skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Attention:

The NSF Public Access Repository (PAR) system and access will be unavailable from 11:00 PM ET on Friday, May 2 until 12:00 AM ET on Saturday, May 3 due to maintenance. We apologize for the inconvenience.


Title: A spin-refrigerated cavity quantum electrodynamic sensor
Abstract Quantum sensors based on solid-state defects, in particular nitrogen-vacancy (NV) centers in diamond, enable precise measurement of magnetic fields, temperature, rotation, and electric fields. Cavity quantum electrodynamic (cQED) readout, in which an NV ensemble is hybridized with a microwave mode, can overcome limitations in optical spin detection and has resulted in leading magnetic sensitivities at the pT-level. This approach, however, remains far from the intrinsic spin-projection noise limit due to thermal Johnson-Nyquist noise and spin saturation effects. Here we tackle these challenges by combining recently demonstrated spin refrigeration techniques with comprehensive nonlinear modeling of the cQED sensor operation. We demonstrate that the optically-polarized NV ensemble simultaneously provides magnetic sensitivity and acts as a heat sink for the deleterious thermal microwave noise background, even when actively probed by a microwave field. Optimizing the NV-cQED system, we demonstrate a broadband sensitivity of 576 ± 6 fT/$$\sqrt{{{{\rm{Hz}}}}}$$ Hz around 15 kHz in ambient conditions. We then discuss the implications of this approach for the design of future magnetometers, including near-projection-limited devices approaching 3 fT/$$\sqrt{{{{\rm{Hz}}}}}$$ Hz sensitivity enabled by spin refrigeration.  more » « less
Award ID(s):
2317134
PAR ID:
10557242
Author(s) / Creator(s):
; ; ; ; ; ;
Publisher / Repository:
Nature Publishing Group
Date Published:
Journal Name:
Nature Communications
Volume:
15
Issue:
1
ISSN:
2041-1723
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract Spin defects in van der Waals materials offer a promising platform for advancing quantum technologies. Here, we propose and demonstrate a powerful technique based on isotope engineering of host materials to significantly enhance the coherence properties of embedded spin defects. Focusing on the recently-discovered negatively charged boron vacancy center ($${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B ) in hexagonal boron nitride (hBN), we grow isotopically purified h10B15N crystals. Compared to$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B in hBN with the natural distribution of isotopes, we observe substantially narrower and less crowded$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B spin transitions as well as extended coherence timeT2and relaxation timeT1. For quantum sensing,$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B centers in our h10B15N samples exhibit a factor of 4 (2) enhancement in DC (AC) magnetic field sensitivity. For additional quantum resources, the individual addressability of the$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B hyperfine levels enables the dynamical polarization and coherent control of the three nearest-neighbor15N nuclear spins. Our results demonstrate the power of isotope engineering for enhancing the properties of quantum spin defects in hBN, and can be readily extended to improving spin qubits in a broad family of van der Waals materials. 
    more » « less
  2. Abstract Optically active spin defects in van der Waals materials are promising platforms for modern quantum technologies. Here we investigate the coherent dynamics of strongly interacting ensembles of negatively charged boron-vacancy ($${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B ) centers in hexagonal boron nitride (hBN) with varying defect density. By employing advanced dynamical decoupling sequences to selectively isolate different dephasing sources, we observe more than 5-fold improvement in the measured coherence times across all hBN samples. Crucially, we identify that the many-body interaction within the$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B ensemble plays a substantial role in the coherent dynamics, which is then used to directly estimate the concentration of$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B . We find that at high ion implantation dosage, only a small portion of the created boron vacancy defects are in the desired negatively charged state. Finally, we investigate the spin response of$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B to the local charged defects induced electric field signals, and estimate its ground state transverse electric field susceptibility. Our results provide new insights on the spin and charge properties of$${{{{{{{{\rm{V}}}}}}}}}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ V B , which are important for future use of defects in hBN as quantum sensors and simulators. 
    more » « less
  3. Abstract LetXbe ann-element point set in thek-dimensional unit cube$$[0,1]^k$$ [ 0 , 1 ] k where$$k \ge 2$$ k 2 . According to an old result of Bollobás and Meir (Oper Res Lett 11:19–21, 1992) , there exists a cycle (tour)$$x_1, x_2, \ldots , x_n$$ x 1 , x 2 , , x n through thenpoints, such that$$\left( \sum _{i=1}^n |x_i - x_{i+1}|^k \right) ^{1/k} \le c_k$$ i = 1 n | x i - x i + 1 | k 1 / k c k , where$$|x-y|$$ | x - y | is the Euclidean distance betweenxandy, and$$c_k$$ c k is an absolute constant that depends only onk, where$$x_{n+1} \equiv x_1$$ x n + 1 x 1 . From the other direction, for every$$k \ge 2$$ k 2 and$$n \ge 2$$ n 2 , there existnpoints in$$[0,1]^k$$ [ 0 , 1 ] k , such that their shortest tour satisfies$$\left( \sum _{i=1}^n |x_i - x_{i+1}|^k \right) ^{1/k} = 2^{1/k} \cdot \sqrt{k}$$ i = 1 n | x i - x i + 1 | k 1 / k = 2 1 / k · k . For the plane, the best constant is$$c_2=2$$ c 2 = 2 and this is the only exact value known. Bollobás and Meir showed that one can take$$c_k = 9 \left( \frac{2}{3} \right) ^{1/k} \cdot \sqrt{k}$$ c k = 9 2 3 1 / k · k for every$$k \ge 3$$ k 3 and conjectured that the best constant is$$c_k = 2^{1/k} \cdot \sqrt{k}$$ c k = 2 1 / k · k , for every$$k \ge 2$$ k 2 . Here we significantly improve the upper bound and show that one can take$$c_k = 3 \sqrt{5} \left( \frac{2}{3} \right) ^{1/k} \cdot \sqrt{k}$$ c k = 3 5 2 3 1 / k · k or$$c_k = 2.91 \sqrt{k} \ (1+o_k(1))$$ c k = 2.91 k ( 1 + o k ( 1 ) ) . Our bounds are constructive. We also show that$$c_3 \ge 2^{7/6}$$ c 3 2 7 / 6 , which disproves the conjecture for$$k=3$$ k = 3 . Connections to matching problems, power assignment problems, related problems, including algorithms, are discussed in this context. A slightly revised version of the Bollobás–Meir conjecture is proposed. 
    more » « less
  4. Abstract Squeezed light has long been used to enhance the precision of a single optomechanical sensor. An emerging set of proposals seeks to use arrays of optomechanical sensors to detect weak distributed forces, for applications ranging from gravity-based subterranean imaging to dark matter searches; however, a detailed investigation into the quantum-enhancement of this approach remains outstanding. Here, we propose an array of entanglement-enhanced optomechanical sensors to improve the broadband sensitivity of distributed force sensing. By coherently operating the optomechanical sensor array and distributing squeezing to entangle the optical fields, the array of sensors has a scaling advantage over independent sensors (i.e.,$$\sqrt{M}\to M$$ M M , whereMis the number of sensors) due to coherence as well as joint noise suppression due to multi-partite entanglement. As an illustration, we consider entanglement-enhancement of an optomechanical accelerometer array to search for dark matter, and elucidate the challenge of realizing a quantum advantage in this context. 
    more » « less
  5. Abstract A search for decays to invisible particles of Higgs bosons produced in association with a top-antitop quark pair or a vector boson, which both decay to a fully hadronic final state, has been performed using proton-proton collision data collected at$${\sqrt{s}=13\,\text {Te}\hspace{-.08em}\text {V}}$$ s = 13 Te V by the CMS experiment at the LHC, corresponding to an integrated luminosity of 138$$\,\text {fb}^{-1}$$ fb - 1 . The 95% confidence level upper limit set on the branching fraction of the 125$$\,\text {Ge}\hspace{-.08em}\text {V}$$ Ge V Higgs boson to invisible particles,$${\mathcal {B}({\textrm{H}} \rightarrow \text {inv})}$$ B ( H inv ) , is 0.54 (0.39 expected), assuming standard model production cross sections. The results of this analysis are combined with previous$${\mathcal {B}({\textrm{H}} \rightarrow \text {inv})}$$ B ( H inv ) searches carried out at$${\sqrt{s}=7}$$ s = 7 , 8, and 13$$\,\text {Te}\hspace{-.08em}\text {V}$$ Te V in complementary production modes. The combined upper limit at 95% confidence level on$${\mathcal {B}({\textrm{H}} \rightarrow \text {inv})}$$ B ( H inv ) is 0.15 (0.08 expected). 
    more » « less