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Spin-accumulation and spin-current profiles are calculated for a disordered Pt film subjected to an in-plane electric current within the nonequilibrium Green's function approach. In the bulklike region of the sample, this approach captures the intrinsic spin Hall effect found in other calculations. Near the surfaces, the results reveal qualitative differences with the results of the widely used spin-diffusion model, even when the boundary conditions are modified to try to account for them. One difference is that the effective spin-diffusion length for transverse spin transport is significantly different from its longitudinal counterpart and is instead similar to the mean-free path. This feature may be generic for spin currents generated via the intrinsic spin Hall mechanism because of the differences in transport mechanisms compared to longitudinal spin transport. Orbital accumulation in the Pt film is only significant in the immediate vicinity of the surfaces and has a small component penetrating into the bulk only in the presence of spin-orbit coupling, as a secondary effect induced by the spin accumulation.
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Determination of orbital relaxation in Ti/Ni heterostructure via orbital pumping
Orbital current has attracted significant attention in recent years due to its potential for energy-efficient magnetization control without the need for materials with strong spin–orbit coupling. However, the fundamental mechanisms governing orbital transport remain elusive. In this study, we systematically explore orbital transport in Ti/Ni bilayers through orbital pumping, drawing an analogy to spin pumping. The orbital current is generated and injected into the Ti layer via the microwave-driven orbital dynamics in Ni, facilitated by its strong spin–orbit correlation. We employed thickness-dependent ferromagnetic resonance measurements and angular-dependent inverse orbital Hall effect (IOHE) detection to probe orbital transport in Ti based on the conventional spin-pumping methodology. The observed enhancement in the damping factor indicates an orbital-diffusion length of ∼5.3 ± 3.7 nm, while IOHE-based estimation suggests a value of around 4.0 ± 1.2 nm, which confirms its short orbital-diffusion length. Furthermore, oblique Hanle measurements in the longitudinal configuration reveal an orbital relaxation time of approximately 16 ps. Our results establish that orbital pumping, analogous to the conventional spin-pumping framework, can serve as a robust technique for elucidating orbital transport mechanisms, paving the way for the design of efficient spin-orbitronic devices.
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- Award ID(s):
- 2011978
- PAR ID:
- 10637647
- Publisher / Repository:
- American Institute of Physics
- Date Published:
- Journal Name:
- Journal of Applied Physics
- Volume:
- 138
- Issue:
- 12
- ISSN:
- 0021-8979
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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