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1. Patterns of bubble bursting and weak explosive activity in an active lava lake: Halema‘uma‘u, Kīlauea in 2015

   https://doi.org/https://doi.org/10.3133/pp1867E  

   Mintz, B G ; Houghton, B F ; Llewellin, E ; Orr, T R ; Taddeucci, J ; Carey, R J ; Kueppers, U ; Gaudin, D ; Patrick, M R ; Burton, M ; et al ( January 2021 , US Geological Survey professional paper)

   null (Ed.)

   The rise of the Halemaʻumaʻu lava lake in 2013–2018 to depths commonly 40 meters or less below the rim of the vent was an excellent opportunity to study outgassing and the link to associated eruptive activity. We use videography to investigate the rise and bursting of bubbles through the free surface of the lake in 2015. We focus on low-energy explosive activity (spattering) in which the ascent and bursting of meter-sized, mechanically decoupled bubbles trigger the ejection of fluidal bombs to tens of meters above the free surface. A decay in initial pyroclast velocity with time follows the same functional form as that observed for ejecta at Stromboli (Italy), suggesting a similar bubble-burst mechanism. We also find that the upward velocity of the bubble crust as it bursts is around 2.5 times higher than the velocity of the bubble as it rises through the lake surface, indicating that the bubbles are over-pressurized. Prior to bursting, bubbles emerge at velocities of 4 to 14 meters per second, suggesting rise from depths of at least tens of meters but unaffected by the deeper circulation of the lava lake. We identify three styles of bubble bursting: (1) isolated, widely spaced, single bursts, (2) recurring clusters of discrete bubbles, and (3) prolonged episodes of overlapping bubble bursts along elongate narrow sources typically parallel to the margins of the lava lake. We call these styles of bursting isolated events, clusters, and prolonged episodes, respectively. The frequency of bubble bursting and the mass fluxes of gas and pyroclasts increase from styles 1 to 3. The intensity (mass eruption rate) for single bubble bursts ranges from 280 to 3,500 kilograms per second. The total erupted mass of pyroclasts for a single burst is <4,000 kilograms (kg) and for a single well-constrained prolonged episode is about 107 kg. These numbers place the observed spattering at the lowest end of basaltic explosivity in terms of erupted mass (that is, magnitude). Most ejecta fell back into the crater; only strands of Pele’s hair rose to heights where they could be advected downwind from the vent. 

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2. Melting of glacier ice enhanced by bursting air bubbles

   https://doi.org/10.1038/s41561-023-01262-8  

   Wengrove, Meagan E. ; Pettit, Erin C. ; Nash, Jonathan D. ; Jackson, Rebecca H. ; Skyllingstad, Eric D. ( September 2023 , Nature Geoscience)

   Feedbacks between ice melt, glacier flow and ocean circulation can rapidly accelerate ice loss at tidewater glaciers and alter projections of sea-level rise. At the core of these projections is a model for ice melt that neglects the fact that glacier ice contains pressurized bubbles of air due to its formation from compressed snow. Current model estimates can underpredict glacier melt at termini outside the region influenced by the subglacial discharge plume by a factor of 10–100 compared with observations. Here we use laboratory-scale experiments and theoretical arguments to show that the bursting of pressurized bubbles from glacier ice could be a source of this discrepancy. These bubbles eject air into the seawater, delivering additional buoyancy and impulses of turbulent kinetic energy to the boundary layer, accelerating ice melt. We show that real glacier ice melts 2.25 times faster than clear bubble-free ice when driven by natural convection in a laboratory setting. We extend these results to the geophysical scale to show how bubble dynamics contribute to ice melt from tidewater glaciers. Consequently, these results could increase the accuracy of modelled predictions of ice loss to better constrain sea-level rise projections globally.

    

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3. Effects of Salinity Beyond Coalescence on Submicron Aerosol Distributions

   https://doi.org/10.1029/2022JD038222  

   Dubitsky, L. ; Stokes, M. D. ; Deane, G. B. ; Bird, J. C. ( May 2023 , Journal of Geophysical Research: Atmospheres)

   Bubbles entrained by ocean waves rise to the surface and burst, creating a shower of droplets which contribute to sea spray aerosols. Submicron‐sized droplets, of which an estimated 60%–80% come from a bursting bubble film cap, play a key role in global climate atmospheric processes. However, many aspects of predicting the number and size of submicron drops emitted from a bursting bubble remain unknown. It is well‐documented that higher salinity increases submicron droplet production, which has been attributed to the role of salt in the suppression of bubble coalescence. We experimentally show that submicron drop production increases with salinity despite using a salt that does not affect bubble coalescence, indicating that salinity plays a role in the physics of submicron aerosol formation beyond coalescence. Laboratory experiments are conducted using sodium acetate solutions of salinityS = 0.001–0.1 M with millimeter‐sized bubbles generated via a needle. Unlike previous studies, the measured droplet size distributions are converted to formation diameter, revealing that the peak aerosol formation diameter decreases with higher salinity. Applying this diameter conversion to past studies, we find the peak formation diameter exhibits a scaling ofD_form ∼ S^−0.32across three orders of magnitude in salinity and for a variety of salts, bubble coalescence behaviors, and bubble generation mechanisms. This result suggests that salinity has a systematic effect on the length scale of the rupturing bubble film which generates the aerosols. Consequently, salinity likely impacts the submicron aerosol production in oceanic environments even if bubble coalescence is negligible.

    

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4. Enrichment of saccharides at the air–water interface: a quantitative comparison of sea surface microlayer and foam

   https://doi.org/10.1071/EN22094  

   Jayarathne, Thilina ; Gamage, Dilini Kirindigoda ; Prather, Kimberly A. ; Stone, Elizabeth A. ( January 2023 , Environmental Chemistry)

   Croot, Peter (Ed.)

   Environmental context Saccharides contribute substantially to dissolved organic carbon in the ocean and are enriched at the ocean surface. In this study, we demonstrate that saccharides are more enriched in persistent whitecap foam compared to the sea surface. The maturation of bubbles at the air–water interface is thus expected to enhance the enrichment of organic matter at the ocean surface and ultimately in the sea spray aerosol that forms when bubbles burst at the ocean surface. Rationale Organic matter accumulates at the ocean surface. Herein, we provide the first quantitative assessment of the enrichment of dissolved saccharides in persistent whitecap foam and compare this enrichment to the sea surface microlayer (SSML) during a 9 day mesocosm experiment involving a phytoplankton bloom generated in a Marine Aerosol Reference Tank (MART). Methodology Free monosaccharides were quantified directly, total saccharides were determined following mild acid hydrolysis and the oligo/polysaccharide component was determined as the difference between total and free monosaccharides. Results Total saccharides contributed a significant fraction of dissolved organic carbon (DOC), accounting for 13% of DOC in seawater, 27% in SSML and 31% in foam. Median enrichment factors (EFs), calculated as the ratio of the concentrations of saccharides relative to sodium in SSML or foam to that of seawater, ranged from 1.7 to 6.4 in SSML and 2.1–12.1 in foam. Based on median EFs, xylitol, mannitol, glucose, galactose, mannose, xylose, fucose, rhamnose and ribose were more enriched in foam than SSML. Discussion The greatest EFs for saccharides coincided with high chlorophyll levels, indicating increasing ocean surface enrichment of saccharides during phytoplankton blooms. Higher enrichments of organic matter in sea foam over the SSML indicate that surface active organic compounds become increasingly enriched on persistent bubble film surfaces. These findings help to explain how marine organic matter becomes highly enriched in sea spray aerosol that is generated by bursting bubbles at the ocean surface. 

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5. Ocean emission of microplastic

   https://doi.org/10.1093/pnasnexus/pgad296  

   Shaw, Daniel B ; Li, Qi ; Nunes, Janine K ; Deike, Luc ( September 2023 , PNAS Nexus)

   Zhang, Jiahua (Ed.)

   Microplastics are globally ubiquitous in marine environments, and their concentration is expected to continue rising at significant rates as a result of human activity. They present a major ecological problem with well-documented environmental harm. Sea spray from bubble bursting can transport salt and biological material from the ocean into the atmosphere, and there is a need to quantify the amount of microplastic that can be emitted from the ocean by this mechanism. We present a mechanistic study of bursting bubbles transporting microplastics. We demonstrate and quantify that jet drops are efficient at emitting microplastics up to 280μm in diameter and are thus expected to dominate the emitted mass of microplastic. The results are integrated to provide a global microplastic emission model which depends on bubble scavenging and bursting physics; local wind and sea state; and oceanic microplastic concentration. We test multiple possible microplastic concentration maps to find annual emissions ranging from 0.02 to 7.4—with a best guess of 0.1—mega metric tons per year and demonstrate that while we significantly reduce the uncertainty associated with the bursting physics, the limited knowledge and measurements on the mass concentration and size distribution of microplastic at the ocean surface leaves large uncertainties on the amount of microplastic ejected.

    

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