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Abstract Cloud droplet number concentration (Nd) is a key microphysical property that is largely controlled by the balance between sources and sinks of aerosols that serve as cloud condensation nuclei (CCN). Despite being a key sink of CCN, the impact of coalescence scavenging on Southern Ocean (SO) cloud is poorly known. We apply a simple source‐and‐sink budget model based on parameterizations to austral summer aircraft observations to test model behavior and examine the relative influence of processes that determineNdin SO stratocumulus clouds. The model predictsNdwith little bias and a correlation coefficient of ∼0.7 compared with observations. Coalescence scavenging is found to be an important sink of CCN in both liquid and mixed‐phase precipitating stratocumulus and reduces the predictedNdby as much as 90% depending on the precipitation rate. The free tropospheric aerosol source controlsNdmore strongly than the surface aerosol source during austral summer.
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Influences of Recent Particle Formation on Southern Ocean Aerosol Variability and Low Cloud Properties
Abstract Controls on pristine aerosol over the Southern Ocean (SO) are critical for constraining the strength of global aerosol indirect forcing. Observations of summertime SO clouds and aerosols in synoptically varied conditions during the 2018 SOCRATES aircraft campaign reveal novel mechanisms influencing pristine aerosol‐cloud interactions. The SO free troposphere (3–6 km) is characterized by widespread, frequent new particle formation events contributing to much larger concentrations (≥1,000 mg−1) of condensation nuclei (diameters > 0.01 μm) than in typical sub‐tropical regions. Synoptic‐scale uplift in warm conveyor belts and sub‐polar vortices lifts marine biogenic sulfur‐containing gases to free‐tropospheric environments favorable for generating Aitken‐mode aerosol particles (0.01–0.1 μm). Free‐tropospheric Aitken particles subside into the boundary layer, where they grow in size to dominate the sulfur‐based cloud condensation nuclei (CCN) driving SO cloud droplet number concentrations (Nd ∼ 60–100 cm−3). Evidence is presented for a hypothesized Aitken‐buffering mechanism which maintains persistently high summertime SONdagainst precipitation removal through CCN replenishment from activation and growth of boundary layer Aitken particles. Nudged hindcasts from the Community Atmosphere Model (CAM6) are found to underpredict Aitken and accumulation mode aerosols andNd, impacting summertime cloud brightness and aerosol‐cloud interactions and indicating incomplete representations of aerosol mechanisms associated with ocean biology.
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- PAR ID:
- 10362541
- Publisher / Repository:
- DOI PREFIX: 10.1029
- Date Published:
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Volume:
- 126
- Issue:
- 8
- ISSN:
- 2169-897X
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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