skip to main content


Title: Enhanced stimulated Raman scattering during intense laser propagation

Stimulated Raman scattering is ubiquitous in many high-intensity laser environments. Parametric four-wave mixing between the pump and Raman sidebands can affect the Raman gain, but stringent phase matching requirements and strongly nonlinear dynamics obscure clear understanding of its effects at high laser powers. Here we investigate four-wave mixing in the presence of strong self-focusing and weak ionization at laser powers above the Kerr critical power. Theoretical analysis shows that the plasma generated at focus naturally leads to phase matching conditions suitable for enhanced Raman gain, almost without regard to the initial phase mismatch. Multidimensional nonlinear optical simulations with multiphoton and collisional ionization confirm the enhancement and suggest that it may lead to significantly higher Raman losses in some high-intensity laser environments.

 
more » « less
Award ID(s):
1903414
NSF-PAR ID:
10384743
Author(s) / Creator(s):
; ; ; ; ; ;
Publisher / Repository:
Optical Society of America
Date Published:
Journal Name:
Optics Express
Volume:
30
Issue:
26
ISSN:
1094-4087; OPEXFF
Page Range / eLocation ID:
Article No. 46944
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Strong amplification in integrated photonics is one of the most desired optical functionalities for computing, communications, sensing, and quantum information processing. Semiconductor gain and cubic nonlinearities, such as four-wave mixing and stimulated Raman and Brillouin scattering, have been among the most studied amplification mechanisms on chip. Alternatively, material platforms with strong quadratic nonlinearities promise numerous advantages with respect to gain and bandwidth, among which nanophotonic lithium niobate is one of the most promising candidates. Here, we combine quasi-phase matching with dispersion engineering in nanophotonic lithium niobate waveguides and achieve intense optical parametric amplification. We measure a broadband phase-sensitive on-chip amplification larger than 50 dB/cm in a 6-mm-long waveguide. We further confirm high gain operation in the degenerate and nondegenerate regimes by amplifying vacuum fluctuations to macroscopic levels, with on-chip gains exceeding 100 dB/cm over 600 nm of bandwidth around 2 µm. Our results unlock new possibilities for on-chip few-cycle nonlinear optics, mid-infrared photonics, and quantum photonics.

     
    more » « less
  2. Josephson Traveling Wave Parametric Amplifiers (J-TWPAs) are promising platforms for realizing broadband quantum-limited amplification of microwave signals. However, substantial gain in such systems is attainable only when strict constraints on phase matching of the signal, idler and pump waves are satisfied -- this is rendered particularly challenging in the presence of nonlinear effects, such as self- and cross-phase modulation, which scale with the intensity of propagating signals. In this work, we present a simple J-TWPA design based on left-handed (negative-index) nonlinear Josephson metamaterial, which realizes autonomous phase matching without the need for any complicated circuit or dispersion engineering. The resultant efficiency of four-wave mixing process can implement gains in excess of 20 dB over few GHz bandwidths with much shorter lines than previous implementations. Furthermore, the autonomous nature of phase matching considerably simplifies the J-TWPA design than previous implementations based on right-handed (positive index) Josephson metamaterials, making the proposed architecture particularly appealing from a fabrication perspective. The left-handed JTL introduced here constitutes a new modality in distributed Josephson circuits, and forms a crucial piece of the unified framework that can be used to inform the optimal design and operation of broadband microwave amplifiers. 
    more » « less
  3. Recently, our groups have introduced the notion of optical parametric amplification based on non-Hermitian phase matching wherein the incorporation of loss can lead to gain in this nonlinear optical process. Previous simulation results using second-order nonlinear optical coupled-mode theory have demonstrated the potential of this technique as an alternative to the stringent phase-matching condition, which is often difficult to achieve in semiconductor platforms. Here we fortify this notion for the case of third-order nonlinearity by considering parametric amplification in silicon nanowires and illustrate the feasibility of these devices by employing rigorous finite-difference time-domain analysis using realistic materials and geometric parameters. Particularly, we demonstrate that by systematic control of the optical loss of the idler in a four-wave mixing process, we can achieve efficient unidirectional energy conversion from the pump to the signal component even when the typical phase-matching condition is violated. Importantly, our simulations show that a signal gain of∼<#comment/>9dBfor a waveguide length of a few millimeters is possible over a large bandwidth of several hundreds of nanometers (∼<#comment/>600nm). This bandwidth is nearly 2 orders of magnitude larger than what can be achieved in the conventional silicon-photonics-based four-wave mixing process.

     
    more » « less
  4. Four-wave mixing (FWM) of optical fields has been extensively used in quantum information processing, sensing, and memories. It also forms a basis for nonlinear spectroscopies such as transient grating, stimulated Raman, and photon echo where phase matching is used to select desired components of the third-order response of matter. Here we report an experimental study of the two-dimensional quantum noise intensity difference spectra of a pair of squeezed beams generated by FWM in hot Rb vapor. The measurement reveals details of the χ ( 3 ) susceptibility dressed by the strong pump field which induces an AC Stark shift, with higher spectral resolution compared to classical measurements of probe and conjugate beam intensities. We demonstrate how quantum correlations of squeezed light can be utilized as a spectroscopic tool which unlike their classical counterparts are robust to external noise. 
    more » « less
  5. Abstract Diamond has attracted great interest as an appealing material for various applications ranging from classical to quantum optics. To date, Raman lasers, single photon sources, quantum sensing and quantum communication have been demonstrated with integrated diamond devices. However, studies of the nonlinear optical properties of diamond have been limited, especially at the nanoscale. Here, a metasurface consisting of plasmonic nanogap cavities is used to enhance both χ (2) and χ (3) nonlinear optical processes in a wedge-shaped diamond slab with a thickness down to 12 nm. Multiple nonlinear processes were enhanced simultaneously due to the relaxation of phase-matching conditions in subwavelength plasmonic structures by matching two excitation wavelengths with the fundamental and second-order modes of the nanogap cavities. Specifically, third-harmonic generation (THG) and second-harmonic generation (SHG) are both enhanced 1.6 × 10 7 -fold, while four-wave mixing is enhanced 3.0 × 10 5 -fold compared to diamond without the metasurface. Even though diamond lacks a bulk χ (2) due to centrosymmetry, the observed SHG arises from the surface χ (2) of the diamond slab and is enhanced by the metasurface elements. The efficient, deeply subwavelength diamond frequency converter demonstrated in this work suggests an approach for conversion of color center emission to telecom wavelengths directly in diamond. 
    more » « less