An official website of the United States government
Abstract We model the pseudogap state of the hole- and electron-doped cuprates as a metal with hole and/or electron pocket Fermi surfaces. In the absence of long-range antiferromagnetism, such Fermi surfaces violate the Luttinger requirement of enclosing the same area as free electrons at the same density. Using the Ancilla theory of such a pseudogap state, we describe the onset of conventionald-wave superconductivity by the condensation of a chargeeHiggs boson transforming as a fundamental under the emergent SU(2) gauge symmetry of a backgroundπ-flux spin liquid. In all cases, we find that thed-wave superconductor has gapless Bogoliubov quasiparticles at 4 nodal points on the Brillouin zone diagonals with significant velocity anisotropy, just as in the BCS state. This includes the case of the electron-doped pseudogap metal with only electron pockets centered at wavevectors (π, 0), (0, π), and an electronic gap along the zone diagonals. Remarkably, in this case, too, gapless nodal Bogoliubov quasiparticles emerge within the gap at 4 points along the zone diagonals upon the onset of superconductivity.
more »
« less
Quantum oscillations in the hole-doped cuprates and the confinement of spinons
A long-standing problem in the study of the under-hole-doped cuprates has been the description of the Fermi surfaces underlying the high magnetic field quantum oscillations, and their connection to the higher temperature pseudogap metal. Harrison and Sebastian [Phys. Rev. Lett.106, 226402 (2011)] proposed that the pseudogap “Fermi arcs” are reconstructed into an electron pocket by field-induced charge density wave order. But computations on such a model [Zhang and Mei,Europhys. Lett.114, 47008 (2016)] show an unobserved additional oscillation frequency from a Fermi surface arising from the backsides of the hole pockets completing the Fermi arcs. We describe a transition from a fractionalized Fermi liquid (FL*) model of the pseudogap metal, to a metal with bidirectional charge density wave order without fractionalization. We show that the confinement of the fermionic spinon excitations of the FL* across this transition can eliminate the unobserved oscillation frequency.
more »
« less
- Award ID(s):
- 2245246
- PAR ID:
- 10573109
- Publisher / Repository:
- National Academy of Sciences
- Date Published:
- Journal Name:
- Proceedings of the National Academy of Sciences
- Volume:
- 121
- Issue:
- 50
- ISSN:
- 0027-8424
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Abstract The class ofAV3Sb5(A=K, Rb, Cs) kagome metals hosts unconventional charge density wave states seemingly intertwined with their low temperature superconducting phases. The nature of the coupling between these two states and the potential presence of nearby, competing charge instabilities however remain open questions. This phenomenology is strikingly highlighted by the formation of two ‘domes’ in the superconducting transition temperature upon hole-doping CsV3Sb5. Here we track the evolution of charge correlations upon the suppression of long-range charge density wave order in the first dome and into the second of the hole-doped kagome superconductor CsV3Sb5−xSnx. Initially, hole-doping drives interlayer charge correlations to become short-ranged with their periodicity diminished along the interlayer direction. Beyond the peak of the first superconducting dome, the parent charge density wave state vanishes and incommensurate, quasi-1D charge correlations are stabilized in its place. These competing, unidirectional charge correlations demonstrate an inherent electronic rotational symmetry breaking in CsV3Sb5, and reveal a complex landscape of charge correlations within its electronic phase diagram. Our data suggest an inherent 2kfcharge instability and competing charge orders in theAV3Sb5class of kagome superconductors.more » « less
-
Colossal negative magnetoresistance is a well-known phenomenon, notably observed in hole-doped ferromagnetic manganites. It remains a major research topic due to its potential in technological applications. In contrast, topological semimetals show large but positive magnetoresistance, originated from the high-mobility charge carriers. Here, we show that in the highly electron-doped region, the Dirac semimetal CeSbTe demonstrates similar properties as the manganites. CeSb0.11Te1.90hosts multiple charge density wave modulation vectors and has a complex magnetic phase diagram. We confirm that this compound is an antiferromagnetic Dirac semimetal. Despite having a metallic Fermi surface, the electronic transport properties are semiconductor-like and deviate from known theoretical models. An external magnetic field induces a semiconductor metal–like transition, which results in a colossal negative magnetoresistance. Moreover, signatures of the coupling between the charge density wave and a spin modulation are observed in resistivity. This spin modulation also produces a giant anomalous Hall response.more » « less
-
We describe the confining instabilities of a proposed quantum spin liquid underlying the pseudogap metal state of the hole-doped cuprates. The spin liquid can be described by a SU(2) gauge theory ofNf= 2 massless Dirac fermions carrying fundamental gauge charges—this is the low-energy theory of a mean-field state of fermionic spinons moving on the square lattice withπ-flux per plaquette in the ℤ2center of SU(2). This theory has an emergent SO(5)fglobal symmetry and is presumed to confine at low energies to the Néel state. At nonzero doping (or smaller Hubbard repulsionUat half-filling), we argue that confinement occurs via the Higgs condensation of bosonic chargons carrying fundamental SU(2) gauge charges also moving inπℤ2-flux. At half-filling, the low-energy theory of the Higgs sector hasNb= 2 relativistic bosons with a possible emergent SO(5)bglobal symmetry describing rotations between ad-wave superconductor, period-2 charge stripes, and the time-reversal breaking “d-density wave” state. We propose a conformal SU(2) gauge theory withNf= 2 fundamental fermions,Nb= 2 fundamental bosons, and a SO(5)f×SO(5)bglobal symmetry, which describes a deconfined quantum critical point between a confining state which breaks SO(5)fand a confining state which breaks SO(5)b. The pattern of symmetry breaking within both SO(5)s is determined by terms likely irrelevant at the critical point, which can be chosen to obtain a transition between Néel order andd-wave superconductivity. A similar theory applies at nonzero doping and largeU, with longer-range couplings of the chargons leading to charge order with longer periods.more » « less
-
Reactions of carbon with a heavy main group metal (M = Sb, Bi, or Te) in an excess of lanthanum/nickel eutectic flux lead to formation of a family of carbide compounds La3MC2with a new structure type. The monoclinic structure features C24−anions octahedrally coordinated by six La3+cations, andManions surrounded by 8 La3+cations. These compounds are not charge‐balanced and lie on the border between intermetallic carbides and mixed anion salts. Density of states calculations show a pseudogap at the Fermi level for La3BiC2, which indicates that this compound is a poor metal with optimized LaBi bonding interactions.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript
- Journal Article:
- https://doi.org/10.1073/pnas.2418633121
