Indoor dust can be a major source of heavy metals, nutrients, and bacterial contamination in residential environments and may cause serious health problems. The goal of this research is to characterize chemical and bacterial contaminants of indoor, settled house dust in the Houston Metropolitan region. To achieve this, a total of 31 indoor dust samples were collected, along with household survey data, which were subsequently analyzed for elemental and bacterial concentrations. Microscopic and geospatial analysis was conducted to characterize and map potential hotspots of contamination. Interestingly Cd, Cr, Cu, Pb, and Zn concentrations of all 31 indoor dust samples were significantly enriched and exceeded soil background concentrations. Furthermore, As, Cd, Pb, and Zn concentrations in the dust samples were significantly correlated to the enteric bacterial load concentrations. Human health assessment revealed that cancer risk values via ingestion for Cd, Cr, and Ni were greater than the acceptable range. Of our 31 dust sample isolates, three Gram-negative and 16 Gram-positive pathogenic bacteria were identified, capable of causing a wide range of diseases. Our results demonstrate that both chemical and bacterial characterization of indoor dust coupled with spatial mapping is essential to assess and monitor human and ecological health risks.
more »
« less
Automated corona discharge (CD) for efficient and broad-spectrum surface and air sterilization
In the past three years, the COVID-19 pandemic has caused serious health, environmental, societal, and economic challenges globally. Sterilization is one of the most efficient methods to mitigate the spread of infectious viruses like SARS-CoV-2. However, extreme sterilization practices can cause serious health and environmental problems worldwide. Heat, ultraviolet C (UVC), and chemical disinfectants require high energy consumption and can cause health concerns, environmental pollution, and chemical overuse. In this paper, we evaluated the efficiency of corona discharge (CD) as an environmentally and energy-friendly sterilization method on different surfaces for sterilization. It was confirmed that CD is an efficient sterilization process for most surfaces and personal protective equipment (PPE). CD allows for a reduction in disinfectant use, addresses the PPE shortage problem, and reduces plastic pollution and biowaste. The air sterilization effect of CD creates a promising option to reduce airborne pathogens. To address the safety concerns of CD, the heat, UVC, and ozone emissions of CD were confirmed to be within a safe range. A wireless, affordable CD robot was developed with the capability to scan along pre-designed paths while having the capability to avoid static and moving obstacles. Automated CD devices and robots can be favorable sterilization solutions for the future as a contactless, more environmentally friendly, efficient, affordable, and portable solution.
more »
« less
- Award ID(s):
- 2114216
- PAR ID:
- 10450314
- Date Published:
- Journal Name:
- Journal of Materials Chemistry C
- ISSN:
- 2050-7526
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Nonthermal atmospheric pressure plasmas transform input electrical energy efficiently into reactive species, charged particles, and photons. This “activated gas” is being investigated as solutions for a range of environmental and health problems facing society today. In this Perspective, we take a cursory look at a few of these societal problems and the reflected role that plasmas may play in charting the pathway to a solution buoyed by supporting research. Here, we survey the plasma-based opportunities in the removal of trace contaminants in water supporting methodologies such as water reuse, which addresses scarcity and pollution, the opportunity posed by plasmas-based chemical depolymerization for plastics recycling, and the application of plasmas for food security, which includes sterilization of foodstuffs and the improvement of crop yield. Finally, we also included a short review on how plasmas may help control disease spread. In each case, the scope of the problem is presented along with the potential plasma-based solution.more » « less
-
null (Ed.)The lithium-sulfur (Li-S) redox battery system is considered to be the most promising next-generation energy storage technology due to its high theoretical specific capacity (1673 mAh g−1), high energy density (2600 Wh kg−1), low cost, and the environmentally friendly nature of sulfur. Though this system is deemed to be the next-generation energy storage device for portable electronics and electric vehicles, its poor cycle life, low coulombic efficiency and low rate capability limit it from practical applications. These performance barriers were linked to several issues like polysulfide (LiPS) shuttle, inherent low conductivity of charge/discharge end products, and poor redox kinetics. Here, we review the recent developments made to alleviate these problems through an electrocatalysis approach, which is considered to be an effective strategy not only to trap the LiPS but also to accelerate their conversion reactions kinetics. Herein, the influence of different chemical interactions between the LiPS and the catalyst surfaces and their effect on the conversion of liquid LiPS to solid end products are reviewed. Finally, we also discussed the challenges and perspectives for designing cathode architectures to enable high sulfur loading along with the capability to rapidly convert the LiPS.more » « less
-
more » « less
Abstract With the ongoing need for water conservation, the American Southwest has worked to increase harvested rainwater efforts to meet municipal needs. Concomitantly, environmental pollution is prevalent, leading to concerns regarding the quality of harvested rainwater.
Project Harvest , a co-created community science project, was initiated with communities that neighbor sources of pollution. To better understand how a participant’s socio-demographic factors affect home characteristics and rainwater harvesting infrastructure, pinpoint gardening practices, and determine participant perception of environmental pollution, a 145-question “Home Description Survey” was administered toProject Harvest participants (n = 167) by projectpromotoras (community health workers). Race/ethnicity and community were significantly associated (p < 0.05) with participant responses regarding proximity to potential sources of pollution, roof material, water harvesting device material, harvesting device capacity, harvesting device age, garden amendments, supplemental irrigation, and previous contaminant testing. Further, the study has illuminated the idiosyncratic differences in how underserved communities perceive environmental pollution and historical past land uses in their community. We propose that the collection of such data will inform the field on how to tailor environmental monitoring efforts and results for constituent use, how community members may alter activities to reduce environmental hazard exposure, and how future studies can be designed to meet the needs of environmentally disadvantaged communities. -
more » « less
Abstract The accumulation of plastic waste, due to lack of recycling, has led to serious environmental pollution. Although mechanical recycling can alleviate this issue, it inevitably reduces the molecular weight and weakens the mechanical properties of materials and is not suitable for mixed materials. Chemical recycling, on the other hand, breaks the polymer into monomers or small‐molecule constituents, allowing for the preparation of materials of quality comparable to that of the virgin polymers and can be applied to mixed materials. Mechanochemical degradation and recycling leverages the advantages of mechanical techniques, such as scalability and efficient energy use, to achieve chemical recycling. We summarize recent progress in mechanochemical degradation and recycling of synthetic polymers, including both commercial polymers and those designed for more efficient mechanochemical degradation. We also point out the limitations of mechanochemical degradation and present our perspectives on how the challenges can be mitigated for a circular polymer economy.
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1039/d3tc00558e
