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Title: Softening of a flat phonon mode in the kagome ScV6Sn6
Abstract

Geometrically frustrated kagome lattices are raising as novel platforms to engineer correlated topological electron flat bands that are prominent to electronic instabilities. Here, we demonstrate a phonon softening at thekz = πplane in ScV6Sn6. The low energy longitudinal phonon collapses at ~98 K andq = $$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$131312due to the electron-phonon interaction, without the emergence of long-range charge order which sets in at a different propagation vectorqCDW = $$\frac{1}{3}\frac{1}{3}\frac{1}{3}$$131313. Theoretical calculations corroborate the experimental finding to indicate that the leading instability is located at$$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$131312of a rather flat mode. We relate the phonon renormalization to the orbital-resolved susceptibility of the trigonal Sn atoms and explain the approximately flat phonon dispersion. Our data report the first example of the collapse of a kagome bosonic mode and promote the 166 compounds of kagomes as primary candidates to explore correlated flat phonon-topological flat electron physics.

 
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Award ID(s):
2011750
NSF-PAR ID:
10508186
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;
Publisher / Repository:
Nature Communication
Date Published:
Journal Name:
Nature Communications
Volume:
14
Issue:
1
ISSN:
2041-1723
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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