The impacts of Stratospheric Aerosol Injection (SAI) on the atmosphere and surface climate depend on when and where the sulfate aerosol precursors are injected, as well as on how much surface cooling is to be achieved. We use a set of CESM2(WACCM6) SAI simulations achieving three different levels of global mean surface cooling and demonstrate that unlike some direct surface climate impacts driven by the reflection of solar radiation by sulfate aerosols, the SAI‐induced changes in the high latitude circulation and ozone are more complex and could be non‐linear. This manifests in our simulations by disproportionally larger Antarctic springtime ozone loss, significantly larger intra‐ensemble spread of the Arctic stratospheric jet and ozone responses, and non‐linear impacts on the extratropical modes of surface climate variability under the strongest‐cooling SAI scenario compared to the weakest one. These potential non‐linearities may add to uncertainties in projections of regional surface impacts under SAI.
Abstract. Despite offsetting global mean surface temperature, various studies demonstrated that stratospheric aerosol injection (SAI) could influence the recovery of stratospheric ozone and have important impacts on stratospheric and tropospheric circulation, thereby potentially playing an important role in modulating regional and seasonal climate variability. However, so far, most of the assessments of such an approach have come from climate model simulations in which SO2 is injected only in a single location or a set of locations. Here we use CESM2-WACCM6 SAI simulations under a comprehensive set of SAI strategies achieving the same global mean surface temperature with different locations and/or timing of injections, namely an equatorial injection, an annual injection of equal amounts of SO2 at 15∘ N and 15∘ S, an annual injection of equal amounts of SO2 at 30∘ N and 30∘ S, and a polar strategy injecting SO2 at 60∘ N and 60∘ S only in spring in each hemisphere. We demonstrate that despite achieving the same global mean surface temperature, the different strategies result in contrastingly different magnitudes of the aerosol-induced lower stratospheric warming, stratospheric moistening, strengthening of stratospheric polar jets in both hemispheres, and changes in the speed of the residual circulation. These impacts tend to maximise under the equatorial injection strategy and become smaller as the aerosols are injected away from the Equator into the subtropics and higher latitudes. In conjunction with the differences in direct radiative impacts at the surface, these different stratospheric changes drive different impacts on the extratropical modes of variability (Northern and Southern Annular modes), including important consequences on the northern winter surface climate, and on the intensity of tropical tropospheric Walker and Hadley circulations, which drive tropical precipitation patterns. Finally, we demonstrate that the choice of injection strategy also plays a first-order role in the future evolution of stratospheric ozone under SAI throughout the globe. Overall, our results contribute to an increased understanding of the fine interplay of various radiative, dynamical, and chemical processes driving the atmospheric circulation and ozone response to SAI and lay the foundation for designing an optimal SAI strategy that could form a basis of future multi-model intercomparisons.
more » « less- Award ID(s):
- 2038246
- NSF-PAR ID:
- 10484143
- Publisher / Repository:
- EGU
- Date Published:
- Journal Name:
- Atmospheric Chemistry and Physics
- Volume:
- 23
- Issue:
- 21
- ISSN:
- 1680-7324
- Page Range / eLocation ID:
- 13665 to 13684
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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null (Ed.)Abstract. A new set of stratospheric aerosol geoengineering (SAG) model experiments has been performed with Community Earth System Model version 2 (CESM2) with the Whole Atmosphere Community Climate Model (WACCM6) that are based on the Coupled Model Intercomparison Project phase 6 (CMIP6) overshoot scenario (SSP5-34-OS) as a baseline scenario to limit global warming to 1.5 or 2.0 ∘C above 1850–1900 conditions. The overshoot scenario allows us to applying a peak-shaving scenario that reduces the needed duration and amount of SAG application compared to a high forcing scenario. In addition, a feedback algorithm identifies the needed amount of sulfur dioxide injections in the stratosphere at four pre-defined latitudes, 30∘ N, 15∘ N, 15∘ S, and 30∘ S, to reach three surface temperature targets: global mean temperature, and interhemispheric and pole-to-Equator temperature gradients. These targets further help to reduce side effects, including overcooling in the tropics, warming of high latitudes, and large shifts in precipitation patterns. These experiments are therefore relevant for investigating the impacts on society and ecosystems. Comparisons to SAG simulations based on a high emission pathway baseline scenario (SSP5-85) are also performed to investigate the dependency of impacts using different injection amounts to offset surface warming by SAG. We find that changes from present-day conditions around 2020 in some variables depend strongly on the defined temperature target (1.5 ∘C vs. 2.0 ∘C). These include surface air temperature and related impacts, the Atlantic Meridional Overturning Circulation, which impacts ocean net primary productivity, and changes in ice sheet surface mass balance, which impacts sea level rise. Others, including global precipitation changes and the recovery of the Antarctic ozone hole, depend strongly on the amount of SAG application. Furthermore, land net primary productivity as well as ocean acidification depend mostly on the global atmospheric CO2 concentration and therefore the baseline scenario. Multi-model comparisons of experiments that include strong mitigation and carbon dioxide removal with some SAG application are proposed to assess the robustness of impacts on societies and ecosystems.more » « less
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Abstract The specifics of the simulated injection choices in the case of stratospheric aerosol injections (SAI) are part of the crucial context necessary for meaningfully discussing the impacts that a deployment of SAI would have on the planet. One of the main choices is the desired amount of cooling that the injections are aiming to achieve. Previous SAI simulations have usually either simulated a fixed amount of injection, resulting in a fixed amount of warming being offset, or have specified one target temperature, so that the amount of cooling is only dependent on the underlying trajectory of greenhouse gases. Here, we use three sets of SAI simulations achieving different amounts of global mean surface cooling while following a middle‐of‐the‐road greenhouse gas emission trajectory: one SAI scenario maintains temperatures at 1.5°C above preindustrial levels (PI), and two other scenarios which achieve additional cooling to 1.0°C and 0.5°C above PI. We demonstrate that various surface impacts scale proportionally with respect to the amount of cooling, such as global mean precipitation changes, changes to the Atlantic Meridional Overturning Circulation and to the Walker Cell. We also highlight the importance of the choice of the baseline period when comparing the SAI responses to one another and to the greenhouse gas emission pathway. This analysis leads to policy‐relevant discussions around the concept of a reference period altogether, and to what constitutes a relevant, or significant, change produced by SAI.
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Abstract. Solar climate intervention using stratospheric aerosol injection (SAI) has been proposed as a method which could offset some of the adverse effects of global warming. The Assessing Responses and Impacts of Solar climate intervention on the Earth system with Stratospheric Aerosol Injection (ARISE-SAI) set of simulations is based on a moderate-greenhouse-gas-emission scenario and employs injection of sulfur dioxide at four off-equatorial locations using a control algorithm which maintains the global-mean surface temperature at 1.5 K above pre-industrial conditions (ARISE-SAI-1.5), as well as the latitudinal gradient and inter-hemispheric difference in surface temperature. This is the first comparison between two models (CESM2 and UKESM1) applying the same multi-target SAI strategy. CESM2 is successful in reaching its temperature targets, but UKESM1 has considerable residual Arctic warming. This occurs because the pattern of temperature change in a climate with SAI is determined by both the structure of the climate forcing (mainly greenhouse gases and stratospheric aerosols) and the climate models' feedbacks, the latter of which favour a strong Arctic amplification of warming in UKESM1. Therefore, research constraining the level of future Arctic warming would also inform any hypothetical SAI deployment strategy which aims to maintain the inter-hemispheric and Equator-to-pole near-surface temperature differences. Furthermore, despite broad agreement in the precipitation response in the extratropics, precipitation changes over tropical land show important inter-model differences, even under greenhouse gas forcing only. In general, this ensemble comparison is the first step in comparing policy-relevant scenarios of SAI and will help in the design of an experimental protocol which both reduces some known negative side effects of SAI and is simple enough to encourage more climate models to participate.
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Abstract By injecting SO
2 into the stratosphere at four latitudes (30°, 15°N/S), it might be possible not only to reduce global mean surface temperature but also to minimize changes in the equator‐to‐pole and inter‐hemispheric gradients of temperature, further reducing some of the impacts arising from climate change relative to equatorial injection. This can happen only if the aerosols are transported to higher latitudes by the stratospheric circulation, ensuring that a greater part of the solar radiation is reflected back to space at higher latitudes, compensating for the reduced sunlight. However, the stratospheric heating produced by these aerosols modifies the circulation and strengthens the stratospheric polar vortex which acts as a barrier to the transport of air toward the poles. We show how the heating results in a feedback where increasing injection rates lead to stronger high‐latitudinal transport barriers. This implies a potential limitation in the high‐latitude aerosol burden and subsequent cooling.
- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.5194/acp-23-13665-2023
