Aerosol indirect effects are one of the leading contributors to cloud radiative properties relevant to climate. Aerosol particles become cloud droplets when the ambient relative humidity (saturation ratio) exceeds a critical value, which depends on the particle size and chemical composition. In the traditional formulation of this problem, only average, uniform saturation ratios are considered. Using experiments and theory, we examine the effects of fluctuations, produced by turbulence. Our measurements, from a multiphase, turbulent cloud chamber, show a clear transition from a regime in which the mean saturation ratio dominates to one in which the fluctuations determine cloud properties. The laboratory measurements demonstrate cloud formation in mean-subsaturated conditions (i.e., relative humidity <100%) in the fluctuation-dominant activation regime. The theoretical framework developed to interpret these measurements predicts a transition from a mean- to a fluctuation-dominated regime, based on the relative values of the mean and standard deviation of the environmental saturation ratio and the critical saturation ratio at which aerosol particles activate or become droplets. The theory is similar to the concept of stochastic condensation and can be used in the context of the atmosphere to explore the conditions under which droplet activation is driven by fluctuations as opposed to mean supersaturation. It provides a basis for future development of cloud droplet activation parameterizations that go beyond the internally homogeneous parcel calculations that have been used in the past.
- Award ID(s):
- 1754244
- PAR ID:
- 10401921
- Date Published:
- Journal Name:
- Journal of the Atmospheric Sciences
- Volume:
- 79
- Issue:
- 12
- ISSN:
- 0022-4928
- Page Range / eLocation ID:
- 3145 to 3162
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
more » « less
-
A minimalist model of microphysical properties in cloudy Rayleigh-Bénard convection is developed based on mass and number balances for cloud droplets growing by vapor condensation. The model is relevant to a turbulent mixed-layer in which a steady forcing of supersaturation can be defined, e.g., a model of the cloudy boundary layer or a convection-cloud chamber. The model assumes steady injection of aerosol particles that are activated to form cloud droplets, and the removal of cloud droplets through sedimentation. Simplifying assumptions include the consideration of mean properties in steady state, neglect of coalescence growth, and no detailed representation of the droplet size distribution. Closed-form expressions for cloud droplet radius, number concentration, and liquid water content are derived. Limits of fast and slow microphysics, compared to the turbulent mixing time scale, are explored, and resulting expressions for the scaling of microphysical properties in fast and slow regimes are obtained. Scaling of microphysics with layer thickness is also explored, suggesting that liquid water content and cloud droplet number concentration increase, and mean droplet radius decreases with increasing layer thickness. Finally, the analytical model is shown to compare favorably to solutions of the fully-coupled set of governing ordinary differential equations that describe the system, and the predicted power law for liquid water mixing ratio versus droplet activation rate is observed to be consistent with measurements from the Pi convection-cloud chamber.more » « less
-
more » « less
Abstract Turbulent fluctuations of scalar and velocity fields are critical for cloud microphysical processes, e.g., droplet activation and size distribution evolution, and can therefore influence cloud radiative forcing and precipitation formation. Lagrangian and Eulerian water vapor, temperature, and supersaturation statistics are investigated in direct numerical simulations (DNS) of turbulent Rayleigh–Bénard convection in the Pi Convection Cloud Chamber to provide a foundation for parameterizing subgrid-scale fluctuations in atmospheric models. A subgrid model for water vapor and temperature variances and covariance and supersaturation variance is proposed, valid for both clear and cloudy conditions. Evaluation of phase change contributions through an a priori test using DNS data shows good performance of the model. Supersaturation is a nonlinear function of temperature and water vapor, and relative external fluxes of water vapor and heat (e.g., during entrainment-mixing and phase change) influence turbulent supersaturation fluctuations. Although supersaturation has autocorrelation and structure functions similar to the independent scalars (temperature and water vapor), the autocorrelation time scale of supersaturation differs. Relative scalar fluxes in DNS without cloud make supersaturation PDFs less skewed than the adiabatic case, where they are highly negatively skewed. However, droplet condensation changes the PDF shape response: it becomes positively skewed for the adiabatic case and negatively skewed when the sidewall relative fluxes are large. Condensation also increases correlations between water vapor and temperature in the presence of relative scalar fluxes but decreases correlations for the adiabatic case. These changes in correlation suppress supersaturation variability for the nonadiabatic cases and increase it for the adiabatic case. Implications of this work for subgrid microphysics modeling using a Lagrangian stochastic scheme are also discussed.
-
more » « less
Abstract Water vapor supersaturation in clouds is a random variable that drives activation and growth of cloud droplets. The Pi Convection–Cloud Chamber generates a turbulent cloud with a microphysical steady state that can be varied from clean to polluted by adjusting the aerosol injection rate. The supersaturation distribution and its moments, e.g., mean and variance, are investigated for varying cloud microphysical conditions. High-speed and collocated Eulerian measurements of temperature and water vapor concentration are combined to obtain the temporally resolved supersaturation distribution. This allows quantification of the contributions of variances and covariances between water vapor and temperature. Results are consistent with expectations for a convection chamber, with strong correlation between water vapor and temperature; departures from ideal behavior can be explained as resulting from dry regions on the warm boundary, analogous to entrainment. The saturation ratio distribution is measured under conditions that show monotonic increase of liquid water content and decrease of mean droplet diameter with increasing aerosol injection rate. The change in liquid water content is proportional to the change in water vapor concentration between no-cloud and cloudy conditions. Variability in the supersaturation remains even after cloud droplets are formed, and no significant buffering is observed. Results are interpreted in terms of a cloud microphysical Damköhler number (Da), under conditions corresponding to
, i.e., the slow-microphysics regime. This implies that clouds with very clean regions, such that is satisfied, will experience supersaturation fluctuations without them being buffered by cloud droplet growth. Significance Statement The saturation ratio (humidity) in clouds controls the growth rate and formation of cloud droplets. When air in a turbulent cloud mixes, the humidity varies in space and time throughout the cloud. This is important because it means cloud droplets experience different growth histories, thereby resulting in broader size distributions. It is often assumed that growth and evaporation of cloud droplets buffers out some of the humidity variations. Measuring these variations has been difficult, especially in the field. The purpose of this study is to measure the saturation ratio distribution in clouds with a range of conditions. We measure the in-cloud saturation ratio using a convection cloud chamber with clean to polluted cloud properties. We found in clouds with low concentrations of droplets that the variations in the saturation ratio are not suppressed.
-
more » « less
Abstract Numerical simulations of turbulent moist Rayleigh–Bénard convection driving CCN activation and droplet growth in the laboratory Pi chamber are discussed. Supersaturation fluctuations come from isobaric mixing of warm and humid air rising from the lower boundary with colder air featuring lower water vapor concentrations descending from the upper boundary. Lagrangian particle–based microphysics is used to represent the growth of haze CCN and cloud droplets with kinetic, solute, and surface tension effects included. Dry CCN spectra in the range between 2- and 200-nm radii from field observations are considered. Increasing the total CCN concentration from pristine to polluted conditions results in an increase in the droplet concentration and reduction in the mean droplet radius and spectral width. These are in agreement with Pi chamber observations and numerical simulations, as well as with numerous past studies of CCN cloud-base activation in natural clouds. The key result is that a relatively small fraction of the available CCN is activated in the Pi chamber fluctuating supersaturations, from about a half in the pristine case to only a 10th in the polluted case. The activation fraction as a function of the dry CCN radius is similar in all simulations, close to zero at the CCN small end, increasing to a maximum at CCN radius around 50 nm, and decreasing to close to zero at the large CCN end. This is explained as too small supersaturations to activate small CCN as in natural clouds and insufficient time to allow large CCN reaching the critical radius.
Significance Statement Impact of turbulence on the formation and growth of cloud droplets is an important cloud physics problem. Laboratory experiments in the Michigan Technological University cloud chamber provide key insights into this problem. Numerical simulations of cloud chamber processes discussed in this paper complement laboratory experiments by providing insights difficult or impossible to obtain in the laboratory. The study contrasts the formation and growth of cloud droplets in the laboratory cloud chamber with processes taking place in natural clouds. The differences documented in this paper pose questions concerning the impact of turbulence on the formation and growth of cloud droplets as a result of interactions of clouds with their environment.
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1175/JAS-D-22-0051.1
