Structural integrity and quality of short fiber composite parts produced by Big Area Additive Manufacturing (BAAM) are largely affected by inherent bead microstructural features such as voids. Unfortunately, our understanding of void nucleation and evolution during polymer deposition process is lacking. Flow modeling focused on the associated microstructural formation provides a means for better understanding the process-structure-properties relations in large area extrusion deposition additive manufacturing of fiber reinforced composites. Our prior computational effort that investigated mechanisms that may promote micro-void formation was based on 2-dimensional planar models of a single ellipsoidal fiber motion in purely viscous polymer extrusion/deposition flow through a BAAM nozzle. Here we present a 3D finite element modelling approach to simulate single fiber out-of-plane rotations utilizing velocity and velocity gradient values computed along streamlines obtained from a 3D extrusion/deposition simulation of the BAAM polymer deposition process. The pressure distribution on the fiber’s surface along the flow path provides new insight into potential micro-void nucleation mechanism. Results show low pressure regions occur near the fiber’s surface which varies across the printed bead and through its thickness.
more »
« less
Simulation of fiber-induced melt pressure fluctuations within large scale polymer composite deposition beads
The process-structure-property relationship in Large Area Additive Manufacturing (LAAM) technology is an ongoing area of research as the inherent microstructural properties (chiefly fibers and voids) affect the performance of printed parts. Unfortunately, we currently lack adequate understanding of micro void nucleation and evolution during the LAAM and fused deposition modelling (FDM) processes. Modeling of the polymer melt flow during the extrusion process is important in understanding the underlying microstructural formation and associated properties of the print, that determines the part performance in service conditions. In this paper we compute fiber-induced local pressure fluctuations which may promote void formation in the bead’s microstructure. On a macro-scale, we determine flow fields of a purely viscous, Newtonian planar polymer deposition flow through a LAAM nozzle which are utilized on a micro-scale model where we simulate the evolution of a single ellipsoidal fiber along streamlines obtained from the macro-model. On the micro-scale, we determine instantaneous values of the translational and rotational velocities of the rigid ellipsoidal fiber that satisfies a balance of hydrodynamic forces and couples on the fiber’s surface based on a Newton Raphson algorithm and we track the fiber’s motion along the flow path via an explicit numerical iterative algorithm. Model verification is achieved by benchmarking results with solutions from well-known Jeffery’s equation of motion of a particle in homogeneous simple shear flow. We account for rotary diffusivity due to short-range fiber-fiber interaction in the FEA simulation by determining an effective fluid domain size representative of the interaction coefficient of the melt flow through a correlation analysis that yields an equivalent steady state orientation based on the Advani- Tucker equation. We also consider different possible motions of the fiber along individual LAAM flow paths from a given set of random initial fiber conditions to determine pressure bounds on the fiber surface along each streamline. For improved computational efficiency, calculations are carried out with respect to the fiber’s local coordinate axes to overcome the rigor of adaptive remeshing during the quasi-transient analysis. Results show low pressure extremes near the fiber’s surface which varies across the printed bead as well as through its thickness. Discussion is provided to gain insight into the effect of low-pressure extremes on micro void formation, particularly at the nozzle exit and during die swell/expansion.
more »
« less
- Award ID(s):
- 2055628
- PAR ID:
- 10507218
- Publisher / Repository:
- Elsevier
- Date Published:
- Journal Name:
- Additive Manufacturing
- Volume:
- 80
- Issue:
- C
- ISSN:
- 2214-8604
- Page Range / eLocation ID:
- 103980
- Subject(s) / Keyword(s):
- Large area additive manufacturing (LAAM) Microstructures Porosity Computational Modelling Finite element analysis (FEA)
- Format(s):
- Medium: X Size: 14.812MB
- Size(s):
- 14.812MB
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
The formation and development of micro-voids within the bead microstructure of a polymer composite during the extrusion/deposition additive manufacturing process continues to be of interest given the adverse effect these features have on part quality. A computational method is employed here to investigate potential volatile-induced micro-void nucleation mechanism which simulates the evolution of a single rigid ellipsoidal fiber in purely viscous polymer extrusion/deposition flow through a Large Area Additive Manufacturing (LAAM) nozzle. Our previous studies on potential micro-void nucleation mechanisms have assumed a Newtonian fluid property definition for the polymer melt flow, the current study assesses the effect of assuming a generalized Newtonian fluid (GNF) model on the fiber’s response. Preliminary findings based on Jeffery’s flow assumption reveal the fiber’s orientation kinetics are unaffected by the shear thinning fluid behavior, however there is a reduction in the pressure distribution on the fiber’s surface as the power law index is decreased which is expected to reduce the likelihood for microvoid nucleation.more » « less
-
Micro-voids within the bead microstructure of additively manufactured short carbon fiber- reinforced polymer composites are known to compromise the material performance. Unfortunately, a comprehensive understanding of the formation mechanisms of micro-voids during polymer processing is currently lacking. The present study considers micro-void nucleation at fiber inter-faces, particularly those occurring at the end of suspended fibers. Micro-computed tomography (μCT) image acquisition techniques are used to characterize microstructural features of a 13wt% carbon fiber reinforced ABS compo-site bead manufactured via Large Area Additive Manufacturing (LAAM). The results reveal a significant collection of micro-voids at the tips of fibers approaching 80% of the total micro-void volume fraction. In addition, fiber tip micro-voids are relatively larger and less spherical than micro-voids isolated within the ABS matrix. Theoretical formulations of several known mechanisms for micro-void nucleation during LAAM material processing indicate that local-ized fluid pressure likely plays a pivotal role in micro-void formation. To better expose this mechanism, we simulate the hydrostatic flow-field pressure distri-bution surrounding a single rigid fiber suspended in simple shear flow using fi-nite element analysis (FEA). Computed results demonstrate that the polymer matrix pressure decreases significantly at the fiber ends where micro-void nucleation is experimentally observed to occur. Our approach provides the fiber surface pressure distribution in simple shear flow that typifies nozzle regions with extreme flow conditions, enhancing our understanding of micro-void development mechanisms as the polymer melt flows through the nozzle.more » « less
-
The presence of voids within the microstructure of short carbon fiber polymer composites produced by additive manufacturing (AM) technology are known to alter the expected material behavior that impair part performance. Previous research efforts aimed at understanding the formation mechanisms of these micro-voids during the polymer extrusion/deposition process have not kept up with the advancement of this AM technology. The present study investigates the phenomenon of micro-void nucleation at the fiber/matrix interface, especially those that form at fiber tips, by characterizing the microstructural configuration of a 13 % carbon fiber filled ABS polymer composite print bead specimen using 3D X-ray micro computed tomography image acquisition and analysis. The results reveal a high level of micro-voids segregation at the ends of fibers that are relatively larger in size and less spherical as compared to micro-voids isolated within the ABS matrix. Additionally, by simulating the hydrostatic flow-field pressure distribution surrounding a single rigid ellipsoidal fibre in colloidal suspension using Jeffery’s model equations, we show that the pressure drops to a critical value at the fibre tips where the micro-voids nucleation is experimentally observed to occur. The study helps to improve our understanding of the potential mechanisms that may be responsible for micro-void development within beads printed with extrusion/ deposition AM.more » « less
-
Short carbon fiber-reinforced composite materials produced by large-area additive manufacturing (LAAM) are attractive due to their lightweight, favorable mechanical properties, multifunctional applications, and low manufacturing costs. However, the physical and mechanical properties of short carbon-fiber-reinforced composites 3D printed via LAAM systems remain below expectations due in part to the void formation within the bead microstructure. This study aimed to assess void characteristics including volume fraction and sphericity within the microstructure of 13 wt% short carbon fiber acrylonitrile butadiene styrene (SCF/ABS). Our study evaluated SCF/ABS as a pellet, a single freely extruded strand, a regularly deposited single bead, and a single bead manufactured with a roller during the printing process using a high-resolution 3D micro-computed tomography (µCT) system. Micro voids were shown to exist within the microstructure of the SCF/ABS pellet and tended to become more prevalent in a single freely extruded strand which showed the highest void volume fraction among all the samples studied. Results also showed that deposition on the print bed reduced the void volume fraction and applying a roller during the printing process caused a further reduction in the void volume fraction. This study also reports the void’s shape within the microstructure in terms of sphericity which indicated that SCF/ABS single freely extruded strands had the highest mean void sphericity (voids tend to be more spherical). Moreover, this study evaluated the effect of printing process parameters, including nozzle temperature, extrusion speed and nozzle height above the printing table on the void volume fraction and sphericity within the microstructure of regularly deposited single beads.more » « less
An official website of the United States government

