skip to main content


Title: Spectral control of nonclassical light pulses using an integrated thin-film lithium niobate modulator
Abstract

Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.

 
more » « less
Award ID(s):
2137723
NSF-PAR ID:
10380556
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ;
Publisher / Repository:
Nature Publishing Group
Date Published:
Journal Name:
Light: Science & Applications
Volume:
11
Issue:
1
ISSN:
2047-7538
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract

    The scaling of many photonic quantum information processing systems is ultimately limited by the flux of quantum light throughout an integrated photonic circuit. Source brightness and waveguide loss set basic limits on the on-chip photon flux. While substantial progress has been made, separately, towards ultra-low loss chip-scale photonic circuits and high brightness single-photon sources, integration of these technologies has remained elusive. Here, we report the integration of a quantum emitter single-photon source with a wafer-scale, ultra-low loss silicon nitride photonic circuit. We demonstrate triggered and pure single-photon emission into a Si3N4photonic circuit with ≈ 1 dB/m propagation loss at a wavelength of ≈ 930 nm. We also observe resonance fluorescence in the strong drive regime, showing promise towards coherent control of quantum emitters. These results are a step forward towards scaled chip-integrated photonic quantum information systems in which storing, time-demultiplexing or buffering of deterministically generated single-photons is critical.

     
    more » « less
  2. Techniques to control the spectro-temporal properties of quantum states of light at ultrafast time scales are crucial for numerous applications in quantum information science. In this work, we report an all-optical time lens for quantum signals based on Bragg-scattering four-wave mixing with picosecond resolution. Our system achieves a temporal magnification factor of 158 with single-photon level inputs, which is sufficient to overcome the intrinsic timing jitter of superconducting nanowire single-photon detectors. We demonstrate discrimination of two terahertz-bandwidth, single-photon-level pulses with 2.1 ps resolution (electronic jitter corrected resolution of 1.25 ps). We draw on elegant tools from Fourier optics to further show that the time-lens framework can be extended to perform complex unitary spectro-temporal transformations by imparting optimized temporal and spectral phase profiles to the input waveforms. Using numerical optimization techniques, we show that a four-stage transformation can realize an efficient temporal mode sorter that demultiplexes 10 Hermite–Gaussian (HG) modes. Our time-lens-based framework represents a new toolkit for arbitrary spectro-temporal processing of single photons, with applications in temporal mode quantum processing, high-dimensional quantum key distribution, temporal mode matching for quantum networks, and quantum-enhanced sensing with time-frequency entangled states.

     
    more » « less
  3. We propose an on-chip triply resonant electro-optic modulator architecture for RF-to-optical signal conversion and provide a detailed theoretical analysis of the optimal “circuit-level” device geometries and their performance limits. The designs maximize the RF-optical conversion efficiency through simultaneous resonant enhancement of the RF drive signal, a continuous-wave (CW) optical pump, and the generated optical sideband. The optical pump and sideband are resonantly enhanced in respective supermodes of a two-coupled-cavity optical resonator system, while the RF signal can be enhanced in addition by an LC circuit formed by capacitances of the optical resonator active regions and (integrated) matching inductors. We show that such designs can offer 15-50 dB improvement in conversion efficiency over conventional microring modulators. In the proposed configurations, the photon lifetime (resonance linewidth) limits the instantaneous RF bandwidth of the electro-optic response but does not limit its central RF frequency. The latter is set by the coupling strength between the two coupled cavities and is not subject to the photon lifetime constraint inherent to conventional singly resonant microring modulators. This feature enables efficient operation at high RF carrier frequencies without a reduction in efficiency commonly associated with the photon lifetime limit and accounts for 10-30 dB of the total improvement. Two optical configurations of the modulator are proposed: a “basic” configuration with equal Q-factors in both supermodes, most suitable for narrowband RF signals, and a “generalized” configuration with independently tailored supermode Q-factors that supports a wider instantaneous bandwidth. A second significant 5-20 dB gain in modulation efficiency is expected from RF drive signal enhancement by integrated LC resonant matching, leading to the total expected improvement of 15-50 dB. Previously studied triply-resonant modulators, with coupled longitudinal (across the free spectral range (FSR)) modes, have large resonant mode volume for typical RF frequencies, which limits the interaction between the optical and RF fields. In contrast, the proposed modulators support maximally tightly confined resonant modes, with strong coupling between the mode fields, which increases and maintains high device efficiency across a range of RF frequencies. The proposed modulator architecture is compact, efficient, capable of modulation at high RF carrier frequencies and can be applied to any cavity design or modulation mechanism. It is also well suited to moderate Q, including silicon, implementations, and may be enabling for future CMOS RF-electronic-photonic systems on chip.

     
    more » « less
  4. Semiconductor quantum dots embedded in micropillar cavities are excellent emitters of single photons when pumped resonantly. Often, the same spatial mode is used to both resonantly excite a quantum-dot state and to collect the emitted single photons, requiring cross polarization to reduce the uncoupled scattered laser light. This inherently reduces the source brightness to 50%. Critically, for some quantum applications the total efficiency from generation to detection must be over 50%. Here, we demonstrate a resonant-excitation approach to creating single photons that is free of any cross polarization, and in fact any filtering whatsoever. It potentially increases single-photon rates and collection efficiencies, and simplifies operation. This integrated device allows us to resonantly excite single quantum-dot states in several cavities in the plane of the device using connected waveguides, while the cavity-enhanced single-photon fluorescence is directed vertically (off-chip) in a Gaussian mode. We expect this design to be a prototype for larger chip-scale quantum photonics.

     
    more » « less
  5. Time-frequency (TF) filtering of analog signals has played a crucial role in the development of radio-frequency communications and is currently being recognized as an essential capability for communications, both classical and quantum, in the optical frequency domain. How best to design optical time-frequency (TF) filters to pass a targeted temporal mode (TM), and to reject background (noise) photons in the TF detection window? The solution for ‘coherent’ TF filtering is known—the quantum pulse gate—whereas the conventional, more common method is implemented by a sequence of incoherent spectral filtering and temporal gating operations. To compare these two methods, we derive a general formalism for two-stage incoherent time-frequency filtering, finding expressions for signal pulse transmission efficiency, and for the ability to discriminate TMs, which allows the blocking of unwanted background light. We derive the tradeoff between efficiency and TM discrimination ability, and find a remarkably concise relation between these two quantities and the time-bandwidth product of the combined filters. We apply the formalism to two examples—rectangular filters or Gaussian filters—both of which have known orthogonal-function decompositions. The formalism can be applied to any state of light occupying the input temporal mode, e.g., ‘classical’ coherent-state signals or pulsed single-photon states of light. In contrast to the radio-frequency domain, where coherent detection is standard and one can use coherent matched filtering to reject noise, in the optical domain direct detection is optimal in a number of scenarios where the signal flux is extremely small. Our analysis shows how the insertion loss and SNR change when one uses incoherent optical filters to reject background noise, followed by direct detection, e.g. photon counting. We point out implications in classical and quantum optical communications. As an example, we study quantum key distribution, wherein strong rejection of background noise is necessary to maintain a high quality of entanglement, while high signal transmission is needed to ensure a useful key generation rate.

     
    more » « less