani, T. ; Wallace, A. ; Whitmore, M. ; et al ( September 2022 , Journal of the Optical Society of America B)

   We report on spectroscopic measurements on the$4f^{7}6s^2{}^8{S}_{7/2}^{\circ <\#comment/>}\to <\#comment/>4f^7{(}^8{S}^{\circ <\#comment/>})6s6p{(}^1{P}^{\circ <\#comment/>}){}^8{P}_{9/2}$transition in neutral europium-151 and europium-153 at 459.4 nm. The center of gravity frequencies for the 151 and 153 isotopes, reported for the first time in this paper, to our knowledge, were found to be 652,389,757.16(34) MHz and 652,386,593.2(5) MHz, respectively. The hyperfine coefficients for the$6s6p{(}^1{P}^{\circ <\#comment/>}){}^8{P}_{9/2}$state were found to be$\mathrm{A}(151)=-<\#comment/>228.84(2)\mathrm{M}\mathrm{H}\mathrm{z}$,$\mathrm{B}(151)=226.9(5)\mathrm{M}\mathrm{H}\mathrm{z}$and$\mathrm{A}(153)=-<\#comment/>101.87(6)\mathrm{M}\mathrm{H}\mathrm{z}$,$\mathrm{B}(153)=575.4(1.5)\mathrm{M}\mathrm{H}\mathrm{z}$, which all agree with previously published results except for A(153), which shows a small discrepancy. The isotope shift is found to be 3163.8(6) MHz, which also has a discrepancy with previously published results.
5. Ultralow-threshold thin-film lithium niobate optical parametric oscillator

   https://doi.org/10.1364/OPTICA.418984  

   Lu, Juanjuan ; Al Sayem, Ayed ; Gong, Zheng ; Surya, Joshua B. ; Zou, Chang-Ling ; Tang, Hong X. ( April 2021 , Optica)

   Materials with strong second-order (${\mathrm{\chi <\#comment/>}}^{(2)}$) optical nonlinearity, especially lithium niobate, play a critical role in building optical parametric oscillators (OPOs). However, chip-scale integration of low-loss${\mathrm{\chi <\#comment/>}}^{(2)}$materials remains challenging and limits the threshold power of on-chip${\mathrm{\chi <\#comment/>}}^{(2)}$OPO. Here we report an on-chip lithium niobate optical parametric oscillator at the telecom wavelengths using a quasi-phase-matched, high-quality microring resonator, whose threshold power ($\sim <\#comment/>30\text{µ<\#comment/>}\mathrm{W}$) is 400 times lower than that in previous${\mathrm{\chi <\#comment/>}}^{(2)}$integrated photonics platforms. An on-chip power conversion efficiency of 11% is obtained from pump to signal and idler fields at a pump power of 93 µW. The OPO wavelength tuning is achieved by varying the pump frequency and chip temperature. With the lowest power threshold among all on-chip OPOs demonstrated so far, as well as advantages including high conversion efficiency, flexibility in quasi-phase-matching, and device scalability, the thin-film lithium niobate OPO opens new opportunities for chip-based tunable classical and quantum light sources and provides a potential platform for realizing photonic neural networks.