Color centers in solids, such as the nitrogen-vacancy center in diamond, offer well-protected and well-controlled localized electron spins that can be employed in various quantum technologies. Moreover, the long coherence time of the surrounding spinful nuclei can enable a robust quantum register controlled through the color center. We design pulse sequence protocols that drive the electron spin to generate robust entangling gates with these nuclear memory qubits. We find that compared to using Carr-Purcell-Meiboom-Gill (CPMG) alone, Uhrig decoupling sequence and hybrid protocols composed of CPMG and Uhrig sequences improve these entangling gates in terms of fidelity, spin control range, and spin selectivity. We provide analytical expressions for the sequence protocols and also show numerically the efficacy of our method on nitrogen-vacancy centers in diamond. Our results are broadly applicable to color centers weakly coupled to a small number of nuclear spin qubits.
Electron spins in solid-state systems offer the promise of spin-based information processing devices. Single-walled carbon nanotubes (SWCNTs), an all-carbon one-dimensional material whose spin-free environment and weak spin-orbit coupling promise long spin coherence times, offer a diverse degree of freedom for extended range of functionality not available to bulk systems. A key requirement limiting spin qubit implementation in SWCNTs is disciplined confinement of isolated spins. Here, we report the creation of highly confined electron spins in SWCNTs via a bottom-up approach. The record long coherence time of 8.2 µs and spin-lattice relaxation time of 13 ms of these electronic spin qubits allow demonstration of quantum control operation manifested as Rabi oscillation. Investigation of the decoherence mechanism reveals an intrinsic coherence time of tens of milliseconds. These findings evident that combining molecular approaches with inorganic crystalline systems provides a powerful route for reproducible and scalable quantum materials suitable for qubit applications.
more » « less- NSF-PAR ID:
- 10398181
- Publisher / Repository:
- Nature Publishing Group
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 14
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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Color centers in solids, such as the nitrogen-vacancy center in diamond, offer well-protected and well-controlled localized electron spins that can be employed in various quantum technologies. Moreover, the long coherence time of the surrounding spinful nuclei can enable a robust quantum register controlled through the color center.We design pulse sequence protocols that drive the electron spin to generate robust entangling gates with these nuclear memory qubits.We find that compared to using Carr-Purcell-Meiboom-Gill (CPMG) alone, Uhrig decoupling sequence and hybrid protocols composed of CPMG and Uhrig sequences improve these entangling gates in terms of fidelity, spin control range, and spin selectivity. We provide analytical expressions for the sequence protocols and also show numerically the efficacy of our method on nitrogen-vacancy centers in diamond. Our results are broadly applicable to color centers weakly coupled to a small number of nuclear spin qubits.more » « less
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