Short carbon fiber-reinforced polymer composites are widely used in polymer extrusion additive manufacturing (AM), including large-area additive manufacturing (LAAM), due to their enhanced mechanical properties as compared to neat polymers. However, the mechanical properties of these composites depend on microstructural characteristics, including fibers and micro-voids, which are determined during processing. In this work, the correlation between fibers and micro-voids within the microstructure of LAAM polymer composites throughout various processing stages of short carbon fiber-reinforced acrylonitrile butadiene styrene (SCF/ABS) is investigated. The processing stages considered here include the incoming pellets, a single freely extruded strand, a single regularly deposited bead, and a single regularly deposited bead pressed by a mechanical roller. A high-resolution X-ray micro-computed tomography (µCT) system is employed to characterize the microstructural features in terms of the fibers (volume fraction, fiber orientation tensor) and micro-voids (volume fraction, sphericity) in the SCF/ABS samples. The results indicate that micro-voids exist within the microstructure of the SCF/ABS composite in all four stages considered here and that the micro-void volume fraction and micro-void sphericity vary among the test samples. Moreover, the results show a considerable variation in fiber orientation and fiber volume fraction within the microstructure throughout all the stages considered; however, all the samples show the highest alignment in the extrusion/print direction. Furthermore, a correlation is identified between the fiber orientation and the micro-void volume fraction within samples from all four stages considered here. This finding suggests that fibers tend to align more in the extrusion/print direction in regions with less micro-void content.
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Numerical modelling on polymer composites prepared via large area extrusion-deposition additive manufacturing: fibre orientation, material inhomogeneity, and thermal-mechanical responses during material loading process
The flow-induced fibre orientation formed during polymer extrusions causes the composite to exhibit non-homogeneous thermal-mechanical behaviours during Large Area extrusion deposition Additive Manufacturing (LAAM) processes. This study numerically evaluates the fibre orientation state of a 20 wt.% short carbon fibre reinforced polyethylenimine fabricated by LAAM. The fibre orientation state of the solidified deposited bead is determined by a fully coupled flow/orientation simulation approach. The material properties of deposited composites are computed by assuming that the deposited bead has heterogeneous regions with varying local fibre orientation states. A finite element simulation is performed to model the LAAM process of a thin-wall structure, where the predicted inhomogeneous material properties are employed. Computed results show notable differences between simulations performed by employing homogenous properties and those obtained using heterogeneous properties. The bead-direction tensile stress contours computed under the heterogeneous assumption are comparable to experimental data in the literature, supporting our numerical approach.
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- Award ID(s):
- 2055628
- PAR ID:
- 10608188
- Publisher / Repository:
- Taylor and Francis
- Date Published:
- Journal Name:
- Plastics, Rubber and Composites
- Volume:
- 52
- Issue:
- 8
- ISSN:
- 1465-8011
- Page Range / eLocation ID:
- 435 to 456
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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