Abstract The profiles of marine boundary layer (MBL) cloud and drizzle microphysical properties are important for studying the cloud‐to‐rain conversion and growth processes in MBL clouds. However, it is challenging to simultaneously retrieve both cloud and drizzle microphysical properties within an MBL cloud layer using ground‐based observations. In this study, methods were developed to first decompose drizzle and cloud reflectivity in MBL clouds from Atmospheric Radiation Measurement cloud radar reflectivity measurements and then simultaneously retrieve cloud and drizzle microphysical properties during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE‐ENA) campaign. These retrieved microphysical properties, such as cloud and drizzle particle size (rcandrm,d), their number concentration (NcandNd) and liquid water content (LWCcandLWCd), have been validated by aircraft in situ measurements during ACE‐ENA (~158 hr of aircraft data). The mean surface retrieved (in situ measured)rc,Nc, andLWCcare 10.9 μm (11.8 μm), 70 cm−3(60 cm−3), and 0.21 g m−3(0.22 g m−3), respectively. For drizzle microphysical properties, the retrieved (in situ measured)rd,Nd, andLWCdare 44.9 μm (45.1 μm), 0.07 cm−3(0.08 cm−3), and 0.052 g m−3(0.066 g m−3), respectively. Treating the aircraft in situ measurements as truth, the estimated median retrieval errors are ~15% forrc, ~35% forNc, ~30% forLWCcandrd, and ~50% forNdandLWCd. The findings from this study will provide insightful information for improving our understanding of warm rain processes, as well as for improving model simulations. More studies are required over other climatic regions. 
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                            Cumulus Cloud and Drizzle Microphysics Relationships With Complete CCN Spectra
                        
                    
    
            Abstract Comparisons of high‐resolution extended range CCN spectra measured at 100 m altitude with cloud and drizzle microphysics in the Rain in Cumulus over the Ocean (RICO) aircraft field project are presented. CCN concentrations,NCCN, active at supersaturations,S, >0.1% showed positive relationships with cloud droplet concentrations,Nc, measured at intermediate (606–976 m) and very high altitudes (1,763–3,699 m). These correlation coefficients,R, progressively increased withSwhile the two‐tailed probabilities, P2, progressively decreased with S to < 10−6at 1.6%S. More important were the positive relationships betweenNCCNactive atS < 0.1% and drizzle drop concentrations,Nd, at high (977–1,662 m), very high and high‐very high altitudes combined (977–3,699 m). All of these relationships were consistent for eight different cloud liquid water content,Lc, thresholds (forNc) andLcbins (forNd) ranging from 0.0002 to 0.3 g/m3. Negative relationships between CCN modality and low altitude (76–475 m) cloudiness coupled with no relationship ofNCCNactive at any S withNcof these low clouds indicated a cloud effect on ambient aerosol. This is a demonstration of clouds causing bimodal aerosol. 
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                            - Award ID(s):
- 1940645
- PAR ID:
- 10446473
- Publisher / Repository:
- DOI PREFIX: 10.1029
- Date Published:
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Volume:
- 126
- Issue:
- 15
- ISSN:
- 2169-897X
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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