This content will become publicly available on May 31, 2025
- Award ID(s):
- 2312311
- NSF-PAR ID:
- 10515515
- Publisher / Repository:
- Nature Review Materials
- Date Published:
- Journal Name:
- Nature Reviews Materials
- ISSN:
- 2058-8437
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
null (Ed.)In moiré crystals formed by stacking van der Waals materials, surprisingly diverse correlated electronic phases and optical properties can be realized by a subtle change in the twist angle. Here, we discover that phonon spectra are also renormalized in MoS2 twisted bilayers, adding an insight to moiré physics. Over a range of small twist angles, the phonon spectra evolve rapidly owing to ultra-strong coupling between different phonon modes and atomic reconstructions of the moiré pattern. We develop a low-energy continuum model for phonons that overcomes the outstanding challenge of calculating the properties of large moiré supercells and successfully captures the essential experimental observations. Remarkably, simple optical spectroscopy experiments can provide information on strain and lattice distortions in moiré crystals with nanometre-size supercells. The model promotes a comprehensive and unified understanding of the structural, optical and electronic properties of moiré superlattices.more » « less
-
Topological mosaic pattern (TMP) can be formed in two-dimensional (2D) moiré superlattices, a set of periodic and spatially separated domains with distinct topologies that give rise to periodic edge states on the domain walls. In this study, we demonstrate that these periodic edge states play a crucial role in determining global topological properties. By developing a continuum model for periodic edge states with 𝐶6𝑧 and 𝐶3𝑧 rotational symmetry, we predict that a global topological phase transition at the charge neutrality point (CNP) can be driven by the size of domain walls and moiré period. The Wannier representation analysis reveals that these periodic edge states are fundamentally chiral 𝑝𝑥±𝑖𝑝𝑦 orbitals. The interplay between on-site chiral orbital rotation and neighboring hopping among chiral orbitals leads to band inversion and a topological phase transition. Our work establishes a general model for tuning local and global topological phases, paving the way for future research on strongly correlated topological flat minibands within topological mosaic patterns.more » « less
-
Transition metal dichalcogenide (TMD) moiré superlattices have emerged as a significant area of study in condensed matter physics. Thanks to their superior optical properties, tunable electronic band structure, strong Coulomb interactions, and quenched electron kinetic energy, they offer exciting avenues to explore correlated quantum phenomena, topological properties, and light–matter interactions. In recent years, scanning tunneling microscopy (STM) has made significant impacts on the study of these fields by enabling intrinsic surface visualization and spectroscopic measurements with unprecedented atomic scale detail. Here, we spotlight the key findings and innovative developments in imaging and characterization of TMD heterostructures via STM, from its initial implementation on the in situ grown sample to the latest photocurrent tunneling microscopy. The evolution in sample design, progressing from a conductive to an insulating substrate, has not only expanded our control over TMD moiré superlattices but also promoted an understanding of their structures and strongly correlated properties, such as the structural reconstruction and formation of generalized two-dimensional Wigner crystal states. In addition to highlighting recent advancements, we outline upcoming challenges, suggest the direction of future research, and advocate for the versatile use of STM to further comprehend and manipulate the quantum dynamics in TMD moiré superlattices.more » « less
-
Flat-band materials such as the kagome metals or moiré superlattices are of intense current interest. Flat bands can result from the electron motion on numerous (special) lattices and usually exhibit topological properties. Their reduced bandwidth proportionally enhances the effect of Coulomb interaction, even when the absolute magnitude of the latter is relatively small. Seemingly unrelated to these materials is the large family of strongly correlated electron systems, which include the heavy-fermion compounds, and cuprate and pnictide superconductors. In addition to itinerant electrons from large, strongly overlapping orbitals, they frequently contain electrons from more localized orbitals, which are subject to a large Coulomb interaction. The question then arises as to what commonality in the physical properties and microscopic physics, if any, exists between these two broad categories of materials. A rapidly increasing body of strikingly similar phenomena across the different platforms — from electronic localization–delocalization transitions to strange-metal behaviour and unconventional superconductivity — suggests that similar underlying principles could be at play. Indeed, it has recently been suggested that flat-band physics can be understood in terms of Kondo physics. Inversely, the concept of electronic topology from lattice symmetry, which is fundamental in flat-band systems, is enriching the field of strongly correlated electron systems, in which correlation-driven topological phases are increasingly being investigated. In this Perspective article, we elucidate this connection, survey the new opportunities for cross-fertilization across platforms and assess the prospect for new insights that may be gained into correlation physics and its intersection with electronic topology.more » « less
-
Abstract Moiré potential profile can form flat electronic bands and manifest correlated states of electrons, where carrier doping is essential for observing those correlations. In this work, we uncover a hidden but remarkable many-electron effect: doped carriers form a two-dimensional plasmon and strongly couple with quasiparticles to renormalize moiré potential and realize ultra-flat bands. Using many-body perturbation theory, we demonstrate this effect in twisted MoS2/WS2heterobilayer. The moiré potential is significantly enhanced upon carrier doping, and the bandwidth is reduced by order of magnitude, leading to drastic quenching of electronic kinetic energy and stronger correlation. We further predict that the competition between correlated mechanisms can be effectively controlled via doping, giving hope to a quantum transition between Mott and charge-transfer insulating states. Our work reveals that the potential renormalization effect of doping is much more significant in determining and controlling many-electron electronic correlations than sole filling-factor tuning in semiconducting moiré crystals.