Abstract Spin waves, collective dynamic magnetic excitations, offer crucial insights into magnetic material properties. Rare‐earth iron garnets offer an ideal spin‐wave (SW) platform with long propagation length, short wavelength, gigahertz frequency, and applicability to magnon spintronic platforms. Of particular interest, thulium iron garnet (TmIG) has attracted huge interest recently due to its successful growth down to a few nanometers, observed topological Hall effect, and spin‐orbit torque‐induced switching effects. However, there is no direct spatial measurement of its SW properties. This work uses diamond nitrogen‐vacancy (NV) magnetometry in combination with SW electrical transmission spectroscopy to study SW transport properties in TmIG thin films. NV magnetometry allows probing spin waves at the sub‐micrometer scale, seen by the amplification of the local microwave magnetic field due to the coupling of NV spin qubits with the stray magnetic field produced by the microwave‐excited spin waves. By monitoring the NV spin resonances, the SW properties in TmIG thin films are measured as a function of the applied magnetic field, including their amplitude, decay length (≈50 µm), and wavelength (0.8–2 µm). These results pave the way for studying spin qubit‐magnon interactions in rare‐earth magnetic insulators, relevant to quantum magnonics applications. 
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                            Parallel pumping of magnons in inhomogeneous spin textures probed through NV spin relaxometry
                        
                    
    
            We combine micromagnetic simulations and nitrogen-vacancy (NV) defect center spin relaxometry measurements to study magnon modes in inhomogeneous spin textures. A thin, micrometer-scale ferromagnetic disk is magnetized in a vortex state in which the magnetization curls around a central core. Micromagnetic simulations show that at zero applied field, the magnetization dynamics of the disk consist of a low frequency gyrotropic mode and higher frequency azimuthal magnon modes, all far detuned from the NV spin transition frequencies. An in-plane static magnetic field breaks the azimuthal symmetry of the vortex state, resulting in the magnon modes transforming in frequency and spatial profile as the field increases. Experimentally, we probe the dynamics of vortex magnetization as a function of applied in-plane static field and ac driving frequency by optically monitoring a nearby NV defect center spin. At certain values of the applied magnetic field, we observe enhanced spin relaxation when driving at twice the frequency of the NV ground state spin transition in optically detected magnetic resonance measurements. We attribute this effect to parallel pumping of a magnon mode in the disk producing magnons at half the excitation frequency. Micromagnetic simulations support this finding, showing spatial and spectral overlap of a confined magnon mode and an NV spin transition, with sufficient interaction strength to explain the observed signal. 
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                            - Award ID(s):
- 2326528
- PAR ID:
- 10593601
- Publisher / Repository:
- American Institute of Physics
- Date Published:
- Journal Name:
- Journal of Applied Physics
- Volume:
- 135
- Issue:
- 7
- ISSN:
- 0021-8979
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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