Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO2, NO, and NOxin the UTLS ASM anticyclone from satellite measurements. Observations of NO2from the Optical Spectrograph and InfraRed Imager System, the Atmospheric Chemistry Experiment ‐ Fourier Transform Spectrometer (ACE‐FTS), and the Stratospheric Aerosol and Gas Experiment III on the International Space Station are considered. The PRATMO photochemical box model is used to quantify the NOxphotochemistry, and to derive the NOxconcentration using OSIRIS NO2and O3observations. The satellite data show a relative minimum in NO2over the ASM in the summer months, while the corresponding NO and NOxanomalies are elevated, mainly due to low O3and cold temperatures within the ASM. The observations within the ASM show reasonable agreement to simulations from the Whole Atmosphere Community Climate Model.
- Award ID(s):
- 1743753
- NSF-PAR ID:
- 10378634
- Date Published:
- Journal Name:
- Atmospheric Measurement Techniques
- Volume:
- 15
- Issue:
- 16
- ISSN:
- 1867-8548
- Page Range / eLocation ID:
- 4767 to 4783
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
more » « less
Abstract -
Abstract. Cirrus clouds that form in the tropical tropopause layer(TTL) can play a key role in vertical transport through the uppertroposphere and lower stratosphere, which can significantly impact theradiative energy budget and stratospheric chemistry. However, the lack ofrealistic representation of natural ice cloud habits in microphysicalparameterizations can lead to uncertainties in cloud-related processes andcloud–climate feedbacks. The main goal of this study is to investigate therole of different cloud regimes and the associated ice habits in regulatingthe properties of the TTL. We compare aircraft measurements from theStratoClim field campaign to a set of numerical experiments at the scale of large-eddy simulations (LESs) for the same case study that employ differentmicrophysics schemes. Aircraft measurements over the southern slopes of theHimalayas captured high ice water content (HIWC) up to 2400 ppmv and iceparticle aggregates exceeding 700 µm in size with unusually longresidence times. The observed ice particles were mainly of liquid origin,with a small amount formed in situ. The corresponding profile of ice water content (IWC) fromthe ERA5 reanalysis corroborates the presence of HIWC detrained from deep-convective plumes in the TTL but underestimates HIWC by an order ofmagnitude. In the TTL, only the scheme that predicts ice habits canreproduce the observed HIWC, ice number concentration, and bimodal iceparticle size distribution. The lower range of particle sizes is mostlyrepresented by planar and columnar habits, while the upper range isdominated by aggregates. Large aggregates with sizes between 600 and 800 µm have fall speeds of less than 20 cm s−1, which explains thelong residence time of the aggregates in the TTL. Planar ice particles ofliquid origin contribute substantially to HIWC. The columnar and aggregatehabits are in the in situ range with lower IWC and number concentrations. Forall habits, the ice number concentration increases with decreasingtemperature. For the planar ice habit, relative humidity is inverselycorrelated with fall speed. This correlation is less evident for the othertwo ice habits. In the lower range of supersaturation with respect to ice,the columnar habit has the highest fall speed. The difference in ice numberconcentration across habits can be up to 4 orders of magnitude, withaggregates occurring in much smaller numbers. We demonstrate and quantifythe linear relationship between the differential sedimentation of pristineice crystals and the size of the aggregates that form when pristine crystalscollide. The slope of this relationship depends on which pristine ice habitsediments faster. Each simulated ice habit is associated with distinctradiative and latent heating rates. This study suggests that a modelconfiguration nested down to LES scales with a microphysicalparameterization that predicts ice shape evolution is crucial to provide anaccurate representation of the microphysical properties of TTL cirrus andthus the associated (de)hydration process.more » « less
-
more » « less
Abstract Tropopause‐overshooting convection transports air from the lower troposphere to the upper troposphere and lower stratosphere (UTLS) where the resulting chemistry and mixing of trace gases can modify the radiation budget. While recent work has examined output from model simulations as well as aircraft and satellite observations of the impacts of tropopause‐overshooting convection on UTLS composition, the range of potential impacts and their dependence on characteristics of storms and their environments is not known. Here, two 10‐day periods, one representative of springtime convection and one representative of summertime convection, were simulated with the Weather Research and Forecasting (WRF) model with Chemistry to examine the range of UTLS composition impacts from tropopause‐overshooting convection. Overall, springtime convection has a larger impact on UTLS composition than summertime convection, with a net effect of increasing water vapor (H2O) in the lower stratosphere and increasing ozone (O3) in the upper troposphere. Springtime convection frequently increases the domain average H2O mixing ratio in the lowermost stratosphere by over 20% while changes in stratospheric H2O from summertime convection are much lower (∼7%–11% increase), reflecting a dependence of the maximum possible H2O increase on UTLS temperature. Increases in upper troposphere O3mixing ratios span the range 8%–19% from springtime convection and are minimal from summertime convection. Changes in the composition of the UTLS from tropopause‐overshooting convection are largely dependent on the height and temperature of the tropopause, with the largest changes being in environments with relatively low tropopause heights between 11 and 13 km (typical of springtime environments in the United States).
-
Abstract. The tropical tropopause layer (TTL; 14–18.5 km) is the gateway formost air entering the stratosphere, and therefore processes within thislayer have an outsized influence in determining global stratospheric ozoneand water vapor concentrations. Despite the importance of this layer thereare few in situ measurements with the necessary detail to resolve the fine-scale processes within this region. Here, we introduce a novel platform forhigh-resolution in situ profiling that lowers and retracts a suspendedinstrument package beneath drifting long-duration balloons in the tropics.During a 100 d circumtropical flight, the instrument collected over a hundred 2 km profiles of temperature, water vapor, and aerosol at 1 m resolution, yielding unprecedented geographic sampling and verticalresolution. The instrument system integrates proven sensors for water vapor,temperature, pressure, and cloud and aerosol particles with an innovativemechanical reeling and control system. A technical evaluation of the systemperformance demonstrated the feasibility of this new measurement platformfor future missions with minor modifications. Six instruments planned fortwo upcoming field campaigns are expected to provide over 4000 profilesthrough the TTL, quadrupling the number of high-resolution aircraft andballoon profiles collected to date. These and future measurements willprovide the necessary resolution to diagnose the importance of competingmechanisms for the transport of water vapor across the TTL.more » « less
-
more » « less
Abstract Radiative cooling of the lowest atmospheric levels is of strong importance for modulating atmospheric circulations and organizing convection, but detailed observations and a robust theoretical understanding are lacking. Here we use unprecedented observational constraints from subsidence regimes in the tropical Atlantic to develop a theory for the shape and magnitude of low‐level longwave radiative cooling in clear‐sky, showing peaks larger than 5–10 K/day at the top of the boundary layer. A suite of novel scaling approximations is first developed from simplified spectral theory, in close agreement with the measurements. The radiative cooling peak height is set by the maximum lapse rate in water vapor path, and its magnitude is mainly controlled by the ratio of column relative humidity above and below the peak. We emphasize how elevated intrusions of moist air can reduce low‐level cooling, by sporadically shading the spectral range which effectively cools to space. The efficiency of this spectral shading depends both on water content and altitude of moist intrusions; its height dependence cannot be explained by the temperature difference between the emitting and absorbing layers, but by the decrease of water vapor extinction with altitude. This analytical work can help to narrow the search for low‐level cloud patterns sensitive to radiative‐convective feedbacks: the most organized patterns with largest cloud fractions occur in atmospheres below 10% relative humidity and feel the strongest low‐level cooling. This motivates further assessment of favorable conditions for radiative‐convective feedbacks and a robust quantification of corresponding shallow cloud dynamics in current and warmer climates.
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.5194/amt-15-4767-2022
