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If an adhesive is meant to be temporary, roughness often poses a challenge for design. An adhesive could be made soft so that it can deform and increase surface contact but a softer material will in general hold a smaller load. Bioinspired adhesives, made with numerous microscale posts, show promise as roughness tolerant adhesives but are complicated to fabricate. In this work, we show how thin polymer sheets, when crumpled into a roughly spherical shape, form a very simple and roughness tolerant adhesive system. We use micro and macro-scale experiments to measure adhesion forces between various substrates and crumpled polydimethylsiloxane sheets. We find the force-displacement curves resemble probe-tack experiments of traditional pressure sensitive adhesives and that moderate tensile forces are required to initiate interfacial failure. Notably, we see that sticky crumples often perform better on long wavelength roughness than they do on smooth substrates. In order to improve the peak pull-off forces, we create a sticky crumple from a thin sheet of a glassy polymer, polycarbonate, coated with an adhesive layer. This elasto-plastic sticky crumple achieves high pull-off forces even on the rough surface of a landscaping brick.
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Ultrahigh strength and shear-assisted separation of sliding nanocontacts studied in situ
Abstract The behavior of materials in sliding contact is challenging to determine since the interface is normally hidden from view. Using a custom microfabricated device, we conduct in situ, ultrahigh vacuum transmission electron microscope measurements of crystalline silver nanocontacts under combined tension and shear, permitting simultaneous observation of contact forces and contact width. While silver classically exhibits substantial sliding-induced plastic junction growth, the nanocontacts exhibit only limited plastic deformation despite high applied stresses. This difference arises from the nanocontacts’ high strength, as we find the von Mises stresses at yield points approach the ideal strength of silver. We attribute this to the nanocontacts’ nearly defect-free nature and small size. The contacts also separate unstably, with pull-off forces well below classical predictions for rupture under pure tension. This strongly indicates that shearing reduces nanoscale pull-off forces, predicted theoretically at the continuum level, but not directly observed before.
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- PAR ID:
- 10377717
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 13
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1038/s41467-022-30290-y
