An official website of the United States government
Nanosecond Pulsed High Frequency Discharges (NPHFD) are gaining popularity over conventional spark and arc discharges as they have been shown to increase energy efficiency, enhance ignition probability and sustained kernel growth, and offer more flexibility and control for ignition applications under various conditions. Hence, it is important to determine the impact of different factors such as the optimal pulse energy, background flow conditions, inter-pulse time, mixture equivalence ratio, etc. on the success of ignition of premixed mixtures with NPHFD. This work presents a numerical investigation of the morphology of ignition kernel development with both single-pulse and multiple-pulse discharges. Nanosecond non-equilibrium plasma discharges are modeled between pin-pin electrodes in a subsonic ignition tunnel with quiescent and flowing premixed mixtures of methane and air. Large eddy simulations (LES) are conducted to investigate the reasons for successful and failed ignition in different scenarios. A single pulse discharge in the presence of electrodes, in a quiescent medium, elucidates the gas recirculation pattern caused by the plasma pulse which results in a separated toroidal kernel from the primary ignition kernel between the electrodes. Convection heat loss to the mean flow results in quenching of the high temperature, radical-rich hot-spots creeping on the electrode walls, and leaving only the semi-toroidal kernel to propagate downstream. Finally, simulations with multiple pulses with different inter-pulse times have been conducted to analyze the synergistic effect of overlapping kernels with high temperature and OH concentration, which has been attributed as the primary reason for higher ignition probabilities in the “fully coupled” regime reported in the experiments. Successful ignition kernel formation is reported with 3 pulses at a pulse repetition frequency of 300 kHz in the fully coupled regime. This kernel volume was almost 4 times, and develops in two-thirds the time, compared to the ignition kernel volume formed by the single pulse discharge with the same total energy. Ten pulses with twice as much total energy were deposited at a much lower frequency of 2 kHz, which resulted in disjoint hot-spots that fail to form an ignition kernel in the decoupled regime.
more »
« less
Large eddy simulation of plasma assisted ignition: Effects of pulse repetition frequency, number of pulses, and pulse energy
The impacts of the pulse repetition frequency (PRF), number of pulses, and energy per pulse in a train of nanosecond discharge pulses on the ignition of a flowing lean premixed methane–air mixture are investigated using numerical simulations. A phenomenological plasma model coupled with a compressible reacting flow solver is used for these simulations. The simulation strategy has been well validated by comparing the experimental schlieren and OH planar laser induced fluorescence (PLIF) results with the numerical schlieren (i.e., density gradient) and OH density profiles, respectively. The characteristics of the ignition kernels produced by each discharge pulse and their interaction with each other as functions of the PRF are investigated. Three regimes were defined in the literature based on this interaction of the ignition kernels — fully coupled, partially coupled, and decoupled. This study uses numerical simulations to probe into the constructive and destructive effects, that ultimately determine ignition success, in these different regimes. The complete overlap of kernels and the complete lack of synergy between kernels produced by consecutive pulses are attributed to the success and failure of ignition and flame propagation in the fully coupled and decoupled regimes, respectively. In the partially coupled regime, the convection heat loss driven by the shock-turned-acoustic wave of the next discharge pulse, on the kernel produced by the previous discharge pulse, in addition to diffusion losses, contribute to ignition failure. However, the expansion of the next kernel in a region of higher average temperature and radical concentration created by the previous kernel could help to bridge the gap between the two kernels and result in successful ignition. The important parameters of energy per pulse, number of pulses, and equivalence ratio affect the competition between these constructive and destructive effects, which eventually determines the ignition success in this regime. Finally, the change in the nature of interaction between consecutive kernels from decoupled to partially coupled, at the same frequency but with different energies per pulse, is also shown.
more »
« less
- Award ID(s):
- 2002635
- PAR ID:
- 10562102
- Publisher / Repository:
- Elsevier
- Date Published:
- Journal Name:
- Combustion and Flame
- Volume:
- 267
- Issue:
- C
- ISSN:
- 0010-2180
- Page Range / eLocation ID:
- 113574
- Subject(s) / Keyword(s):
- Plasma assisted combustion Nanosecond repetitively pulsed plasma Pulse repetition frequency (PRF) Ignition Kernel development
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract The present work improves a phenomenological plasma-assisted combustion model by integrating the spatiotemporal distribution of plasma power density, thereby considering the evolution of plasma streamers in the modeling, and subsequently, better predicting the ignition kernel evolution. The improved phenomenological model is validated against experiments representing the plasma discharge and post-discharge ignition kernel evolution. Specifically, the new model demonstrates a more accurate prediction of ultrafast gas heating and O2dissociation during the plasma discharge, compared to the original model. In addition, the new model is found to closely match the experimental pressure wave and heated channel profiles post-discharge without the need for tuning the energy deposition (unlike the original model), highlighting its accuracy of post-discharge ignition kernel dynamics. The improved phenomenological model is then employed to investigate ignition kernel evolution for a stoichiometric methane-air discharge across various discharge gap configurations. Simulations reveal a non-uniform temperature and streamer distribution progressing from the electrode tips toward the center, contrasting uniform cylindrical discharges previously described in the original model. Streamer propagation is observed to be faster for larger gaps when maintained at the same average electric field for different discharge gaps. The tendency of smaller gaps to produce detached toroidal ignition kernels is observed, while larger gaps promote cylindrical and attached ignition kernels. Interactions between successive ignition kernels from consecutive discharges varied significantly, with the smallest gap (1 mm) promoting the quenching of the preceding ignition kernel due to the initial kernel–kernel separation. The intermediate gap (2 mm) promotes detached kernel growth. In contrast, in the largest gap (4 mm), kernels consistently combine and expand attached to electrodes. The impact of homogeneous isotropic turbulence is also explored, showing the persistence of ignition kernels early on but eventually quenching due to enhanced radical and heat losses with pronounced turbulence intensity.more » « less
-
Laminar burning speed calculation at high pressures is challenging because of unstable surface conditions at large flame kernel diameters. It is therefore desired to take these measurements at small dimensions (i.e., during and immediately after the ignition discharge process) when the flame kernel is smooth and stable. Taking accurate measurements at these sizes is challenging because the kernel growth rate does not only depend on the chemical reaction but also on other phenomena such as energy discharge, as well as radiative and conductive energy losses. The effect of these events has not been adequately assessed, due to the generation of ionized gas (i.e., plasma). In order to better understand the effect of the ignition plasma in this work, spark ignition in air for 1–5 atm of pressure is studied. Understanding the ignition event and modeling its behavior is important to capture accurate combustion measurements at pressures pertinent to the advanced high-pressure engines and technologies. The relationship between the electrical energy supplied to the spark and the thermal energy dissipated within a gas mixture has been studied. This work relates the electrical discharge power to the volume of the ignition kernel measured via schlieren imagery. Voltage and current data are also captured as the input to a thermodynamic model which is used to predict the volume versus time data of the spark event. The model, which utilizes measured electrical power, thermodynamic properties of ionized air, and radiation losses in air show agreement with the experimental kernel measurements in terms of overall shape of the volume data within the measured kernel uncertainty. With these results and further experimental validation the present model is considered to represent the relationship between the electrical spark power and the measured ignition kernel volume. Future work will be done to determine inaccuracies present in the arc discharge regime as well as the effectiveness of the model in combustible media.more » « less
-
Abstract Pulsed dielectric barrier discharges (DBD) in He–H 2 O and He–H 2 O–O 2 mixtures are studied in near atmospheric conditions using temporally and spatially resolved quantitative 2D imaging of the hydroxyl radical (OH) and hydrogen peroxide (H 2 O 2 ). The primary goal was to detect and quantify the production of these strongly oxidative species in water-laden helium discharges in a DBD jet configuration, which is of interest for biomedical applications such as disinfection of surfaces and treatment of biological samples. Hydroxyl profiles are obtained by laser-induced fluorescence (LIF) measurements using 282 nm laser excitation. Hydrogen peroxide profiles are measured by photo-fragmentation LIF (PF-LIF), which involves photo-dissociating H 2 O 2 into OH with a 212.8 nm laser sheet and detecting the OH fragments by LIF. The H 2 O 2 profiles are calibrated by measuring PF-LIF profiles in a reference mixture of He seeded with a known amount of H 2 O 2 . OH profiles are calibrated by measuring OH-radical decay times and comparing these with predictions from a chemical kinetics model. Two different burst discharge modes with five and ten pulses per burst are studied, both with a burst repetition rate of 50 Hz. In both cases, dynamics of OH and H 2 O 2 distributions in the afterglow of the discharge are investigated. Gas temperatures determined from the OH-LIF spectra indicate that gas heating due to the plasma is insignificant. The addition of 5% O 2 in the He admixture decreases the OH densities and increases the H 2 O 2 densities. The increased coupled energy in the ten-pulse discharge increases OH and H 2 O 2 mole fractions, except for the H 2 O 2 in the He–H 2 O–O 2 mixture which is relatively insensitive to the additional pulses.more » « less
-
Laminar flame speeds at high pressure are difficult to experimentally observe. Typically, high-pressure flame diagnostic is accomplished through observation of a spherically expanding flame in a constant volume chamber. However, flame instabilities at large radius and ignition effects at small radius limit measurable pressure range for Laminar flame speeds. Advanced combustion devices which operate at high pressures to improve capabilities and efficiencies require high quality laminar flame speed to aid in simulations and development. To expand the measurable range of flame data for high pressure flame measurement, this study proposes the further investigation of the ignition source and the incorporation of ignition diagnostics into the traditional flame speed analysis. To achieve this goal in future research, experimental spark propagation is observed and described in detail with the goal of improved experimental control and understanding. Parameters such as pressure, composition, electrode geometry and surface quality are discussed and the implication it has on the observed schlieren kernel propagation. Careful preparation of the ignition source can lead to improved surface and shape for future flame measurements. It is also shown that the thermal energy dissipated into the gas during discharge can be captured experimentally through measurement of the spark voltage, current and plasma sheath voltage drop. With the experimentally captured thermal energy, a simple energy balance can be used to describe the size of the observed ignition kernel for radius larger than 0.3 mm (following breakdown). The measurement of the thermal energy is described utilizing two experimental methods to find the discharge voltage of the nonequilibrium region at the boundary of the electrodes.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1016/j.combustflame.2024.113574
