skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


This content will become publicly available on November 27, 2025

Title: Ultrafast Nematic Dynamics of FeSe Film
Femtosecond spectroscopy of FeSe film shows distinct transient nematic behavior below and above superconducting critical temperature. Results reveal correlations between photoinduced nematicity, quasiparticle formation, superconducting and pseudogap openings, emphasizing electronic correlations and preformed electron pairing.  more » « less
Award ID(s):
1905691
PAR ID:
10558099
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
Optica Publishing Group
Date Published:
ISBN:
978-1-957171-95-1
Page Range / eLocation ID:
JTu5A.14
Format(s):
Medium: X
Location:
Denver, Colorado
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract The class ofAV3Sb5(A=K, Rb, Cs) kagome metals hosts unconventional charge density wave states seemingly intertwined with their low temperature superconducting phases. The nature of the coupling between these two states and the potential presence of nearby, competing charge instabilities however remain open questions. This phenomenology is strikingly highlighted by the formation of two ‘domes’ in the superconducting transition temperature upon hole-doping CsV3Sb5. Here we track the evolution of charge correlations upon the suppression of long-range charge density wave order in the first dome and into the second of the hole-doped kagome superconductor CsV3Sb5−xSnx. Initially, hole-doping drives interlayer charge correlations to become short-ranged with their periodicity diminished along the interlayer direction. Beyond the peak of the first superconducting dome, the parent charge density wave state vanishes and incommensurate, quasi-1D charge correlations are stabilized in its place. These competing, unidirectional charge correlations demonstrate an inherent electronic rotational symmetry breaking in CsV3Sb5, and reveal a complex landscape of charge correlations within its electronic phase diagram. Our data suggest an inherent 2kfcharge instability and competing charge orders in theAV3Sb5class of kagome superconductors. 
    more » « less
  2. Abstract We study the ground state properties of the Hubbard model on three-leg triangular cylinders using large-scale density-matrix renormalization group simulations. At half-filling, we identify an intermediate gapless spin liquid phase, which has one gapless spin mode and algebraic spin–spin correlations but exponential decay scalar chiral–chiral correlations, between a metallic phase at weak coupling and Mott insulating dimer phase at strong interaction. Upon light doping the gapless spin liquid, the system exhibits power-law charge-density-wave (CDW) correlations but short-range single-particle, spin–spin, and chiral–chiral correlations. Similar to CDW correlations, the superconducting correlations also decay in power-law but oscillate in sign as a function of distance, which is consistent with the striped pair-density wave. When further doping the gapless spin liquid phase or doping the dimer order phase, another phase takes over, which has similar CDW correlations but all other correlations decay exponentially. 
    more » « less
  3. Modern computing and communication technologies such as supercomputers and the Internet are based on optically connected networks of microwave-frequency information processors. An analogous architecture has been proposed for quantum networks, using optical photons to distribute entanglement between remote superconducting quantum processors. Here we report a step towards such a network by observing non-classical correlations between photons in an optical link and a superconducting quantum device. We generate these states of light through a spontaneous parametric down-conversion process in a chip-scale piezo-optomechanical transducer, and we measure a microwave–optical cross-correlation exceeding the Cauchy–Schwarz classical bound for thermal states. As further evidence of the non-classical character of the microwave–optical photon pairs, we observe antibunching in the microwave state conditioned on detection of an optical photon. Such a transducer can be readily connected to an independent superconducting qubit module and serve as a key building block for optical quantum networks of microwave-frequency qubits. 
    more » « less
  4. Abstract A number of experiments have evidenced signatures of enhanced superconducting correlations after photoexcitation. Initially, these experiments were interpreted as resulting from quasi-static changes in the Hamiltonian parameters, for example, due to lattice deformations or melting of competing phases. Yet, several recent observations indicate that these conjectures are either incorrect or do not capture all the observed phenomena, which include reflectivity exceeding unity, large shifts of Josephson plasmon edges, and appearance of new peaks in terahertz reflectivity. These observations can be explained from the perspective of a Floquet theory involving a periodic drive of system parameters, but the origin of the underlying oscillations remains unclear. In this paper, we demonstrate that following incoherent photoexcitation, long-lived oscillations are generally expected in superconductors with low-energy Josephson plasmons, such as in cuprates or fullerene superconductor K 3 C 60 . These oscillations arise from the parametric generation of plasmon pairs due to pump-induced perturbation of the superconducting order parameter. We show that this bi-plasmon response can persist even above the transition temperature as long as strong superconducting fluctuations are present. Our analysis offers a robust framework to understand light-induced superconducting behavior, and the predicted bi-plasmon oscillations can be directly detected using available experimental techniques. 
    more » « less
  5. The quantitative description of correlated electron materials remains a modern computational challenge. We demonstrate a numerical strategy to simulate correlated materials at the fully ab initio level beyond the solution of effective low-energy models and apply it to gain a detailed microscopic understanding across a family of cuprate superconducting materials in their parent undoped states. We uncover microscopic trends in the electron correlations and reveal the link between the material composition and magnetic energy scales through a many-body picture of excitation processes involving the buffer layers. Our work illustrates a path toward a quantitative and reliable understanding of more complex states of correlated materials at the ab initio many-body level. 
    more » « less