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Title: Fine structure splitting cancellation in highly asymmetric InAs/InP droplet epitaxy quantum dots
We find the fine structure splitting (FSS) of a single exciton, which splits its degenerate ground-state manifold into singlets, nearly vanishes in highly asymmetric quantum dots (QDs) due to the cancellation of splitting effects with markedly different origin. The dots simulated are those that emerge on top of etch pits through the droplet epitaxy growth process; these etch pit dots break square ( C 4 v ) spatial symmetry, which has been previously associated with small FSS. Configuration interaction calculations predict a vanishing FSS at a specific finite etch pit displacement from the center of the dot, for a structure far from square symmetry. We thus predict that highly asymmetric QDs may still display negligible FSS, providing avenues for high-fidelity generation of indistinguishable, polarization entangled photon pairs on demand. Published by the American Physical Society2024  more » « less
Award ID(s):
1921877
PAR ID:
10596142
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
American Physical Society
Date Published:
Journal Name:
Physical Review B
Volume:
109
Issue:
20
ISSN:
2469-9950
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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