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Complex ferromagnetic oxides have been identified as possible candidate materials for sources of spin currents. Here we study bilayers of ferromagnetic (La2/3Sr1/3)MnO3 (LSMO) and metallic CaRuO3 (CRO) on LSAT substrates as a model system for spin pumping. Ferromagnetic resonance (FMR) measurements of these bilayers show evidence of spin pumping across the interface in the form of an increase in Gilbert damping with the addition of CRO. FMR indicates that the presence of CRO modifies the magnetic anisotropy of the LSMO. By increasing CRO thickness, we find a reduction of the out-of-plane anisotropy and simultaneous rotation of the easy axis within the plane, from the ⟨110⟩ to ⟨100⟩ axis. The evolution of magnetic anisotropy determined by FMR disagrees with that measured by bulk SQUID magnetometry and is accompanied by structural distortions in the LSMO layer as measured by x-ray diffraction, thus suggesting a change in magnetic anisotropy attributed to structural distortions imposed on LSMO by CRO. These results suggest that while LSMO and CRO remain promising candidates for efficient pure spin current generation and detection, respectively, epitaxial integration of perovskites will cause additional changes which must be accounted for in spintronics applications.
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Determination of anisotropy constants via fitting of magnetic hysteresis to numerical calculation of Stoner–Wohlfarth model
Anisotropy constants of magnetic materials are typically determined through angle-resolved Ferromagnetic Resonance (ar-FMR) and torque magnetometry, which can be time consuming measurements, thus limiting their utility. The Stoner–Wohlfarth model can be used to numerically fit measured magnetic hysteresis curves to more easily determine these anisotropy constants. To demonstrate this, 10 nm bct FexCoyMnz single-crystal films grown by molecular beam epitaxy on MgO(001) substrates were investigated. The hysteresis behavior measured by vibrating sample magnetometry was least-squares fit against numerically calculated hysteresis curves generated from the Stoner–Wohlfarth model to extract the anisotropy constants. The cubic anisotropy of different compositions of FeCoMn films was at ∼104 J/m3, which is on the same order of magnitude of bct Fe and Co thin films measured by ar-FMR and torque magnetometry techniques.
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- Award ID(s):
- 1809846
- PAR ID:
- 10597290
- Publisher / Repository:
- American Institute of Physics
- Date Published:
- Journal Name:
- AIP Advances
- Volume:
- 11
- Issue:
- 8
- ISSN:
- 2158-3226
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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