Abstract Surface properties are critical to the capabilities of superconducting microwave devices. The native oxide of niobium-based devices is thought to consist of a thin normal conducting layer. To improve understanding on the importance of this layer, an attempt was made to replace it with a more easily controlled gold film. A niobium sample host microwave cavity was used to measure the surface resistance in continuous wave operation at and . Sample conditions studied include temperatures ranging from to with RF magnetic fields on the sample surface ranging from to the maximum field before the superconducting properties were lost (quench field). The nominal film thickness of the gold layer was increased from to in five steps to study the impact of the normal layer thickness on surface resistance on a single niobium substrate. The film was found to reduce the surface resistance of the sample and to enhance the quench field. With the exception of the final step from a gold film to , the magnitude of the surface resistance increased substantially with gold film thickness. The nature of the surface resistance field-dependence appeared to be roughly independent from the gold layer thickness. This initial study provides new perspectives and suggests avenues for optimizing and designing surfaces for resonant cavities in particle accelerators and quantum information applications.
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Hardware, methodology and applications of 2 + D backscatter Mössbauer spectroscopy with simultaneous x-ray and γ-ray detection
Abstract A unique method is presented for the acquisition and analysis of57Fe backscatter Mössbauer spectra with simultaneous detection of the resonant 14.4 keVγ-rays and the characteristic 6.4 keV x-rays, using a custom-built multi-parameter analyser constructed on the basis of commercial analogue to digital converters and high-speed digital latches. The system allows for the simultaneous registration of Doppler-modulation velocities and photon energies, with up to 4096 and 8192 digital channels respectively. This arrangement is in contrast to most related systems, which detect at a single narrow energy window per detector. Samples of arbitrary atomic structure, morphology and surface topography can be studied without altering the setup or the analysis procedure, provided that the samples are at least micrometre sized. The hardware and software that are used to acquire data with minimal dead time are described and the custom and self-contained methods for post-measurement energy discrimination, background correction and velocity-axis folding are discussed. The data are fit using a general Hamiltonian model for the nuclear energy levels of57Fe and a quantum mechanical description of the angular momentum coupling is utilised, with consideration of the crystalline and chemical disorder of the sample under examination. Three examples of distinct magnetic systems, with thicknesses ranging from m to 6 mm, that were studied using this method are presented, these are: an amorphous CoFeB-based ribbon with ultra-soft coercivity for high-frequency applications, magnetically hard Nd-Fe-B thick films on Si substrates, examined in both as-deposited and annealed states, and a sample from the nickel-rich iron meteorite NWA 6259 that contains the atomically ordered, elevated coercivity, phase of FeNi, tetrataenite. The wide applicability and usefulness of this method is thus demonstrated on three distinct sample morphologies that required little to no surface preparation prior to examination.
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- Award ID(s):
- 2118164
- PAR ID:
- 10473266
- Publisher / Repository:
- IOP Publishing
- Date Published:
- Journal Name:
- Measurement Science and Technology
- Volume:
- 35
- Issue:
- 2
- ISSN:
- 0957-0233
- Format(s):
- Medium: X Size: Article No. 025503
- Size(s):
- Article No. 025503
- Sponsoring Org:
- National Science Foundation
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