Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties of ice clouds. In this work, we develop a novel method that differentiates between various phases of mixed-phase clouds, such as clouds dominated by pure liquid or pure ice segments, compared with those having ice crystals surrounded by supercooled liquid water droplets or vice versa. Using this method, we examine the relationship between the macrophysical and microphysical properties of Southern Ocean mixed-phase clouds at −40 to 0 °C (e.g. stratiform and cumuliform clouds) based on the in situ aircraft-based observations during the US National Science Foundation Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. The results show that the exchange between supercooled liquid water and ice crystals from a macrophysical perspective, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the phase exchange from a microphysical perspective, represented by the increasing ice water content (IWC), decreasing liquid water content (LWC), increasing ice mass fraction, and increasing ice particle number fraction (IPNF). The mass exchange between liquid and ice becomes more significant during phase 3 when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show a significant phase change from liquid to ice at a similar temperature (i.e. −17.5 °C) among three types of definitions of mixed-phase clouds based on ice spatial ratio, ice mass fraction, or IPNF. Aerosol indirect effects are quantified for different phases using number concentrations of aerosols greater than 100 or 500 nm (N>100 and N>500, respectively). N>500 shows stronger positive correlations with ice spatial ratios compared with N>100. This result indicates that larger aerosols potentially contain ice-nucleating particles (INPs), which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N>500 is also more significant in phase 2 when ice crystals just start to appear in the mixed phase compared with phase 3 when pure ICRs have formed, possibly due to the competing aerosol indirect effects on primary and secondary ice production in phase 3. The thermodynamic and dynamic conditions are quantified for each phase. The results show stronger in-cloud turbulence and higher updraughts in phases 2 and 3 when liquid and ice coexist compared with pure liquid or ice (phases 1 and 4, respectively). The highest updraughts and turbulence are seen in phase 3 when supercooled liquid droplets are surrounded by ice crystals. These results indicate both updraughts and turbulence support the maintenance of supercooled liquid water amongst ice crystals. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics through various stages of mixed-phase cloud evolution based on this new method that categorizes cloud phases.
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An Evaluation of Phase, Aerosol-Cloud Interactions and Microphysical Properties of Single- and Multi-Layer Clouds Over the Southern Ocean Using in Situ Observations From SOCRATES
Single- and multi-layer clouds are commonly observed over the Southern Ocean in varying synoptic settings, yet few studies have characterized and contrasted their properties. This study provides a statistical analysis of the microphysical properties of single- and multi-layer clouds using in-situ observations acquired during the Southern Ocean Cloud-Radiation Aerosol Transport Experimental Study. The relative frequencies of ice-containing samples (i.e., mixed and ice phase) for multi-layer clouds are 0.05–0.25 greater than for single-layer clouds, depending on cloud layer height. In multi-layer clouds, the lowest cloud layers have the highest ice-containing sample frequencies, which decrease with increasing cloud layer height up to the third highest cloud layer. This suggests a prominent seeder-feeder mechanism over the region. Ice nucleating particle (cloud condensation nuclei) concentrations are positively (negatively) correlated with ice-containing sample frequencies in select cases. Differences in microphysical properties are observed for single- and multi-layer clouds. Drop concentrations (size distributions) are greater (narrower) for single-layer clouds compared with the lowest multi-layer clouds. When differentiating cloud layers by top (single- and highest multi-layer clouds) and non-top layers (underlying multi-layer clouds), total particle size distributions (including liquid and ice) are similarly broader for non-top cloud layers. Additionally, drop concentrations in coupled environments are approximately double those in decoupled environments.
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- Award ID(s):
- 1744965
- PAR ID:
- 10542147
- Publisher / Repository:
- Wiley Publishing - AGU journals
- Date Published:
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Volume:
- 128
- Issue:
- 15
- ISSN:
- 2169-8996
- Page Range / eLocation ID:
- e2023JD038610
- Subject(s) / Keyword(s):
- Southern Ocean cloud microphysics aerosol-cloud interactions
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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