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Title: Accurate equation of state of H2−He binary mixtures up to 5.4 GPa
Brillouin scattering spectroscopy has been used to obtain an accurate (<1%) ρ-P equation of state (EOS) of 1:1 and 9:1 H2-He molar mixtures from 0.5 to 5.4 GPa at 296 K. Our calculated equations of state indicate close agreement with the experimental data right to the freezing pressure of hydrogen at 5.4 GPa. The measured velocities agree on average, within 0.5%, of an ideal mixing model. The ρ-P EOSs presented have a standard deviation of under 0.3% from the measured densities and under 1% deviation from ideal mixing. A detailed discussion of the accuracy, precision, and sources of error in the measurement and analyses of our equations of state is presented.  more » « less
Award ID(s):
2104881
NSF-PAR ID:
10488406
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ;
Corporate Creator(s):
Editor(s):
-
Publisher / Repository:
DOE pages
Date Published:
Journal Name:
Physical Review B
Edition / Version:
1
Volume:
108
Issue:
22
ISSN:
2469-9950
Page Range / eLocation ID:
224112
Subject(s) / Keyword(s):
Hydrogen helium equation of state Brillouin scattering high pressure
Format(s):
Medium: X Size: 4.1 MB Other: pdf
Size(s):
4.1 MB
Sponsoring Org:
National Science Foundation
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"Accurate equation of state of H2−He binary mixtures up to 5.4 GPa". <em>Physical Review B</em> 108 (22). Country unknown/Code not available: DOE pages. <a href="https://doi.org/10.1103/PhysRevB.108.224112">https://doi.org/10.1103/PhysRevB.108.224112.</a> <a href="https://par.nsf.gov/biblio/10488406">https://par.nsf.gov/biblio/10488406</a>. </div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="links-format"><a href="#cite-bib" data-toggle="modal">BibTeX</a> <div id="cite-bib" class="modal" tabindex="-1" role="dialog" aria-labelledby="cite-bib_label" aria-hidden="true"> <div class="modal-dialog"> <div class="modal-content"> <div class="modal-header"> <button type="button" class="close" data-dismiss="modal" aria-hidden="true">×</button> <strong id="cite-bib_label">Cite: BibTeX Format</strong> </div> <div class="modal-body"> @article{osti_10488406,<br/> place = {Country unknown/Code not available}, title = {Accurate equation of state of H2−He binary mixtures up to 5.4 GPa}, url = {https://par.nsf.gov/biblio/10488406}, DOI = {10.1103/PhysRevB.108.224112}, abstractNote = {Brillouin scattering spectroscopy has been used to obtain an accurate (<1%) ρ-P equation of state (EOS) of 1:1 and 9:1 H2-He molar mixtures from 0.5 to 5.4 GPa at 296 K. Our calculated equations of state indicate close agreement with the experimental data right to the freezing pressure of hydrogen at 5.4 GPa. The measured velocities agree on average, within 0.5%, of an ideal mixing model. The ρ-P EOSs presented have a standard deviation of under 0.3% from the measured densities and under 1% deviation from ideal mixing. A detailed discussion of the accuracy, precision, and sources of error in the measurement and analyses of our equations of state is presented.}, journal = {Physical Review B}, volume = {108}, number = {22}, publisher = {DOE pages}, author = {Zoller, Charlie M. and Ahart, Muhtar and Duwal, Sakun and Clay, Raymond C. and Seagle, Christopher T. and Ryu, Young Jay and Tkachev, Sergey and Chariton, Stella and Prakapenka, Vitali and Hemley, Russell J.}, editor = {-} }</div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="divider"></li> </ul> <ul class="nav nav-list" style="font-size: 14px; font-family: Arial Regular;"> <li class="nav-header header-format">Export Metadata</li> <li class="links-format"><a href="https://par.nsf.gov/endnote?osti_id=10488406">EndNote</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:excel/osti-id:10488406">Excel</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:csv/osti-id:10488406">CSV</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:xml/osti-id:10488406">XML</a></li> <li class="divider"></li> </ul> <ul class="nav nav-list" style="font-size: 14px; 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