The nuclear two-photon or double-gamma ( ) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to and half-lives as short as . The half-life for the decay of the first-excited state in bare ions was determined to be 23.9(6) ms, which strongly deviates from expectations. Published by the American Physical Society2024
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Enantioselective One-Photon Excitation of Formic Acid
We use one-photon excitation to promote -shell electrons of formic acid (which has a planar equilibrium structure) to an antibonding orbital. The excited molecule is known to have a (chiral) pyramidal equilibrium structure. In our experiment, we determine the handedness of the excited molecule by imaging the momenta of charged fragments, which occur after its Coulomb explosion triggered by Auger-Meitner decay cascades succeeding the excitation. We find that the handedness of the excited molecule depends on its spatial orientation with respect to the propagation (or polarization) direction of the exciting photon. The effect is largely independent of the exact polarization properties of the light driving the excitation. Published by the American Physical Society2024
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- Award ID(s):
- 2208017
- PAR ID:
- 10620980
- Publisher / Repository:
- American Physical Society
- Date Published:
- Journal Name:
- Physical Review Letters
- Volume:
- 133
- Issue:
- 9
- ISSN:
- 0031-9007
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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