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1. Dynamic optical spectroscopy and pyrometry of static targets under optical and x-ray laser heating at the European XFEL

   https://doi.org/10.1063/5.0142196  

   Ball, O_B; Prescher, C.; Appel, K.; Baehtz, C.; Baron, M_A; Briggs, R.; Cerantola, V.; Chantel, J.; Chariton, S.; Coleman, A_L; et al (August 2023, Journal of Applied Physics)

   Experiments accessing extreme conditions at x-ray free electron lasers (XFELs) involve rapidly evolving conditions of temperature. Here, we report time-resolved, direct measurements of temperature using spectral streaked optical pyrometry of x-ray and optical laser-heated states at the High Energy Density instrument of the European XFEL. This collection of typical experiments, coupled with numerical models, outlines the reliability, precision, and meaning of time dependent temperature measurements using optical emission at XFEL sources. Dynamic temperatures above 1500 K are measured continuously from spectrally- and temporally-resolved thermal emission at 450–850 nm, with time resolution down to 10–100 ns for 1–200 μs streak camera windows, using single shot and integrated modes. Targets include zero-pressure foils free-standing in air and in vacuo, and high-pressure samples compressed in diamond anvil cell multi-layer targets. Radiation sources used are 20-fs hard x-ray laser pulses at 17.8 keV, in single pulses or 2.26 MHz pulse trains of up to 30 pulses, and 250-ns infrared laser single pulses. A range of further possibilities for optical measurements of visible light in x-ray laser experiments using streak optical spectroscopy are also explored, including for the study of x-ray induced optical fluorescence, which often appears as background in thermal radiation measurements. We establish several scenarios where combined emissions from multiple sources are observed and discuss their interpretation. Challenges posed by using x-ray lasers as non-invasive probes of the sample state are addressed. 

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2. X-ray constraints on dark photon tridents

   https://doi.org/10.1103/37gn-x3y1  

   Linden, Tim; Nguyen, Thong_T Q; Tait, Tim_M P (July 2025, Physical Review D)

   Dark photons that are sufficiently light and/or weakly interacting represent a compelling vision of dark matter. Dark photon decay into three photons, which we call the dark photon trident, can be the dominant channel when the dark photon mass falls below the electron pair threshold and can produce a significant flux of x rays. We use 16 years of data from Interrnational Gamma-Ray Astro Physics Laboratory (INTEGRAL)/Spectrometer of INTEGRAL (SPI) to constrain sub-MeV dark photon decay, producing new worlds-best constraints on the kinetic mixing parameter for dark photon masses between 90 and 1022 keV, and comment on the potential for future x-ray observatories to discover the trident decay process. 

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3. Resonant X-ray excitation of the nuclear clock isomer 45Sc

   https://doi.org/10.1038/s41586-023-06491-w  

   Shvyd’ko, Yuri; Röhlsberger, Ralf; Kocharovskaya, Olga; Evers, Jörg; Geloni, Gianluca Aldo; Liu, Peifan; Shu, Deming; Miceli, Antonino; Stone, Brandon; Hippler, Willi; et al (October 2023, Nature)

   Abstract Resonant oscillators with stable frequencies and large quality factors help us to keep track of time with high precision. Examples range from quartz crystal oscillators in wristwatches to atomic oscillators in atomic clocks, which are, at present, our most precise time measurement devices¹. The search for more stable and convenient reference oscillators is continuing^2–6. Nuclear oscillators are better than atomic oscillators because of their naturally higher quality factors and higher resilience against external perturbations^7–9. One of the most promising cases is an ultra-narrow nuclear resonance transition in⁴⁵Sc between the ground state and the 12.4-keV isomeric state with a long lifetime of 0.47 s (ref. ¹⁰). The scientific potential of⁴⁵Sc was realized long ago, but applications require⁴⁵Sc resonant excitation, which in turn requires accelerator-driven, high-brightness X-ray sources¹¹that have become available only recently. Here we report on resonant X-ray excitation of the⁴⁵Sc isomeric state by irradiation of Sc-metal foil with 12.4-keV photon pulses from a state-of-the-art X-ray free-electron laser and subsequent detection of nuclear decay products. Simultaneously, the transition energy was determined as$${\mathrm{12,389.59}}_{+0.12\left({\rm{syst}}\right)}^{\pm 0.15\left({\rm{stat}}\right)}\,{\rm{eV}}$$ ${\mathrm{12,389.59}}_{+0.12\left(\mathrm{syst}\right)}^{\pm 0.15\left(\mathrm{stat}\right)}\mathrm{eV}$with an uncertainty that is two orders of magnitude smaller than the previously known values. These advancements enable the application of this isomer in extreme metrology, nuclear clock technology, ultra-high-precision spectroscopy and similar applications. 

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4. Diffraction data from aerosolized Coliphage PR772 virus particles imaged with the Linac Coherent Light Source

   https://doi.org/10.1038/s41597-020-00745-2  

   Li, Haoyuan; Nazari, Reza; Abbey, Brian; Alvarez, Roberto; Aquila, Andrew; Ayyer, Kartik; Barty, Anton; Berntsen, Peter; Bielecki, Johan; Pietrini, Alberto; et al (December 2020, Scientific Data)

   Abstract Single Particle Imaging (SPI) with intense coherent X-ray pulses from X-ray free-electron lasers (XFELs) has the potential to produce molecular structures without the need for crystallization or freezing. Here we present a dataset of 285,944 diffraction patterns from aerosolized Coliphage PR772 virus particles injected into the femtosecond X-ray pulses of the Linac Coherent Light Source (LCLS). Additional exposures with background information are also deposited. The diffraction data were collected at the Atomic, Molecular and Optical Science Instrument (AMO) of the LCLS in 4 experimental beam times during a period of four years. The photon energy was either 1.2 or 1.7 keV and the pulse energy was between 2 and 4 mJ in a focal spot of about 1.3μm x 1.7μm full width at half maximum (FWHM). The X-ray laser pulses captured the particles in random orientations. The data offer insight into aerosolised virus particles in the gas phase, contain information relevant to improving experimental parameters, and provide a basis for developing algorithms for image analysis and reconstruction. 

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5. Femtosecond temperature measurements of laser-shocked copper deduced from the intensity of the x-ray thermal diffuse scattering

   https://doi.org/10.1063/5.0256844  

   Wark, J_S; Peake, D_J; Stevens, T.; Heighway, P_G; Ping, Y.; Sterne, P.; Albertazzi, B.; Ali, S_J; Antonelli, L.; Armstrong, M_R; et al (April 2025, Journal of Applied Physics)

   We present 50-fs, single-shot measurements of the x-ray thermal diffuse scattering (TDS) from copper foils that have been shocked via nanosecond laser ablation up to pressures above ∼135 GPa. We hence deduce the x-ray Debye–Waller factor, providing a temperature measurement. The targets were laser-shocked with the DiPOLE 100-X laser at the High Energy Density endstation of the European X-ray Free-Electron Laser. Single x-ray pulses, with a photon energy of 18 keV, were scattered from the samples and recorded on Varex detectors. Despite the targets being highly textured (as evinced by large variations in the elastic scattering) and with such texture changing upon compression, the absolute intensity of the azimuthally averaged inelastic TDS between the Bragg peaks is largely insensitive to these changes, and allowing for both Compton scattering and the low-level scattering from a sacrificial ablator layer provides a reliable measurement of T/ΘD2, where ΘD is the Debye temperature. We compare our results with the predictions of the SESAME 3336 and LEOS 290 equations of state for copper and find good agreement within experimental errors. We, thus, demonstrate that single-shot temperature measurements of dynamically compressed materials can be made via thermal diffuse scattering of XFEL radiation. 

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