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1. Partition between supercooled liquid droplets and ice crystals in mixed-phase clouds based on airborne in situ observations

   https://doi.org/10.5194/amt-17-4843-2024  

   Maciel, Flor Vanessa; Diao, Minghui; Yang, Ching An (August 2024, Atmospheric Measurement Techniques)

   Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties of ice clouds. In this work, we develop a novel method that differentiates between various phases of mixed-phase clouds, such as clouds dominated by pure liquid or pure ice segments, compared with those having ice crystals surrounded by supercooled liquid water droplets or vice versa. Using this method, we examine the relationship between the macrophysical and microphysical properties of Southern Ocean mixed-phase clouds at −40 to 0 °C (e.g. stratiform and cumuliform clouds) based on the in situ aircraft-based observations during the US National Science Foundation Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. The results show that the exchange between supercooled liquid water and ice crystals from a macrophysical perspective, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the phase exchange from a microphysical perspective, represented by the increasing ice water content (IWC), decreasing liquid water content (LWC), increasing ice mass fraction, and increasing ice particle number fraction (IPNF). The mass exchange between liquid and ice becomes more significant during phase 3 when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show a significant phase change from liquid to ice at a similar temperature (i.e. −17.5 °C) among three types of definitions of mixed-phase clouds based on ice spatial ratio, ice mass fraction, or IPNF. Aerosol indirect effects are quantified for different phases using number concentrations of aerosols greater than 100 or 500 nm (N>100 and N>500, respectively). N>500 shows stronger positive correlations with ice spatial ratios compared with N>100. This result indicates that larger aerosols potentially contain ice-nucleating particles (INPs), which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N>500 is also more significant in phase 2 when ice crystals just start to appear in the mixed phase compared with phase 3 when pure ICRs have formed, possibly due to the competing aerosol indirect effects on primary and secondary ice production in phase 3. The thermodynamic and dynamic conditions are quantified for each phase. The results show stronger in-cloud turbulence and higher updraughts in phases 2 and 3 when liquid and ice coexist compared with pure liquid or ice (phases 1 and 4, respectively). The highest updraughts and turbulence are seen in phase 3 when supercooled liquid droplets are surrounded by ice crystals. These results indicate both updraughts and turbulence support the maintenance of supercooled liquid water amongst ice crystals. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics through various stages of mixed-phase cloud evolution based on this new method that categorizes cloud phases. 

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2. Cloud Microphysical Properties based on Airborne In Situ Observations and Evaluation of a Weather Forecasting Model and a Global Climate Model

   https://doi.org/https://doi.org/10.31979/etd.7855-fqvh  

   D'Alessandro, John (August 2018, Master’s theses directories)

   Global cloud coverage has a substantial impact on local and global radiative budgets. It is necessary to correctly represent clouds in numerical weather models to improve both weather and climate predictions. This study evaluates in situ airborne observations of cloud microphysical properties and compares results with the Weather Research and Forecasting model (WRF) and Community Atmosphere Model version 5 (CAM5). Dynamical conditions producing supersaturated conditions with respect to ice at high altitudes in regions diagnosed by convective activity are explored using observations taken from the Deep Convective Clouds and Chemistry (DC3) campaign, and results are compared with simulated data from WRF. The WRF analysis tests multiple cloud microphysics schemes and finds the model requires much stronger updrafts to initiate large magnitudes of ice supersaturation (ISS) relative to observations. This is primarily due to the microphysics schemes over-predicting ice particle number concentrations (Ncice), which rapidly deplete the available water vapor. The frequency of different cloud phases and the distribution of relative humidity (RH) over the Southern Ocean is explored using in situ airborne observations taken from the O2/N2 Ratio and CO2 Airborne Southern Ocean Study (ORCAS) and compared with simulated data from CAM5. The CAM5 simulations produce comparable distributions of RH in clear-sky conditions at warmer temperatures (>-20°C). However, simulations fail to capture high frequencies of clear-sky ISS at colder temperatures (< 40°C). In addition, CAM5 underestimates the frequency of subsaturated conditions within ice phase clouds from -40°‒0°C. 

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3. Tethered balloon-borne profile measurements of atmospheric properties in the cloudy atmospheric boundary layer over the Arctic sea ice during MOSAiC: Overview and first results

   https://doi.org/10.1525/elementa.2021.000120  

   Lonardi, Michael; Pilz, Christian; Akansu, Elisa F.; Dahlke, Sandro; Egerer, Ulrike; Ehrlich, André; Griesche, Hannes; Heymsfield, Andrew J.; Kirbus, Benjamin; Schmitt, Carl G.; et al (January 2022, Elementa: Science of the Anthropocene)

   The tethered balloon-borne measurement system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) was deployed over the Arctic sea ice for 4 weeks in summer 2020 as part of the Multidisciplinary drifting Observatory for the Study of Arctic Climate expedition. Using BELUGA, vertical profiles of dynamic, thermodynamic, aerosol particle, cloud, radiation, and turbulence properties were measured from the ground up to a height of 1,500 m. BELUGA was operated during an anomalously warm period with frequent liquid water clouds and variable sea ice conditions. Three case studies of liquid water phase, single-layer clouds observed on 3 days (July 13, 23, and 24, 2020) are discussed to show the potential of the collected data set to comprehensively investigate cloud properties determining cloud evolution in the inner Arctic over sea ice. Simulated back-trajectories show that the observed clouds have evolved within 3 different air masses (“aged Arctic,” “advected over sea ice,” and “advected over open ocean”), which left distinct fingerprints in the cloud properties. Strong cloud top radiative cooling rates agree with simulated results of previous studies. The weak warming at cloud base is mostly driven by the vertical temperature profile between the surface and cloud base. In-cloud turbulence induced by the cloud top cooling was similar in strength compared to former studies. From the extent of the mixing layer, it is speculated that the overall cloud cooling is stronger and thus faster in the warm oceanic air mass. Larger aerosol particle number concentrations and larger sizes were observed in the air mass advected over the sea ice and in the air mass advected over the open ocean. 

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4. Characterizing Ice Nucleating Particles Over the Southern Ocean Using Simultaneous Aircraft and Ship Observations

   https://doi.org/10.1029/2023JD039543  

   Moore, Kathryn A; Hill, Thomas_C J; McCluskey, Christina S; Twohy, Cynthia H; Rainwater, Bryan; Toohey, Darin W; Sanchez, Kevin J; Kreidenweis, Sonia M; DeMott, Paul J (January 2024, Journal of Geophysical Research: Atmospheres)

   Abstract Supercooled liquid clouds are ubiquitous over the Southern Ocean (SO), even to temperatures below −20°C, and comprise a large fraction of the marine boundary layer (MBL) clouds. Earth system models and reanalysis products have struggled to reproduce the observed cloud phase distribution and occurrence of cloud ice in the region. Recent simulations found the microphysical representation of ice nucleation and growth has a large impact on these properties, however, measurements of SO ice nucleating particles (INPs) to validate simulations are sparse. This study presents measurements of INPs from simultaneous aircraft and ship campaigns conducted over the SO in austral summer 2018, which include the first in situ observations in and above cloud in the region. Our results confirm recent observations that INP concentrations are uniformly lower than measurements made in the late 1960s. While INP concentrations below and above cloud are similar, higher ice nucleation efficiency above cloud supports model simulations that the dominant INP composition varies with height. Model parameterizations based solely on aerosol properties capture the mean relationship between INP concentration and temperature but not the observed variability, which is likely related to the only modest correlations observed between INPs and environmental or aerosol metrics. Including wind speed in addition to activation temperature in a marine INP parameterization reduces bias but does not explain the large range of observed INP concentrations. Direct and indirect inference of marine INP size suggests MBL INPs, at least during Austral summer, are dominated by particles with diameters smaller than 500 nm. 

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5. Precipitation Growth Processes in the Comma-Head Region of the 7 February 2020 Northeast Snowstorm: Results from IMPACTS

   https://doi.org/10.1175/JAS-D-22-0118.1  

   Varcie, Megan M.; Zaremba, Troy J.; Rauber, Robert M.; McFarquhar, Greg M.; Finlon, Joseph A.; McMurdie, Lynn A.; Ryzhkov, Alexander; Schnaiter, Martin; Järvinen, Emma; Waitz, Fritz; et al (January 2023, Journal of the Atmospheric Sciences)

   Abstract On 7 February 2020, precipitation within the comma-head region of an extratropical cyclone was sampled remotely and in situ by two research aircraft, providing a vertical cross section of microphysical observations and fine-scale radar measurements. The sampled region was stratified vertically by distinct temperature layers and horizontally into a stratiform region on the west side, and a region of elevated convection on the east side. In the stratiform region, precipitation formed near cloud top as side-plane, polycrystalline, and platelike particles. These habits occurred through cloud depth, implying that the cloud-top region was the primary source of particles. Almost no supercooled water was present. The ice water content within the stratiform region showed an overall increase with depth between the aircraft flight levels, while the total number concentration slightly decreased, consistent with growth by vapor deposition and aggregation. In the convective region, new particle habits were observed within each temperature-defined layer along with detectable amounts of supercooled water, implying that ice particle formation occurred in several layers. Total number concentration decreased from cloud top to the −8°C level, consistent with particle aggregation. At temperatures > −8°C, ice particle concentrations in some regions increased to >100 L −1 , suggesting secondary ice production occurred at lower altitudes. WSR-88D reflectivity composites during the sampling period showed a weak, loosely organized banded feature. The band, evident on earlier flight legs, was consistent with enhanced vertical motion associated with frontogenesis, and at least partial melting of ice particles near the surface. A conceptual model of precipitation growth processes within the comma head is presented. Significance Statement Snowstorms over the northeast United States have major impacts on travel, power availability, and commerce. The processes by which snow forms in winter storms over this region are complex and their snowfall totals are hard to forecast accurately because of a poor understanding of the microphysical processes within the clouds composing the storms. This paper presents a case study from the NASA IMPACTS field campaign that involved two aircraft sampling the storm simultaneously with radars, and probes that measure the microphysical properties within the storm. The paper examines how variations in stability and frontal structure influence the microphysical evolution of ice particles as they fall from cloud top to the surface within the storm. 

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