skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Aerosol-boundary layer interaction modulated entrainment process
Abstract Aerosol-boundary layer interactions play an important role in affecting atmospheric thermodynamics and air pollution. As a key factor in dictating the development of the boundary layer, the entrainment process in the context of aerosol-boundary layer interactions is still poorly understood. Using comprehensive field observations made at a superstation in Beijing, we gain insight into the response of the entrainment process to aerosols. We found that high aerosol loading can significantly suppress the entrainment rate, breaking the conventional linear relationship between sensible heat fluxes and entrainment fluxes. Related to aerosol vertical distributions, aerosol heating effects can alter vertical heat fluxes, leading to a strong interaction between aerosols and the entrainment process in the upper boundary layer. Such aerosol-entrainment coupling can inhibit boundary layer development and explains the great sensitivity of observed entrainment rates to aerosols than can traditional calculations. The notable impact of aerosols on the entrainment process raises holistic thinking about the dynamic framework of the boundary layer in a polluted atmosphere, which may have a significant bearing on the dispersion of air pollutants and the land-atmosphere coupling.  more » « less
Award ID(s):
2126098
PAR ID:
10381841
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
Nature Publishing Group
Date Published:
Journal Name:
npj Climate and Atmospheric Science
Volume:
5
Issue:
1
ISSN:
2397-3722
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. null (Ed.)
    Abstract. The aerosol–planetary boundary layer (PBL) interaction wasproposed as an important mechanism to stabilize the atmosphere andexacerbate surface air pollution. Despite the tremendous progress made inunderstanding this process, its magnitude and significance still have largeuncertainties and vary largely with aerosol distribution and meteorologicalconditions. In this study, we focus on the role of aerosol verticaldistribution in thermodynamic stability and PBL development by jointly usingmicropulse lidar, sun photometer, and radiosonde measurements taken inBeijing. Despite the complexity of aerosol vertical distributions,cloud-free aerosol structures can be largely classified into three types:well-mixed, decreasing with height, and inverse structures. The aerosol–PBLrelationship and diurnal cycles of the PBL height and PM2.5 associated with these different aerosol vertical structures showdistinct characteristics. The vertical distribution of aerosol radiativeforcing differs drastically among the three types, with strong heating in thelower, middle, and upper PBL, respectively. Such a discrepancy in the heatingrate affects the atmospheric buoyancy and stability differently in the threedistinct aerosol structures. Absorbing aerosols have a weaker effect ofstabilizing the lower atmosphere under the decreasing structure than underthe inverse structure. As a result, the aerosol–PBL interaction can bestrengthened by the inverse aerosol structure and can be potentiallyneutralized by the decreasing structure. Moreover, aerosols can both enhanceand suppress PBL stability, leading to both positive and negativefeedback loops. This study attempts to improve our understanding of theaerosol–PBL interaction, showing the importance of the observationalconstraint of aerosol vertical distribution for simulating this interactionand consequent feedbacks. 
    more » « less
  2. Aerosol-cloud interactions (ACIs) are vital for regulating Earth’s climate by influencing energy and water cycles. Yet, effects of ACI bear large uncertainties, evidenced by systematic discrepancies between observed and modeled estimates. This study quantifies a major bias in ACI determinations, stemming from conventional surface or space measurements that fail to capture aerosol at the cloud level unless the cloud is coupled with land surface. We introduce an advanced approach to determine radiative forcing of ACI by accounting for cloud-surface coupling. By integrating field observations, satellite data, and model simulations, this approach reveals a drastic alteration in aerosol vertical transport and ACI effects caused by cloud coupling. In coupled regimes, aerosols enhance cloud droplet number concentration across the boundary layer more homogeneously than in decoupled conditions, under which aerosols from the free atmosphere predominantly affect cloud properties, leading to marked cooling effects. Our findings spotlight cloud-surface coupling as a key factor for ACI quantification, hinting at potential underassessments in traditional estimates. 
    more » « less
  3. Abstract Top‐down entrainment shapes the vertical gradients of sensible heat, latent heat, and CO2fluxes, influencing the interpretation of eddy covariance (EC) measurements in the unstable atmospheric surface layer (ASL). Using large eddy simulations for convective boundary layer flows, we demonstrate that decreased temperature gradients across the entrainment zone increase entrainment fluxes by enhancing the entrainment velocity, amplifying the asymmetry between top‐down and bottom‐up flux contributions. These changes alter scalar flux profiles, causing flux divergence or convergence and leading to the breakdown of the constant flux layer assumption (CFLA) in the ASL. As a result, EC‐measured fluxes either underestimate or overestimate “true” surface fluxes during divergence or convergence phases, contributing to energy balance non‐closure. The varying degrees of the CFLA breakdown are a fundamental cause for the non‐closure issue. These findings highlight the underappreciated role of entrainment in interpreting EC fluxes, addressing non‐closure, and understanding site‐to‐site variability in flux measurements. 
    more » « less
  4. null (Ed.)
    Abstract. Vertical profiles of aerosols are inadequately observed and poorlyrepresented in climate models, contributing to the current large uncertaintyassociated with aerosol–cloud interactions. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Aerosol and CloudExperiments in the Eastern North Atlantic (ACE-ENA) aircraft field campaignnear the Azores islands provided ample observations of verticaldistributions of aerosol and cloud properties. Here we utilize the in situaircraft measurements from the ACE-ENA and ground-based remote-sensing dataalong with an aerosol-aware Weather Research and Forecast (WRF) model tocharacterize the aerosols due to long-range transport over a remote regionand to assess their possible influence on marine-boundary-layer (MBL)clouds. The vertical profiles of aerosol and cloud properties measured viaaircraft during the ACE-ENA campaign provide detailed information revealingthe physical contact between transported aerosols and MBL clouds. TheEuropean Centre for Medium-Range Weather Forecasts Copernicus Atmosphere Monitoring Service (ECMWF-CAMS) aerosol reanalysis data can reproduce the key features of aerosolvertical profiles in the remote region. The cloud-resolving WRF sensitivityexperiments with distinctive aerosol profiles suggest that the transportedaerosols and MBL cloud interactions (ACIs) require not only aerosol plumes to get close to the marine-boundary-layer top but also large cloud topheight variations. Based on those criteria, the observations show that theoccurrence of ACIs involving the transport of aerosol over the eastern NorthAtlantic (ENA) is about 62 % in summer. For the case with noticeable long-range-transport aerosol effects on MBL clouds, the susceptibilities of dropleteffective radius and liquid water content are −0.11 and +0.14,respectively. When varying by a similar magnitude, aerosols originatingfrom the boundary layer exert larger microphysical influence on MBL cloudsthan those entrained from the free troposphere. 
    more » « less
  5. Abstract Clouds, crucial for understanding climate, begin with droplet formation from aerosols, but observations of this fleeting activation step are lacking in the atmosphere. Here we use a time-gated time-correlated single-photon counting lidar to observe cloud base structures at decimeter scales. Results show that the air–cloud interface is not a perfect boundary but rather a transition zone where the transformation of aerosol particles into cloud droplets occurs. The observed distributions of first-arriving photons within the transition zone reflect vertical development of a cloud, including droplet activation and condensational growth. Further, the highly resolved vertical profile of backscattered photons above the cloud base enables remote estimation of droplet concentration, an elusive but critical property to understanding aerosol–cloud interactions. Our results show the feasibility of remotely monitoring cloud properties at submeter scales, thus providing much-needed insights into the impacts of atmospheric pollution on clouds and aerosol-cloud interactions that influence climate. 
    more » « less