skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Topologically distinct atomic insulators
Topological classification of quantum solids often (if not always) groups all trivial atomic or normal insulators (NIs) into the same featureless family. As we argue here, this is not necessarily the case always. In particular, when the global phase diagram of electronic crystals harbors topological insulators with the band inversion at various time-reversal invariant momenta KTIinv in the Brillouin zone, their proximal NIs display noninverted band-gap minima at KNImin=KTIinv. In such systems, once topological superconductors nucleate from NIs, the inversion of the Bogoliubov de Gennes bands takes place at KBdGinv=KNImin, inheriting from the parent state. We showcase this (possibly general) proposal for two-dimensional time-reversal symmetry-breaking insulators. Then, distinct quantized thermal Hall conductivity and responses to dislocation lattice defects inside the paired states (tied with KBdGinv or KNImin), in turn, unambiguously identify different parent atomic NIs.  more » « less
Award ID(s):
2238679
PAR ID:
10482445
Author(s) / Creator(s):
; ;
Publisher / Repository:
American Physical Society
Date Published:
Journal Name:
Physical Review B
Volume:
108
Issue:
4
ISSN:
2469-9950
Page Range / eLocation ID:
L041301
Subject(s) / Keyword(s):
Defects, Thermal Hall effect, Transport phenomena, Topological materials, Topological superconductors, Tight-binding model
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Topological lattice defects, such as dislocations and grain boundaries (GBs), are ubiquitously present in the bulk of quantum materials and externally tunable in metamaterials. In terms of robust modes, localized near the defect cores, they are instrumental in identifying topological crystals, featuring the hallmark band inversion at a finite momentum (translationally active type). Here we show that the GB superlattices in both two-dimensional and three-dimensional translationally active higher-order topological insulators harbor a myriad of dispersive modes that are typically placed at finite energies, but always well-separated from the bulk states. However, when the Burgers vector of the constituting edge dislocations points toward the gapless corners or hinges, both second-order and third-order topological insulators accommodate self-organized emergent topological metals near the zero energy (half-filling) in the GB mini Brillouin zone. We discuss possible material platforms where our proposed scenarios can be realized through the band-structure and defect engineering. 
    more » « less
  2. We highlight recent advances in the theory, materials fabrication, and experimental characterization of strongly correlated and topological states in [111] oriented transition metal oxide thin films and heterostructures, which are notoriously difficult to realize compared to their [001] oriented counterparts. We focus on two classes of complex oxides, with the chemical formulas ABO3 and A2B2O7, where the B sites are occupied by an open-shell transition metal ion with a local moment and the A sites are typically a rare earth element. The [111] oriented quasi-two-dimensional lattices derived from these parent compound lattices can exhibit peculiar geometries and symmetries, namely, a buckled honeycomb lattice, as well as kagome and triangular lattices. These lattice motifs form the basis for emergent strongly correlated and topological states expressed in exotic magnetism, various forms of orbital ordering, topological insulators, topological semimetals, quantum anomalous Hall insulators, and quantum spin liquids. For transition metal ions with high atomic number, spin–orbit coupling plays a significant role and may give rise to additional topological features in the electronic band structure and in the spectrum of magnetic excitations. We conclude this perspective by articulating open challenges and opportunities in this actively developing field. 
    more » « less
  3. The studies of topological insulators (TI) and topological semimetals have been at frontiers of condensed matter physics and material science. Both classes of materials are characterized by robust surface states created by the topology of the bulk band structures and exhibit exotic transport properties. When magnetism is present in topological materials and breaks the time-reversal symmetry, more exotic quantum phenomena can be generated, e.g., quantum anomalous Hall effect (QAHE), axion insulator, and large intrinsic AHE. In this research update, we briefly summarize the recent research progress in magnetic topological materials, including intrinsic magnetic TI and magnetic Weyl semimetals. 
    more » « less
  4. Breaking the time-reversal symmetry on the surface of a topological insulator can open a gap for the linear dispersion and make the Dirac fermions massive. This can be achieved by either doping a topological insulator with magnetic elements or proximity-coupling it to magnetic insulators. While the exchange gap can be directly imaged in the former case, measuring it at the buried magnetic insulator/topological insulator interface remains to be challenging. Here, we report the observation of a large nonlinear Hall effect in iron garnet/Bi2Se3 heterostructures. Besides illuminating its magnetic origin, we also show that this nonlinear Hall effect can be utilized to measure the size of the exchange gap and the magnetic-proximity onset temperature. Our results demonstrate the nonlinear Hall effect as a spectroscopic tool to probe the modified band structure at magnetic insulator/topological insulator interfaces. 
    more » « less
  5. Topological band theory has achieved great success in the high-throughput search for topological band structures both in paramagnetic and magnetic crystal materials. However, a significant proportion of materials are topologically trivial insulators at the Fermi level. In this paper, we show that, remarkably, for a subset of the topologically trivial insulators, knowing only their electron number and the Wyckoff positions of the atoms we can separate them into two groups: the obstructed atomic insulator (OAI) and the atomic insulator (AI). The interesting group, the OAI, have a center of charge not localized on the atoms. Using the theory of topological quantum chemistry, in this work we first derive the necessary and sufficient conditions for a topologically trivial insulator to be a filling enforced obstructed atomic insulator (feOAI) in the 1651 Shubnikov space groups. Remarkably, the filling enforced criteria enable the identification of obstructed atomic bands without knowing the representations of the band structures. Hence, no calculations are needed for the filling enforced criteria, although they are needed to obtain the band gaps. With the help of the Topological Quantum Chemistry website, we have performed a high-throughput search for feOAIs and have found that 957 ICSD entries (638 unique materials) are paramagnetic feOAIs, among which 738 (475) materials have an indirect gap. The metallic obstructed surface states of feOAIs are also showcased by several material examples. Published by the American Physical Society2024 
    more » « less